Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Physics B Atomic Molecular and Optical Physics

Ultrafast time delay as a control parameter in resonant ionization by two XUV ultrashort pulses

Theodoros Mercouris, Yannis Komninos, Cleanthes A. Nicolaides

Published Feb 20, 2020• 2 citations
Publisher

Abstract

Abstract We predict quantitatively that it is possible to use few-femtosecond positive or negative time delays , Δ t , between two XUV Gaussian few-femtosecond pulses of moderate intensities and central frequencies ω 1 and ω 2 , in order to control the probability of ionization at clearly defined exit energies corresponding to the sums of photon frequencies ( ω 1 + ω 1 ), ( ω 2 + ω 2 ), and ( ω 1 + ω 2 , or ω 2 + ω 1 ). The phenomenon is demonstrated quantitatively by obtaining and using nonperturbative solutions of the time-dependent Schrödinger equation for a time-dependent scheme involving the process of two-photon resonant ionization of Helium via the 1 s 2 p P o 1 (58.4 nm) and 1 s 4 p P o 1 (52.22 nm) excited states. The calculations used wavefunctions which are state-specific for the discrete spectrum, (up to the 1 s 7 g

DOI
10.1088/1361-6455/ab787b

Related papers

Control of resonant ionization as a function of time delay between two XUV few-femtosecond pulses. Quantitative application to helium

Theodoros Mercouris, Yannis Komninos, Cleanthes A. Nicolaides

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative solutions of the time dependent Schroedinger equation. Comparison with results from second order time dependent perturbation theory provides additional insight.

arXiv:1908.07552•Aug 20, 2019•0 citations

Discrete-resonance-resonance transitions induced by two laser pulses with an ultrashort time delay: A formal analytic solution and quantitative applications

