This thesis summarizes our study on the properties of ultracold Fermions near a Feshbach resonance. The Feshbach resonance allows for a continuous tuning of the interaction strength between the atoms. With this tunability, many properties predicted for the BCS-BEC crossover region in solids can be shown to exist in this ultracold Fermi gas. With the highly controllable parameters and the clean environment in the experiments, the study of the Bardeen-Cooper-Schrieffer (BCS) to Bose-Einstein Condensation (BEC) crossover in ultracold Fermions provides valuable insights to the strongly interacting crossover region, which has never been achieved before in solids. We first examine the properties of 6 Li and 40 K gases. We find that in the unitary region the properties of the system do not depend on the atom species: outside the unitary region, the properties of the system do depend on the scattering properties of the different atom species. We study the dynamics of the ultracold Fermions in the crossover region in response to the variations in the external magnetic field. We find that the response depends on the time scale and the amplitude of the variations; which is in qualitative agreement with the experimental observations. We derive a set of dynamic mean-field equations for a Fermi gas in an arbitrary potential trap near a wide Feshbach resonance. The equations are more general than the local density approximation (LDA), and less demanding computationally as the Bogoliubov-de-Gennes (BdG) equation. We then analyze the solubility of the equations, as well as solve a simplified version of the equations for illustration and for self-consistency check on the assumptions made during the derivation. We systematically study the possible phases for a trapped Fermi gas with population imbalance near a Feshbach resonance. Our results agree qualitatively well with the recent experimental results, and predict the existence of two exotic non-BCS superfluid phases for the strongly interacting gas with population unbalance: the Breached Pair (BP) phase and the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. Finally, to guide the experimental efforts in the search of new quantum phases, we propose a detection scheme for the possible exotic phases.
This thesis presents experiments probing physics in the crossover between Bose-Einstein condensation (BEC) and BCS superconductivity using an ultracold gas of atomic fermions. Scattering resonances in these ultracold gases (known as Feshbach resonances) provide the unique ability to tune the fermion-fermion interactions. The work presented here pioneered the use of fermionic Feshbach resonances as a highly controllable and tunable system ideal for studying the cusp of the BCS-BEC crossover problem. Here pairs of fermionic atoms have some properties of diatomic molecules and some properties of Cooper pairs. I present studies of a normal Fermi gas at a Feshbach resonance and the work required to cool the gas to temperatures where superfluidity in the crossover is predicted. These studies culminated in our observation of a phase transition at the cusp of the BCS-BEC crossover through condensation of fermionic atom pairs. I also discuss subsequent work that confirmed the crossover nature of the pairs in these condensates.
PACS. 03.75.Hh – Static properties of condensates; thermodynamical, statistical and structural properties. PACS. 03.75.Ss – Degenerate Fermi gases. PACS. 05.30.Fk – Fermion systems and electron gas. Abstract. – We present a theory for a superfluid Fermi gas near the BCS-BEC crossover, including pairing fluctuation contributions to the free energy similar to that considered by Nozières and Schmitt-Rink for the normal phase. In the strong coupling limit, our theory is able to recover the Bogoliubov theory of a weakly interacting Bose gas with a molecular scattering length very close to the known exact result. We compare our results with recent Quantum Monte Carlo simulations both for the ground state and at finite temperature. Excellent agreement is found for all interaction strengths where simulation results are available. The recent experimental realization of strongly interacting Fermi gases of 6 Li and 40 K atoms near a Feshbach resonance has opened up the exciting possibility of investigating the crossover from a Bardeen-Cooper-Schrieffer (BCS) superfluid to a Bose-Einstein condensate (BEC) [1–5]. In these systems, the inter-atomic interaction strength can be varied by tuning
Abstract We present a theoretical review of the recent progress in non-equilibrium BCS (Bardeen-Cooper-Schrieffer)-BEC (Bose-Einstein condensation) crossover physics. As a paradigmatic example, we consider a strongly interacting driven-dissipative two-component Fermi gas where the non-equilibrium steady state is tuned by adjusting the chemical potential difference between two reservoirs that are coupled with the system. As a powerful theoretical tool to deal with this system, we employ the Schwinger-Keldysh Green’s function technique. We systematically evaluate the superfluid transition, as well as the single-particle properties, in the non-equilibrium BCS-BEC crossover region, by adjusting the chemical potential difference between the reservoirs and the strength of an s-wave pairing interaction associated with a Feshbach resonance. In the weak-coupling BCS side, the chemical potential difference is shown to imprint a two-step structure on the particle momentum distribution, leading to an anomalous enhancement of pseudogap, as well as the emergence of exotic Fulde-Ferrell-Larkin-Ovchinnikov-type superfluid instability. Since various non-equilibrium situations have recently been realized in ultracold Fermi gases, the theoretical understanding of non-equilibrium BCS-BEC crossover physics would become increasingly important in this research field.
