Non-classical photons for long-distance quantum applications: from quantum frequency conversion to quantum dots emitting at 1550 nm (Conference Presentation)
Quantum dots reaching the best performances as non-classical light emitters are based on the GaAs platform. The main drawback is their natural emission wavelength, generally around 800-900 nm, so not suitable for fibre-based experiments. In this talk we will discuss two approaches to reach the telecom C-band, within the maximum transmission window of silica fibers. On the one hand, the use of quantum frequency conversion will enable the use of non-linear processes to transfer the high quality NIR photons to any other wavelength, here 1550 nm [1]. On the other hand, growth engineering can be utilized to modify size and strain conditions of the quantum dot, enabling the emission at telecom O- and C-band with the same dot stoichiometry as for the NIR ones [2]. [1] J. H. Weber, et al., Nat. Nanotechnol. 14, 23 (2019). [2] C. Nawrath et al., Appl. Phys. Lett. 115, 023103 (2019).
Quantum dots reaching the best performances as non-classical light emitters are based on the GaAs platform. The main drawback is their natural emission wavelength, generally around 800-900 nm, so not suitable for fibre-based experiments. In this talk we will discuss two approaches to reach the telecom C-band, within the maximum transmission window of silica fibers. On the one hand, the use of quantum frequency conversion will enable the use of non-linear processes to transfer the high quality NIR photons to any other wavelength, here 1550 nm [1]. On the other hand, growth engineering can be utilized to modify size and strain conditions of the quantum dot, enabling the emission at telecom O- and C-band with the same dot stoichiometry as for the NIR ones [2]. [1] J. H. Weber, et al., Nat. Nanotechnol. 14, 23 (2019). [2] C. Nawrath et al., Appl. Phys. Lett. 115, 023103 (2019).
Abstract Long-distance quantum communication and computation is based on the exchange of information via photons as flying qubits. In all foreseen implementations, from quantum relays and networks to remote quantum computing, the photons must be able to propagate over long distances, in silica fibers, with limited absorption and wave packet dispersion. When propagating into silica fibers, photons in the so-called telecom C-band (i.e. wavelength around 1550 nm) will experience the absolute minimum of absorption, together with a limited photon wave packet dispersion. This implies that losses of information will be minimized and additionally, the capability of the photons to quantum interfere (the so-called Hong–Ou–Mandel effect) will be negligibly affected. This motivated the search for efficient non-classical light sources in this wavelength range. In the present review, we discuss the approaches followed to red-shift the emission wavelength from the near-infrared (NIR) to telecom wavelengths. In particular, the use of metamorphic buffers (MMBs) enabled the use of highly developed InAs/GaAs systems, engineering the dots to emit single and entangled photons in the telecom C-band. The main advantage of this approach is set by the choice of the material system: being the same as state-of-the-art structures emitting in the NIR range, it opens the possibility of achieving comparable performances even at telecommunication wavelengths. Here we will discuss the current state-of-the-art in the generation of non-classical photons, comparing the properties and performances of MMB-based results with other competing quantum dot (QD) platforms. We report in particular that very low fine-structure splitting can be observed with conservative values, on average well below 10 μ eV. This allowed for the observation of post-selected entanglement fidelity higher than 0.6. Additionally, on-demand single-photon emission with g ( 0 ) 2 = 0.184 ± 0.002 was observed in addition to a very low emitter density of ≈ 10 7 cm − 2 and a decay time of τ ≈ 1.2 ns comparable to standard InAs QDs emitting in the NIR range. A final highlight on approaches to further improve the current device performances will also be reported.
Single-photon sources based on quantum dots have been shown to exhibit almost ideal properties such as high brightness and purity in terms of clear anti-bunching as well as high two-photon interference visibilities of the emitted photons, making them promising candidates for different quantum information applications such as quantum computing, quantum communication and quantum teleportation. However, as most single-photon sources also quantum dots typically emit light at wavelengths of electronic transitions within the visible or the near infrared range. In order to establish quantum networks with remote building blocks, low-loss single photons at telecom wavelengths are preferable, though. Despite recent progress on emitters of telecom-photons, the most efficient single-photon sources still work at shorter wavelengths. On that matter, quantum frequency down-conversion, being a nonlinear optical process, has been used in recent years to alter the wavelength of single photons to the telecom wavelength range while conserving their nonclassical properties. Characteristics such as lifetime, first-order coherence, anti-bunching and entanglement have been shown to be conserved or even improved due to background suppression during the conversion process, while the conservation of indistinguishability was yet to be shown. Here we present our experimental results on quantum frequency down-conversion of single photons emitted by an InAs/GaAs quantum dot at 903.6 nm following a pulsed excitation of a p-shell exciton at 884 nm. The emitted fluorescence photons are mixed with a strong pump-field at 2155 nm inside a periodically poled lithium niobate ridge waveguide and converted to 1557 nm. Common issues of a large background due to Raman-scattered pump-light photons spectrally overlapping with the converted single photons could largely be avoided, as the pump-wavelength was chosen to be fairly longer than the target wavelength. Additional narrowband spectral filtering at the telecom regime as a result of the small conversion bandwidth and using a high-performance fiber-Bragg-grating solely left the detector dark counts as the only noise source in our setup. Therefore, we could achieve conversion efficiencies of more than 20 %. In order to test the indistinguishability, sequentially emitted photons were fed into a Mach-Zehnder interferometer and spatially as well as temporally overlapped at the output beam splitter. Cross-correlation measurements between both output-ports of the beam splitter exhibit two-photon interference contrasts of more than 40 % prior to and after the down-conversion step. Accordingly, we demonstrate that the process of quantum frequency conversion preserves photon indistinguishability and can be used to establish a versatile source of indistinguishable single photons at the telecom C-Band. Furthermore our scheme allows for converting photons in a wavelength band from 900 nm to 910 nm to the same telecom target wavelength. This enables us to test indistinguishability of frequency-converted photons, originally stemming from different sources with dinstinguishable wavelengths.