Yannis Komninos, Theodoros Mercouris, Cleanthes A. Nicolaides

The paper presents a theory that solves analytically the time-dependent three-level problem of the scheme $\mathrm{discrete}\phantom{\rule{0.28em}{0ex}}|0\ensuremath{\rangle}\phantom{\rule{0.28em}{0ex}}\underset{\mathrm{as}\phantom{\rule{0.16em}{0ex}}\mathrm{pulse}\phantom{\rule{0.16em}{0ex}}{\ensuremath{\omega}}_{1}}{\overset{\mathrm{weak}\phantom{\rule{0.16em}{0ex}}}{\ensuremath{\rightarrow}}}\phantom{\rule{0.28em}{0ex}}\mathrm{resonance}\phantom{\rule{0.28em}{0ex}}|1\ensuremath{\rangle}\phantom{\rule{0.28em}{0ex}}\underset{\mathrm{fs}\phantom{\rule{0.16em}{0ex}}\mathrm{pulse}\phantom{\rule{0.16em}{0ex}}{\ensuremath{\omega}}_{2}}{\overset{\mathrm{moderately}\phantom{\rule{0.16em}{0ex}}\mathrm{strong}\phantom{\rule{0.16em}{0ex}}}{\ensuremath{\rightarrow}}}\phantom{\rule{0.28em}{0ex}}\mathrm{resonance}\phantom{\rule{0.28em}{0ex}}|2\ensuremath{\rangle}$, where $|0\ensuremath{\rangle}$ is a discrete state, and $|1\ensuremath{\rangle}$ and $|2\ensuremath{\rangle}$ are energy-normalized resonance states. The attosecond and femtosecond pulses with central frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$ (${\ensuremath{\omega}}_{1}\ensuremath{\gg}{\ensuremath{\omega}}_{2}$) act with ultrashort time delay, ${t}_{D}$. The formalism leads to analytic expressions for photoelectron emission probabilities, ${P}_{i}(E,t)$, $i=1,2$, in the energy region of the two resonance states, whose calculation in terms of N-electron matrix elements and external control parameters can be carried out economically for any such three-level system. The problem is first solved analytically, within the rotating wave approximation, for the case where the femtosecond pulse is rectangular. The weak attosecond pulse can have any temporal shape. The final solution for two pulses with arbitrary shape (Gaussian in our case) is then achieved by fitting numerically the shape of the femtosecond pulse to a sum of rectangular pulses. The formulas for ${P}_{i}(E,t)$ involve, among other things, the Fano discrete-resonance asymmetry parameter $q$, and the resonance-resonance asymmetry parameter Q, defined by us in previous work. They also involve the complex energy poles of the two resonances, a result which accounts for the whole contribution of the open channels of energy-normalized scattering states into which they decay. The theory is applied to the calculation from first principles, using compact state-specific discrete and resonance wave functions, of observable aspects of the time-resolved dynamics associated with the processes $\mathrm{He}$ $1{s}^{2}$ $^{1}S$ $\ensuremath{\rightarrow}$ $(2s2p)$ $^{1}P^{o}$ $\ensuremath{\leftrightarrow}$ $(2{p}^{2})$ $^{1}D$. Calculations show that the $(2{p}^{2})$ $^{1}D$ resonance is 0.295 eV (4200 nm) below the energy of $(2s2p)$ $^{1}P^{o}$, (60.15 eV), and its width is 0.067 eV. For the transition $1{s}^{2}$ $^{1}S$ $\ensuremath{\rightarrow}$ $(2s2p)$ $^{1}P^{o}$, the full width at half maximum (FWHM) of the Gaussian pulse is 160 as. The few-cycle midinfrared pulse coupling the resonance states is also Gaussian, whose duration is varied in the range of a few decades of femtoseconds. Its intensity is in the range $5\ifmmode\times\else\texttimes\fi{}{10}^{10}--5\ifmmode\times\else\texttimes\fi{}{10}^{11}$ $\mathrm{W}/\mathrm{c}{\mathrm{m}}^{2}$. The external control parameters are the intensity and the FWHM of the femtosecond pulse, as well as the ${t}_{D}$. For a given value of ${t}_{D}$, the FWHM of the second pulse is a crucial control parameter. The results include the time-resolved formation of either the $(2s2p)$ $^{1}P^{o}$ or the $(2{p}^{2})$ $^{1}D$ resonance, while they are coupled with each other. For the $(2s2p)$ $^{1}P^{o}$ state, comparison is made with the case where the time-dependent buildup of its asymmetric profile, excited from $1{s}^{2}$ $^{1}S$ by the same attosecond pulse, is calculated in the absence of coupling to another resonance. The result is in harmony with that of our earlier work on this problem. For the $(2{p}^{2})$ $^{1}D$ resonance excited from $(2s2p)$ $^{1}P^{o}$, the time-resolved buildup of its profile does not develop into an asymmetric peak due to the fact that $Q$ has the very large value of $\ensuremath{\approx}\ensuremath{-}1300$. Instead, it finishes as an Autler-Townes doublet.

Physical Review A•Aug 30, 2018•2 citations

Enhancing Autler-Townes splittings by ultrafast XUV pulses

Wei‐Chao Jiang, Hao Liang, Shun Wang +2 more

We study the photoelectron spectra of hydrogen and helium ionized by intense ultrafast two-color XUV laser pulses by numerically solving the time-dependent Schrödinger equation.The photon energy of the pump pulse is tuned to the 1s-2p excitation energy, inducing Rabi oscillations between these bound states and forming an Autler-Townes (AT) doublet of dressed states.When ionized by a time-delayed ultrafast XUV pulse with duration shorter than the Rabi oscillation period, we find novel and drastically enhanced AT splittings in the photoionization spectrum.We identify their origin in terms of the temporal interference of two attosecond wave packets whose spectral distribution is controlled by the interplay between Rabi frequency and bandwidth of the probe pulse.These time-dependent features in the spectra can be much larger than the standard AT spacing induced by the pump pulse alone and can be controlled by the time delay and the duration of the probe pulse.

