We present a general discussion of the techniques of destabilizing dark states in laser-driven atoms with either a magnetic field or modulated laser polarization. We show that the photon-scattering rate is maximized at a particular evolution rate of the dark state. We also find that the atomic-resonance curve is significantly broadened when the evolution rate is far from this optimum value. These results are illustrated with detailed examples of destabilizing dark states in some commonly trapped ions and supported by insights derived from numerical calculations and simple theoretical models.We present a general discussion of the techniques of destabilizing dark states in laser-driven atoms with either a magnetic field or modulated laser polarization. We show that the photon-scattering rate is maximized at a particular evolution rate of the dark state. We also find that the atomic-resonance curve is significantly broadened when the evolution rate is far from this optimum value. These results are illustrated with detailed examples of destabilizing dark states in some commonly trapped ions and supported by insights derived from numerical calculations and simple theoretical models.

arXiv:quant-ph/0111018Physical Review AFeb 26, 2002186 citations

Destabilization of dark states in MgF molecules

Meng Xia, Ruoxi Gu, Kang Yan +4 more

A significant problem in laser cooling of molecules is the presence of the dark Zeeman sublevels. Herein, a detailed theoretical and experimental study of destabilizing the dark states is reported in magnesium monofluoride molecules. By applying an external magnetic field, the Zeeman sublevels are made to be time dependent and nondegenerate, forcing the dark states to Larmor precess into the bright states. It is found that the laser induced fluorescence signal depends on the angle and the magnitude of the magnetic field. Theoretical calculations are performed by solving the density matrix equations for the multiple-level system, which shows good agreement with experimental data. This study may provide a useful perspective for continuous efforts toward laser cooling of MgF molecules.A significant problem in laser cooling of molecules is the presence of the dark Zeeman sublevels. Herein, a detailed theoretical and experimental study of destabilizing the dark states is reported in magnesium monofluoride molecules. By applying an external magnetic field, the Zeeman sublevels are made to be time dependent and nondegenerate, forcing the dark states to Larmor precess into the bright states. It is found that the laser induced fluorescence signal depends on the angle and the magnitude of the magnetic field. Theoretical calculations are performed by solving the density matrix equations for the multiple-level system, which shows good agreement with experimental data. This study may provide a useful perspective for continuous efforts toward laser cooling of MgF molecules.

Physical Review AJan 27, 202114 citations

Laser Cooling of Atoms and Impact in Theoretical Physics

Ghosh, Pradip N

Jan 1, 19990 citations

Cooling of individual neutral atoms in an optical lattice

Michael J. Gibbons, Peyman Ahmadi, Kevin Fortier +2 more

APSJun 1, 20070 citations

Magneto-optical trap of silver and potassium atoms

Michael Vayninger, Angela Xiang, Nachiket D. Bhanushali +6 more

We demonstrate a dual magneto-optical trap (MOT) of $^{109}\mathrm{Ag}$ and $^{39}\mathrm{K}$ . For silver, a decreasing-field Zeeman slower loads a MOT of $1.5\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at a temperature of 0.74(5) mK, with laser cooling occurring primarily on the ${D}_{2}$ line of $4{d}^{10}5s\phantom{\rule{0.28em}{0ex}}^{2}S_{1/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.28em}{0ex}}^{2}P_{3/2}$ at 328 nm. We create a Ag ``dark spot MOT,'' where shelving the atoms in a dark state enhances the captured atom number by a factor of 2 and the lifetime by a factor of 4. For potassium, we obtain $2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ trapped atoms, and further cooling on the ${D}_{1}$ transition via gray molasses results in a cloud of $1.2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at $7(1)\phantom{\rule{0.28em}{0ex}}\textmu{}\mathrm{K}$. We observe evidence of photoionization loss of the K MOT in the presence of Ag laser-cooling light, necessitating sequential rather than simultaneous loading for the two species. Our results on Ag point to simple and general laser cooling strategies for other coinage metals (Au, Cu). Furthermore, this work lays the foundation for the production of alkali-metal--coinage-metal degenerate quantum mixtures and highly polar molecules.We demonstrate a dual magneto-optical trap (MOT) of $^{109}\mathrm{Ag}$ and $^{39}\mathrm{K}$. For silver, a decreasing-field Zeeman slower loads a MOT of $1.5\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at a temperature of 0.74(5) mK, with laser cooling occurring primarily on the ${D}_{2}$ line of $4{d}^{10}5s\phantom{\rule{0.28em}{0ex}}^{2}S_{1/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.28em}{0ex}}^{2}P_{3/2}$ at 328 nm. We create a Ag ``dark spot MOT,'' where shelving the atoms in a dark state enhances the captured atom number by a factor of 2 and the lifetime by a factor of 4. For potassium, we obtain $2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ trapped atoms, and further cooling on the ${D}_{1}$ transition via gray molasses results in a cloud of $1.2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at $7(1)\phantom{\rule{0.28em}{0ex}}\textmu{}\mathrm{K}$. We observe evidence of photoionization loss of the K MOT in the presence of Ag laser-cooling light, necessitating sequential rather than simultaneous loading for the two species. Our results on Ag point to simple and general laser cooling strategies for other coinage metals (Au, Cu). Furthermore, this work lays the foundation for the production of alkali-metal--coinage-metal degenerate quantum mixtures and highly polar molecules.

arXiv:2507.11434Physical Review ANov 14, 20256 citations

We demonstrate a dual magneto-optical trap (MOT) of

^{109}\mathrm{Ag}

and

^{39}\mathrm{K}

. For silver, a decreasing-field Zeeman slower loads a MOT of $1.5\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at a temperature of 0.74(5) mK, with laser cooling occurring primarily on the

{D}_{2}

line of $4{d}^{10}5s\phantom{\rule{0.28em}{0ex}}^{2}S_{1/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.28em}{0ex}}^{2}P_{3/2}$ at 328 nm. We create a Ag ``dark spot MOT,'' where shelving the atoms in a dark state enhances the captured atom number by a factor of 2 and the lifetime by a factor of 4. For potassium, we obtain $2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ trapped atoms, and further cooling on the

{D}_{1}

transition via gray molasses results in a cloud of $1.2\ifmmode\times\else\texttimes\fi{}{10}^{8}$ atoms at $7(1)\phantom{\rule{0.28em}{0ex}}\textmu{}\mathrm{K}$. We observe evidence of photoionization loss of the K MOT in the presence of Ag laser-cooling light, necessitating sequential rather than simultaneous loading for the two species. Our results on Ag point to simple and general laser cooling strategies for other coinage metals (Au, Cu). Furthermore, this work lays the foundation for the production of alkali-metal--coinage-metal degenerate quantum mixtures and highly polar molecules.