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APS

Cold atomic and molecular beams using buffer-gas cooling

Nathaniel Brahms, David R. Glenn, Robert deCarvalho, Scott V. Nguyen, D. Kielpinski, D. DeMille, John M. Doyle

Published May 1, 2004• 0 citations
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Intense Atomic and Molecular Beams Via Neon Buffer-gas Cooling

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We realize a continuous, intense, cold molecular and atomic beam source based on buffer-gas cooling. Hot vapor (up to 600 K) from an oven is mixed with cold (15 K) neon buffer gas, and then emitted into a high-flux beam. The novel use of cold neon as a buffer gas produces a forward velocity distribution and low-energy tail that is comparable to much colder helium-based sources. We expect this source to be trivially generalizable to a very wide range of atomic and molecular species with significant vapor pressure below 1000 K. The source has properties that make it a good starting point for laser cooling of molecules or atoms, cold collision studies, trapping, or nonlinear optics in buffer-gas-cooled atomic or molecular gases. A continuous guided beam of cold deuterated ammonia with a flux of 3×10\\(^{11}\\) ND\\(_{3}\\) molecules s\\(^{−1}\\) and a continuous free-space beam of cold potassium with a flux of 1×10\\(^{16}\\) K atoms s\\(^{−1}\\) are realized.

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A general cold atomic and molecular beam source

Stephen Maxwell, Nathaniel Brahms, Robert deCarvalho +5 more

We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by particles exiting a hole in the buffer gas cell. We characterize the properties of the beam (flux, forward velocity, temperature) for both an atom (Na) and a molecule (PbO) under varying buffer gas density, and discuss conditions for optimizing these beam parameters. Our source compares favorably to existing techniques of beam formation, for a variety of applications.

Bulletin of the American Physical Society•May 20, 2005•0 citations
We realize a continuous, intense, cold molecular and atomic beam source based on buffer-gas cooling. Hot vapor (up to 600 K) from an oven is mixed with cold (15 K) neon buffer gas, and then emitted into a high-flux beam. The novel use of cold neon as a buffer gas produces a forward velocity distribution and low-energy tail that is comparable to much colder helium-based sources. We expect this source to be trivially generalizable to a very wide range of atomic and molecular species with significant vapor pressure below 1000 K. The source has properties that make it a good starting point for laser cooling of molecules or atoms, cold collision studies, trapping, or nonlinear optics in buffer-gas-cooled atomic or molecular gases. A continuous guided beam of cold deuterated ammonia with a flux of 3×10\\(^{11}\\) ND\\(_{3}\\) molecules s\\(^{−1}\\) and a continuous free-space beam of cold potassium with a flux of 1×10\\(^{16}\\) K atoms s\\(^{−1}\\) are realized.
We realize a continuous, intense, cold molecular and atomic beam source based on buffer-gas cooling. Hot vapor (up to 600 K) from an oven is mixed with cold (15 K) neon buffer gas, and then emitted into a high-flux beam. The novel use of cold neon as a buffer gas produces a forward velocity distribution and low-energy tail that is comparable to much colder helium-based sources. We expect this source to be trivially generalizable to a very wide range of atomic and molecular species with significant vapor pressure below 1000 K. The source has properties that make it a good starting point for laser cooling of molecules or atoms, cold collision studies, trapping, or nonlinear optics in buffer-gas-cooled atomic or molecular gases. A continuous guided beam of cold deuterated ammonia with a flux of 3 × 10 11 ND 3 molecules s −1 and a continuous free-space beam of cold potassium with a flux of 1 × 10 16 K atoms s −1 are realized.
We demonstrate and characterize a high-flux beam source for cold, slow atoms or molecules. The desired species is vaporized using laser ablation, then cooled by thermalization in a cryogenic cell of buffer gas. The beam is formed by particles exiting a hole in the buffer gas cell. We characterize the properties of the beam (flux, forward velocity, temperature) for both an atom (Na) and a molecule (PbO) under varying buffer gas density, and discuss conditions for optimizing these beam parameters. Our source compares favorably to existing techniques of beam formation, for a variety of applications.