Physical Review Research•Aug 25, 2021•31 citations

Attosecond XUV absorption spectroscopy of doubly excited states in helium atoms dressed by a time-delayed femtosecond infrared laser

Z. Q. Yang, Difa Ye, Thomas Ding +2 more

In the present paper, we investigate the time-resolved transient absorption spectroscopy of doubly excited states of helium atoms by solving the time-dependent two-electron Schr\"odinger equation numerically based on a one-dimensional model. The helium atoms are subjected to an extreme ultraviolet (XUV) attosecond pulse and a time-delayed infrared (IR) few-cycle laser pulse. A superposition of doubly excited states populated by the XUV pulse is identified, which interferes with the direct ionization pathway leading to Fano resonance profiles in the photoabsorption spectrum. In the presence of an IR laser, however, the Fano line profiles are strongly modified: A shifting, splitting, and broadening of the original absorption lines is observed when the XUV attosecond pulse and infrared few-cycle laser pulse overlap in time, which is in good agreement with recent experimental results. At certain time delays, we observe symmetric Lorentz, inverted Fano profiles, and even negative absorption cross sections indicating that the XUV light can be amplified during the interaction with atoms. We further prove that the above pictures are general for different doubly excited states by suitably varying the frequency of the IR field to coherently couple the corresponding states.

Physical Review A•Jan 27, 2015•30 citations

Ultimate capabilities for few-cycle pulse formation via resonant interaction of XUV radiation with IR-field-dressed atoms

T. R. Akhmedzhanov, M. Yu. Emelin, V. A. Antonov +3 more

We perform an ab initio study of the ultimate capabilities and limits of applicability of the method for few-cycle pulse formation via the resonant interaction of extreme ultraviolet (XUV) radiation with atoms dressed by a moderately strong infrared (IR) laser field proposed in two earlier works [Y. V. Radeonychev et al., Phys. Rev. Lett. 105, 183902 (2010) and V. A. Polovinkin et al., Opt. Lett. 36, 2296 (2011)]. Taking into account all the multiphoton processes in the systems under consideration on the basis of numerical solution of the three-dimensional time-dependent Schr\"odinger equation (TDSE) in the single-active-electron approximation, we show the possibilities to produce 1.1-fs pulses from 124.6-nm XUV radiation via the linear Stark effect in atomic hydrogen, as well as 500-as pulses from 58.4-nm XUV radiation via excited-state ionization in helium. We derive a generalized analytical solution, which takes into account the interplay between sub-laser-cycle Stark effect and excited-state ionization and allows us to analyze the results of TDSE calculations. We found that the ultimate intensity of the IR field suitable for few-cycle pulse formation via the linear Stark effect or excited-state ionization is limited by the threshold for atomic ionization from the resonant excited state or the ground state, respectively. We show that the pulses with shorter duration can be produced in the medium of ions with higher values of the ionization potential.

Physical Review A•Feb 28, 2017•6 citations

Coherent control of extreme uv absorption and photoemission by the simultaneous irradiation of ultrashort extreme uv and laser pulses

Kenichi L. Ishikawa, Katsumi Midorikawa

We present a theoretical study on the response of a hydrogen atom to the simultaneous irradiation of ultrashort extreme ultraviolet (xuv) and laser pulses. The calculation is based on the time-dependent Schr\"odinger equation. The xuv photon energy is chosen to induce the $1s\ensuremath{-}2p$ transition. Our results indicate that we can transiently reduce the xuv absorption and change the atomic state within a few femtoseconds by injecting a femtosecond laser pulse. The laser-induced photoemission is affected by the addition of an xuv pulse and its yield depends much on the temporal overlap of the two pulses.