We investigate the single-particle properties at
T=0 of a trapped superfluid gas of Fermi atoms with a Feshbach resonance. A tunable pairing interaction associated with the Feshbach resonance leads to the BCS--Bose-Einstein condensate (BEC) crossover, where the character of superfluidity continuously changes from the BCS-type to a BEC of composite bosons. In this paper, we extend our previous work for a uniform superfluid Fermi gas [Y. Ohashi and A. Griffin, Phys. Rev. A 67, 063612 (2003)] to include the effect of a harmonic trap. We do not use the local density approximation (LDA), but directly solve the Bogoliubov--de Gennes (BdG) coupled equations. While our explicit numerical solutions are for a weak (narrow) Feshbach resonance, we argue that the single-particle BdG excitation spectrum will exhibit the same features for a strong (broad) Feshbach resonance. Using these equations, we find self-consistent values for the spatially dependent local density
n(r) as well as the composite BCS order parameter $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\ensuremath{\Delta}}(\mathbf{r})$, the latter describing both the Cooper-pair and molecular condensate contributions. Using these results, we calculate the single-particle density of states in the crossover region, and from this determine the true single-particle energy gap
(Eg) of the trapped Fermi superfluid. This is associated with the in-gap (or Andreev) states in the low-density region at the edge of the trap. We calculate the laser-induced tunneling current $I(\ensuremath{\omega})$ into another hyperfine state, as measured in recent rf spectroscopy experiments. This rf spectrum gives a direct probe of the quasiparticle spectrum. We show how the high-energy part of $I(\ensuremath{\omega})$ gives information about $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\ensuremath{\Delta}}(r=0)$ at the center of the trap (which is comparable to the Fermi energy ${\ensuremath{\epsilon}}_{F}$ in the crossover region). We show that $I(\ensuremath{\omega})$ is very dependent on the spatial profile of the pair potential $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\ensuremath{\Delta}}(r)$ that is used. We also emphasize that the narrow ``unpaired atom" peak in the rf data gives information about
Eg and the low-energy $(⪡{\ensuremath{\epsilon}}_{F})$ in-gap states of a Fermi superfluid. While our calculations are limited to
T=0, we use them to discuss the recent data of Chin et al. and the LDA calculations of T\"orm\"a and co-workers. The LDA, while useful, can lead to an incorrect physical picture of the low-density surface region of the Fermi superfluid.
The study of ultracold atomic Fermi gases is a rapidly exploding subject which is defining new directions in condensed matter and atomic physics. Quite generally what makes these gases so important is their remarkable tunability and controllability. Using a Feshbach resonance one can tune the attractive two-body interactions from weak to strong and thereby make a smooth crossover from a BCS superfluid of Cooper pairs to a Bose-Einstein condensed superfluid. Furthermore, one can tune the population of the two spin states, allowing observation of exotic spin-polarized superfluids, such as the Fulde Ferrell Larkin Ovchinnikov (FFLO) phase. A wide array of powerful characterization tools, which often have direct condensed matter analogues, are available to the experimenter. In this Chapter, we present a general review of the status of these Fermi gases with the aim of communicating the excitement and great potential of the field.
A trapped Fermi gas near a collisional resonance provides a unique laboratory for testing many-body theories in a variety of fields. The ultracold Fermi gas produced in our lab is comprised of the lowest two spin states of
6Li. At 834 G there is a collisional or Feshbach resonance between the two spin states. The scattering length between trapped atoms of opposing spins far exceeds the interparticle spacing of the gas. On resonance, a strongly interacting, unitary, Fermi gas is created which exhibits universal behavior. The unitary Fermi gas is a prototype for other exotic systems in nature from nuclear matter to neutron stars and high temperature superconductors. \n For magnetic fields less than 834 G the scattering length is positive, and pairs Fermi atoms can form molecular dimers. These dimers, comprised of two fermions, are bosons. At ultracold temperatures the molecular bosons populate the lowest energy level and form a Bose Einstein Condensate (BEC). For magnetic fields greater than 834G the scattering length between fermions in opposing spin states is negative, like Cooper pairs formed between electrons in a superconductor. The Bardeen, Cooper, and Shriefer (BCS) theory was developed to describe the pairing effect in the context of superconductors. In our experiment we produce an ultracold unitary gas. By tuning the magnetic field to either side of the Feshbach resonance we can transform the gas into a weakly interacting BEC or BCS superfluid. Therefore, the region near a Feshbach resonance is called the BEC-BCS crossover. \n This dissertation presents a precision measurement of the hydrodynamic sound velocity in an ultracold Fermi gas near a Feshbach resonance. The sound velocity is measured at various magnetic fields both above and below resonance. Moreover, we are able compare our measurements to theoretical descriptions of hydrodynamic sound propagation. Further, our measurement of sound velocity exactly reproduces the non-perturbative case, eliminating the need to consider nonlinear effects. At resonance the sound velocity exhibits universal scaling with the Fermi velocity to within 1.8\\% over a factor of 30 in density. In a near zero temperature unitary gas the average sound velocity at the axial center was measured,
c(0)/vF = 0.364(0.005), as well as the universal constant,
beta = -0.565(0.015). The measurement of sound velocity in an ultracold gas throughout the BEC-BCS crossover provides further evidence of the continuous connection between the physics of the BEC, unitary, and BCS systems.