The use of noise-robust qubit encodings provides a way of extending the lifetime of quantum information at the hardware level. In this work, we introduce the spin Kerr-cat encoding, which leverages a sweet spot near a clock transition in the spectrum of quadrupolar nuclei (having spin
I≥1) to achieve a suppression of charge and magnetic noise leading to qubit dephasing. The basis states of the spin Kerr-cat qubit are given by the two lowest levels of a
Z2-symmetric nuclear-spin Hamiltonian and are well approximated by spin cat states for sufficiently high asymmetry parameters. For nuclei in highly asymmetric electric-field gradients, the nuclear spin could therefore be initialized in the spin-Kerr-cat subspace using SU(2) rotations and measurement rather than full SU(
2I+1) control. We calculate the dephasing time of the spin Kerr-cat qubit under a model of
1/f noise, as well as relaxation of the qubit due to breaking of the
Z2 symmetry by charge-noise-induced fluctuations of the quadrupolar tensor. Using measured parameters for antimony (
123Sb) donors in silicon, we estimate that second-scale
T2∗ times could be achieved with this encoding, with bitflips and leakage occurring on significantly longer timescales. We propose a two-qubit gate acting on spin Kerr-cat qubits and electron-spin qubits, enabled by adiabatically moving an electron on and off the donor potential. Based on numerical simulations, we estimate that with an enhancement of measured quadrupolar couplings by a factor of
≈2, a gate fidelity exceeding
99% could be achieved for spin Kerr cats encoded in
123Sb, with a gate time under
100 ns. By entangling the nuclear spin with an electron spin in this way, the spin Kerr-cat qubit could then be measured using a Pauli spin blockade readout of the electron.
Quantum computing promises exponential advantages for simulating quantum systems and solving certain computational problems beyond the reach of classical computers, but the fragility of qubits and the resulting errors present a major challenge for scalable implementations. One promising approach is to engineer qubits whose physical noise processes are intrinsically biased, enabling more efficient quantum error correction. This dissertation investigates quantum computing with superconducting Kerr-cat qubits, a bosonic qubit architecture in which qubit states are encoded in coherent states of a nonlinear oscillator stabilized by a two-photon drive. This stabilization creates an effective double-well pseudo-potential that strongly suppresses bit-flip errors while enabling universal quantum control, leading to a noise-biased qubit. A superconducting device architecture based on SNAIL nonlinear oscillators is developed to realize Kerr-cat qubits with tunable parameters and high coherence, integrating readout resonators, dedicated filters, and microwave control lines for measurement and manipulation. Universal single-qubit gates are implemented using engineered single-photon and two-photon drives to deform the pseudo-potential, and a cat-quadrature readout method is employed to achieve high-fidelity quantum nondemolition measurement. The performance of the qubits is systematically characterized through lifetime measurements and benchmarking protocols, including quantum process tomography, gate set tomography, and dihedral randomized benchmarking, revealing a strongly biased noise structure with high performance. These results establish an experimental framework for the design, control, and characterization of Kerr-cat qubits and demonstrate their potential as hardware-efficient building blocks for scalable fault-tolerant quantum computing.