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APS

Precise Internal State Spectroscopy In Ion Traps

Dana J. Berkeland

Published Apr 1, 1997• 0 citations
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Precision spectroscopy of a trapped 173^{173}173Yb+^++ ion using a bath of ultracold atoms
We demonstrate precision laser spectroscopy of a trapped 173^{173}173Yb+^++ ion that is not directly laser cooled by coupling it to ultracold atoms. The atomic bath continuously cools the internal degrees of freedom of the ion to its hyperfine ground state via spin-exchange collisions. Successful laser excitation is detected via state-selective charge transfer and subsequent ion loss. We probe the 62S1/2→62P3/26^2S_{1/2}\rightarrow 6^2P_{3/2}62S1/2​→62P3/2​ transition at 329 nm and measure the magnetic and electric hyperfine interaction constants for the 62P3/26^2P_{3/2}62P3/2​ state to be A=−241(1)A=-241(1)A=−241(1) MHz and B=1460(8)B=1460(8)B=1460(8) MHz, respectively. Our results are in agreement with a previous measurement obtained in a hollow-cathode discharge experiment but are a factor of 6-9 more precise. The techniques demonstrated in this work may be extended to perform precision spectroscopy on other ions with complex level structures.
We present a general technique for precision spectroscopy of atoms that lack suitable transitions for efficient laser cooling, internal state preparation, and detection. In our implementation with trapped atomic ions, an auxiliary "logic" ion provides sympathetic laser cooling, state initialization, and detection for a simultaneously trapped "spectroscopy" ion. Detection is achieved by applying a mapping operation to each ion, which results in a coherent transfer of the spectroscopy ion's internal state onto the logic ion, where it is then measured with high efficiency. Experimental realization, by using 9Be+ as the logic ion and 27Al+ as the spectroscopy ion, indicates the feasibility of applying this technique to make accurate optical clocks based on single ions.