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Fast-beam-laser lifetime measurements for energy levels in singly-ionized lutetium and thulium

Michelle Marilyn. McCurdy

Published Jan 1, 1999• 0 citations
Publisher
DOI
10.7939/r3377630p

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Optics and Spectroscopy•Dec 1, 2018•21 citations
AbstractThe hyperfine structure of transitions in the three-step scheme 5 d 6 s ^22 D _3/2–5 d 6 s 6 p ^4 F 5/2∘_{{5/2}}^{^\circ }5/2∘​ –5 d 6 s 7 s ^4 D _3/2– (53 375 cm^–1) 1/2∘_{{1/2}}^{^\circ }1/2∘​ of lutetium ionization is studied for ^175Lu, ^176Lu, and ^177Lu isotopes using the photoionization laser spectroscopy method. Values of the magnetic dipole ( A ) and electric quadrupole ( B ) interaction constants are determined, as well as the energies, the isotope shifts, and the radiative lifetimes for the 5 d 6 s 7 s ^4 D _3/2 and (53 375 cm^–1) 1/2∘_{{1/2}}^{^\circ }1/2∘​ levels.
We present a spectroscopic investigation of 169Tm+^{169}\mathrm{Tm}^+169Tm+ that provides two key foundations for its use as a platform for advanced quantum applications. First, we establish the complete spectroscopic road map for optical cycling (including laser cooling) by performing high-resolution spectroscopy on 169Tm+^{169}\mathrm{Tm}^+169Tm+ ions in an ion trap. We characterize the primary 313 nm313\,\mathrm{nm}313nm and complementary 448/453 nm448/453\,\mathrm{nm}448/453nm cycling transitions, identify the essential near-infrared repumping frequencies, and determine the magnetic-dipole hyperfine AAA constants for all relevant levels. Second, we report a detailed characterization of a metastable state as a candidate for hosting a robust qubit, performing lifetime measurements and Zeeman-resolved microwave hyperfine spectroscopy with kHz\mathrm{kHz}kHz precision.
The hyperfine structure of transitions in the three-step scheme 5d6s22D3/2–5d6s6p4F 5/2∘_{{5/2}}^{^\circ }5/2∘​ –5d6s7s4D3/2– (53 375 cm–1) 1/2∘_{{1/2}}^{^\circ }1/2∘​ of lutetium ionization is studied for 175Lu, 176Lu, and 177Lu isotopes using the photoionization laser spectroscopy method. Values of the magnetic dipole (A) and electric quadrupole (B) interaction constants are determined, as well as the energies, the isotope shifts, and the radiative lifetimes for the 5d6s7s4D3/2 and (53 375 cm–1) 1/2∘_{{1/2}}^{^\circ }1/2∘​ levels.