Physical Review A•Feb 5, 2002•14 citations
Abstract We predict quantitatively that it is possible to use few-femtosecond positive or negative time delays , Δ t , between two XUV Gaussian few-femtosecond pulses of moderate intensities and central frequencies ω 1 and ω 2 , in order to control the probability of ionization at clearly defined exit energies corresponding to the sums of photon frequencies ( ω 1 + ω 1 ), ( ω 2 + ω 2 ), and ( ω 1 + ω 2 , or ω 2 + ω 1 ). The phenomenon is demonstrated quantitatively by obtaining and using nonperturbative solutions of the time-dependent Schrödinger equation for a time-dependent scheme involving the process of two-photon resonant ionization of Helium via the 1 s 2 p P o 1 (58.4 nm) and 1 s 4 p P o 1 (52.22 nm) excited states. The calculations used wavefunctions which are state-specific for the discrete spectrum, (up to the 1 s 7 g
The paper presents a theory that solves analytically the time-dependent three-level problem of the scheme $\mathrm{discrete}\phantom{\rule{0.28em}{0ex}}|0\ensuremath{\rangle}\phantom{\rule{0.28em}{0ex}}\underset{\mathrm{as}\phantom{\rule{0.16em}{0ex}}\mathrm{pulse}\phantom{\rule{0.16em}{0ex}}{\ensuremath{\omega}}_{1}}{\overset{\mathrm{weak}\phantom{\rule{0.16em}{0ex}}}{\ensuremath{\rightarrow}}}\phantom{\rule{0.28em}{0ex}}\mathrm{resonance}\phantom{\rule{0.28em}{0ex}}|1\ensuremath{\rangle}\phantom{\rule{0.28em}{0ex}}\underset{\mathrm{fs}\phantom{\rule{0.16em}{0ex}}\mathrm{pulse}\phantom{\rule{0.16em}{0ex}}{\ensuremath{\omega}}_{2}}{\overset{\mathrm{moderately}\phantom{\rule{0.16em}{0ex}}\mathrm{strong}\phantom{\rule{0.16em}{0ex}}}{\ensuremath{\rightarrow}}}\phantom{\rule{0.28em}{0ex}}\mathrm{resonance}\phantom{\rule{0.28em}{0ex}}|2\ensuremath{\rangle}$, where $|0\ensuremath{\rangle}$ is a discrete state, and $|1\ensuremath{\rangle}$ and $|2\ensuremath{\rangle}$ are energy-normalized resonance states. The attosecond and femtosecond pulses with central frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$ (${\ensuremath{\omega}}_{1}\ensuremath{\gg}{\ensuremath{\omega}}_{2}$) act with ultrashort time delay, tD{t}_{D}tD​. The formalism leads to analytic expressions for photoelectron emission probabilities, Pi(E,t){P}_{i}(E,t)Pi​(E,t), i=1,2i=1,2i=1,2, in the energy region of the two resonance states, whose calculation in terms of N-electron matrix elements and external control parameters can be carried out economically for any such three-level system. The problem is first solved analytically, within the rotating wave approximation, for the case where the femtosecond pulse is rectangular. The weak attosecond pulse can have any temporal shape. The final solution for two pulses with arbitrary shape (Gaussian in our case) is then achieved by fitting numerically the shape of the femtosecond pulse to a sum of rectangular pulses. The formulas for Pi(E,t){P}_{i}(E,t)Pi​(E,t) involve, among other things, the Fano discrete-resonance asymmetry parameter qqq, and the resonance-resonance asymmetry parameter Q, defined by us in previous work. They also involve the complex energy poles of the two resonances, a result which accounts for the whole contribution of the open channels of energy-normalized scattering states into which they decay. The theory is applied to the calculation from first principles, using compact state-specific discrete and resonance wave functions, of observable aspects of the time-resolved dynamics associated with the processes He\mathrm{He}He 1s21{s}^{2}1s2 1S^{1}S1S $\ensuremath{\rightarrow}$ (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po $\ensuremath{\leftrightarrow}$ (2p2)(2{p}^{2})(2p2) 1D^{1}D1D. Calculations show that the (2p2)(2{p}^{2})(2p2) 1D^{1}D1D resonance is 0.295 eV (4200 nm) below the energy of (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po, (60.15 eV), and its width is 0.067 eV. For the transition 1s21{s}^{2}1s2 1S^{1}S1S $\ensuremath{\rightarrow}$ (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po, the full width at half maximum (FWHM) of the Gaussian pulse is 160 as. The few-cycle midinfrared pulse coupling the resonance states is also Gaussian, whose duration is varied in the range of a few decades of femtoseconds. Its intensity is in the range $5\ifmmode\times\else\texttimes\fi{}{10}^{10}--5\ifmmode\times\else\texttimes\fi{}{10}^{11}$ W/cm2\mathrm{W}/\mathrm{c}{\mathrm{m}}^{2}W/cm2. The external control parameters are the intensity and the FWHM of the femtosecond pulse, as well as the tD{t}_{D}tD​. For a given value of tD{t}_{D}tD​, the FWHM of the second pulse is a crucial control parameter. The results include the time-resolved formation of either the (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po or the (2p2)(2{p}^{2})(2p2) 1D^{1}D1D resonance, while they are coupled with each other. For the (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po state, comparison is made with the case where the time-dependent buildup of its asymmetric profile, excited from 1s21{s}^{2}1s2 1S^{1}S1S by the same attosecond pulse, is calculated in the absence of coupling to another resonance. The result is in harmony with that of our earlier work on this problem. For the (2p2)(2{p}^{2})(2p2) 1D^{1}D1D resonance excited from (2s2p)(2s2p)(2s2p) 1Po^{1}P^{o}1Po, the time-resolved buildup of its profile does not develop into an asymmetric peak due to the fact that QQQ has the very large value of $\ensuremath{\approx}\ensuremath{-}1300$. Instead, it finishes as an Autler-Townes doublet.