Semiconductor quantum dots (QDs) are well established as sub-Poissonian sources of entangled photon pairs. To improve the utility of a QD light source, it would be advantageous to extend their emission further into the near infrared, into the low absorption wavelength windows utilised in long-haul optical telecommunication. Initial experiments succeeded in interfering O-band (1260—1360 nm) photons from an InAs/GaAs QD with dissimilar photons from a laser, an important mechanism for quantum teleportation. Interference visibilities as high as 60 ± 6 % were recorded, surpassing the 50 % threshold imposed by classical electrodynamics. Later, polarisation-entanglement of a similar QD was observed, with pairs of telecom-wavelength photons from the radiative cascade of the biexciton state exhibiting fidelities of 92.0 ± 0.2 % to the Bell state. Subsequently, an O-band telecom-wavelength quantum relay was realised. Again using an InAs/GaAs QD device, this represents the first implementation of a sub-Poissonian telecom-wavelength quantum relay, to the best knowledge of the author. The relay proved capable of implementing the famous four-state BB84 protocol, with a mean teleportation fidelity as high as 94.5 ± 2.2 %, which would contribute 0.385 secure bits per teleported qubit. After characterisation by way of quantum process tomography, the performance of the relay was also evaluated to be capable of implementing a six-state QKD protocol. In an effort to further extend the emitted light from a QD into the telecom C-band (1530—1565 nm), alternative material systems were investigated. InAs QDs on a substrate of InP were shown to emit much more readily in the fibre-telecom O- and C-bands than their InAs/GaAs counterparts, largely due to the reduced lattice mismatch between the QD and substrate for InAs/InP (~3 %) compared to InAs/GaAs (~7 %). Additionally, to minimize the fine structure splitting (FSS) of the exciton level, which deteriorates the observed polarisation-entanglement, a new mode of dot growth was investigated. Known as droplet epitaxy (D-E), QDs grown in this mode showed a fourfold reduction in the FSS compared to dots grown in the Stranski-Krastanow mode. This improvement would allow observation of polarisation-entanglement in the telecom C-band. In subsequent work performed by colleagues at the Toshiba Cambridge Research Labs, these D-E QDs were embedded in a p-i-n doped optical cavity, processed with electrical contacts, and found to emit entangled pairs of photons under electrical excitation. The work of this thesis provides considerable technological advances to the field of entangled-light sources, that in the near future may allow for deterministic quantum repeaters operating at megahertz rates, and in the further future could facilitate the distribution of coherent multipartite states across a distributed quantum network.
On-demand indistinguishable single-photon sources are essential for quantum networking and communication. Semiconductor quantum dots are among the most promising candidates, but their typical emission wavelength renders them unsuitable for use in fiber networks. Here, we present quantum frequency conversion of near-infrared photons from a bright quantum dot to the telecommunication C-band, allowing integration with existing fiber architectures. We use a custom-built, tunable 2400 nm seed laser to convert single photons from 942 nm to 1550 nm in a difference-frequency generation process. We achieve an end-to-end conversion efficiency of ≃35%, demonstrate count rates approaching 1 MHz at 1550 nm with g(2)(0)=0.043(1), and achieve Hong-Ou-Mandel (HOM) visibilities of 60%. We expect this scheme to be preferable to quantum dot sources directly emitting at telecom wavelengths for fiber-based quantum networking.
A practical way to link separate nodes in quantum networks is to send photons over the standard telecom fibre network. This requires sub-Poissonian photon sources in the telecom wavelength band around 1550 nm, where the photon coherence time has to be sufficient to enable the many interference-based technologies at the heart of quantum networks. Here, we show that droplet epitaxy InAs/InP quantum dots emitting in the telecom C-band can provide photons with coherence times exceeding 1 ns even under non-resonant excitation, more than a factor two longer than values reported for shorter wavelength quantum dots under similar conditions. We demonstrate that these coherence times enable near-optimal interference with a C-band laser qubit, with visibilities only limited by the quantum dot multiphoton emission. Using entangled photons, we further show teleportation of such qubits in six different bases with average fidelity reaching 88.3$\pm$4%. Beyond direct applications in long-distance quantum communication, the high degree of coherence in these quantum dots is promising for future spin based telecom quantum network applications.
Quantum communication networks are formed of secure links, where information can be transmitted with security guaranteed by the quantum nature of light. An essential building block of such a network is a source of single photons and entangled photon pairs, compatible with the low-loss fibre telecom window around 1550 nm. Previous work based on semiconductor quantum dots (QDs), colour centres in diamond and single atoms has been limited by emission wavelengths unsuitable for long distance applications. Efforts have been made to use standard gallium arsenide based QDs by extending their operating wavelength range, however, electrically driven quantum light emission from quantum dots in this telecommunication window has not yet been demonstrated. In this work, indium phosphide based QD devices have been developed to address this problem. The industry favoured growth method, metalorganic vapour phase epitaxy (MOVPE), has been used to create droplet QDs with low fine structure splitting (FSS). This growth scheme allows us to produce the first optoelectronic devices for single and entangled photon emission in the 1550 nm telecom window. We show single-photon emission with multi-photon events suppressed to 0.11±0.02. Furthermore, we obtain entangled light from the biexciton cascade with a maximum fidelity of 0.87± 0.04 which is sufficient for error correction protocols. We also show extended device operating temperature up to 93 K, allowing operation with liquid nitrogen or simple closed-cycle coolers. Our device can be directly integrated with existing long distance quantum communication, cryptography and quantum relay systems providing a new platform for developing quantum networks.