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Springer eBooks

New Avenues for Matter-Wave-Enhanced Spectroscopy

Jonas Rodewald, Philipp Haslinger, Nadine Dörre, Benjamin A. Stickler, Armin Shayeghi, Klaus Hornberger, Markus Arndt

Published Jan 1, 2018• 2 citations
Publisher

Abstract

Abstract We present matter-wave interferometry as a tool to advance spectroscopy for a wide class of nanoparticles, clusters and molecules. The high sensitivity of de Broglie interference fringes to external perturbations enables measurements in the limit of an individual particle absorbing only a single photon on average, or even no photon at all. The method allows one to extract structural and electronic information from the loss of the interference contrast. It is minimally invasive and works even for dilute ensembles.

DOI
10.1007/978-3-319-64346-5_2

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Physica Scripta•May 17, 2016•14 citations
Abstract We present matter-wave interferometry as a tool to advance spectroscopy for a wide class of nanoparticles, clusters and molecules. The high sensitivity of de Broglie interference fringes to external perturbations enables measurements in the limit of an individual particle absorbing only a single photon on average, or even no photon at all. The method allows one to extract structural and electronic information from the loss of the interference contrast. It is minimally invasive and works even for dilute ensembles.
We present matter-wave interferometry as a tool to advance spectroscopy for a wide class of nanoparticles, clusters and molecules. The high sensitivity of de Broglie interference fringes to external perturbations enables measurements in the limit of an individual particle absorbing only a single photon on average, or even no photon at all. The method allows one to extract structural and electronic information from the loss of the interference contrast. It is minimally invasive and works even for dilute ensembles.
The chapter discusses advances in matter-wave optics with complex molecules, generalizing Young’s double slit to high masses. The quantum wave-particle duality is visualized by monitoring the arrival patterns of molecules diffracted at nanomechanical masks. Each molecule displays particle behavior when it is localized on the detector; however, the overall interference pattern requires their delocalization in free flight. Internal particle properties influence the de Broglie waves in the presence of surfaces or fields—even in interaction with atomically thin gratings. To probe the quantum nature of high-mass molecules, universal beam splitters are combined in a multi-grating interferometer to observe high-contrast matter-wave fringes even for 500 K hot molecules, containing 810 atoms with a mass of 10 000 amu. The high sensitivity of the nanoscale interference fringes to deflection in external fields enables non-invasive measurements of molecular properties. The chapter concludes by discussing research on beam techniques that extend molecular quantum optics to large biomolecules.
Recent progress and future prospects of matter-wave interferometry with complex organic molecules and inorganic clusters are reviewed. Three variants of a near-field interference effect, based on diffraction by material nanostructures, at optical phase gratings, and at ionizing laser fields are considered. The theoretical concepts underlying these experiments and the experimental challenges are discussed. This includes optimizing interferometer designs as well as understanding the role of decoherence. The high sensitivity of matter-wave interference experiments to external perturbations is demonstrated to be useful for accurately measuring internal properties of delocalized nanoparticles. The prospects for probing the quantum superposition principle are investigated in the limit of high particle mass and complexity.
Matter-wave interferometry has become a ubiquitous and reliable tool for studying fundamental forces and phenomena and for realizing sensitive measurements. Our recent experiments with metal clusters have allowed us to demonstrate the quantum-wave nature of nanoparticles exceeding 170 kDa. Interestingly, the same experiments also allow for the preparation of moiré fringes of objects in the megadalton range. In this work, we demonstrate such moiré fringes of large sodium nanoparticles and, owing to the platform's stability, resolve nanometer-scale fringe displacements between successive contrast revivals, directly observing the predicted π-phase flip as a half-period shift. We further discuss how this feature turns the interferometer into a device for advanced sensing, even when operating in the regime where the predictions of quantum and classical physics merge.
Modern quantum optics encompasses a wide field of phenomena that are either related to the discrete quantum nature of light, the quantum wave nature of matter or light-matter interactions.We here discuss new perspectives for quantum optics with biological nanoparticles.We focus in particular on the prospects of matter-wave interferometry with amino acids, nucleotides, polypeptides or DNA strands.We motivate the challenge of preparing these objects in a 'biomimetic' environment and argue that hydrated molecular beam sources are promising tools for quantum-assisted metrology.The method exploits the high sensitivity of matter-wave interference fringes to dephasing and shifts in the presence of external perturbations to access and determine molecular properties.