We study the photoelectron spectra of hydrogen and helium ionized by intense ultrafast two-color XUV laser pulses by numerically solving the time-dependent Schrödinger equation.The photon energy of the pump pulse is tuned to the 1s-2p excitation energy, inducing Rabi oscillations between these bound states and forming an Autler-Townes (AT) doublet of dressed states.When ionized by a time-delayed ultrafast XUV pulse with duration shorter than the Rabi oscillation period, we find novel and drastically enhanced AT splittings in the photoionization spectrum.We identify their origin in terms of the temporal interference of two attosecond wave packets whose spectral distribution is controlled by the interplay between Rabi frequency and bandwidth of the probe pulse.These time-dependent features in the spectra can be much larger than the standard AT spacing induced by the pump pulse alone and can be controlled by the time delay and the duration of the probe pulse.
In the present paper, we investigate the time-resolved transient absorption spectroscopy of doubly excited states of helium atoms by solving the time-dependent two-electron Schr\"odinger equation numerically based on a one-dimensional model. The helium atoms are subjected to an extreme ultraviolet (XUV) attosecond pulse and a time-delayed infrared (IR) few-cycle laser pulse. A superposition of doubly excited states populated by the XUV pulse is identified, which interferes with the direct ionization pathway leading to Fano resonance profiles in the photoabsorption spectrum. In the presence of an IR laser, however, the Fano line profiles are strongly modified: A shifting, splitting, and broadening of the original absorption lines is observed when the XUV attosecond pulse and infrared few-cycle laser pulse overlap in time, which is in good agreement with recent experimental results. At certain time delays, we observe symmetric Lorentz, inverted Fano profiles, and even negative absorption cross sections indicating that the XUV light can be amplified during the interaction with atoms. We further prove that the above pictures are general for different doubly excited states by suitably varying the frequency of the IR field to coherently couple the corresponding states.
We perform an ab initio study of the ultimate capabilities and limits of applicability of the method for few-cycle pulse formation via the resonant interaction of extreme ultraviolet (XUV) radiation with atoms dressed by a moderately strong infrared (IR) laser field proposed in two earlier works [Y. V. Radeonychev et al., Phys. Rev. Lett. 105, 183902 (2010) and V. A. Polovinkin et al., Opt. Lett. 36, 2296 (2011)]. Taking into account all the multiphoton processes in the systems under consideration on the basis of numerical solution of the three-dimensional time-dependent Schr\"odinger equation (TDSE) in the single-active-electron approximation, we show the possibilities to produce 1.1-fs pulses from 124.6-nm XUV radiation via the linear Stark effect in atomic hydrogen, as well as 500-as pulses from 58.4-nm XUV radiation via excited-state ionization in helium. We derive a generalized analytical solution, which takes into account the interplay between sub-laser-cycle Stark effect and excited-state ionization and allows us to analyze the results of TDSE calculations. We found that the ultimate intensity of the IR field suitable for few-cycle pulse formation via the linear Stark effect or excited-state ionization is limited by the threshold for atomic ionization from the resonant excited state or the ground state, respectively. We show that the pulses with shorter duration can be produced in the medium of ions with higher values of the ionization potential.
We present a theoretical study on the response of a hydrogen atom to the simultaneous irradiation of ultrashort extreme ultraviolet (xuv) and laser pulses. The calculation is based on the time-dependent Schr\"odinger equation. The xuv photon energy is chosen to induce the $1s\ensuremath{-}2p$ transition. Our results indicate that we can transiently reduce the xuv absorption and change the atomic state within a few femtoseconds by injecting a femtosecond laser pulse. The laser-induced photoemission is affected by the addition of an xuv pulse and its yield depends much on the temporal overlap of the two pulses.