In this paper, pure silk protein was extracted from Bombyx mori silks and fabricated into a new kind of disordered bio-microfiber structure using electrospinning technology. Coherent random lasing emission with low threshold was achieved in the silk fibroin fibers. The random lasing emission wavelength can be tuned in the range of 33 nm by controlling the pump location with different scattering strengths. Therefore, the bio-microfiber random lasers can be a wide spectral light source when the system is doped with a gain or energy transfer medium with a large fluorescence emission band. Application of the random lasers of the bio-microfibers as a low-coherence light source in speckle-free imaging had also been studied.
In this paper, pure silk protein was extracted from Bombyx mori silks and fabricated into a new kind of disordered bio-microfiber structure using electrospinning technology. Coherent random lasing emission with low threshold was achieved in the silk fibroin fibers. The random lasing emission wavelength can be tuned in the range of 33 nm by controlling the pump location with different scattering strengths. Therefore, the bio-microfiber random lasers can be a wide spectral light source when the system is doped with a gain or energy transfer medium with a large fluorescence emission band. Application of the random lasers of the bio-microfibers as a low-coherence light source in speckle-free imaging had also been studied.
The statistical behavior of spectral intensity fluctuations in a Raman gain random fiber laser is investigated for the first time, to the best of our knowledge. Through a fiber Fabry–Perot tunable filter, the intensity of the filtered single wavelength from random laser (RL) spectra is measured at different pump powers. The probability density function (PDF) of spectral intensity values is analyzed. Well below the lasing threshold, the intensity of a single wavelength is stable in the time domain, and the PDF exhibits a typical Gaussian behavior. However, around the threshold, strong fluctuations in intensity emerge. In this case, the statistical distribution is characterized by a power-law-tailed function consistent with a Lévy α-stable distribution. We identify the statistical evolution as the injected pump power increases, from a Gaussian to a Lévy and then back to a Gaussian distribution, which is similar to the case of RLs with a strong disorder due to the presence of photon scatterers and gain related to electronic transitions in the active medium, indicating the universal existence of such statistical properties in random lasing systems.
Correlations existing between spectral components in multi-wavelength lasers have been the key challenge that hinders these laser sources from being developed to chaotic comb entropy sources for parallel random bit generation. Herein, spectrotemporally uncorrelated multi-order Stokes/anti-Stokes emissions are achieved by cooperatively exploiting nonlinear optical processes including cascaded stimulated Brillouin scattering and quasi-phase-matched four-wave mixing in a Brillouin random fiber laser. Chaotic instabilities induced by random mode resonance are enhanced and disorderly redistributed among different lasing lines through complex nonlinear optical interactions, which comprehensively releases the inherent correlation among multiple Stokes/anti-Stokes emission lines, realizing a chaotic frequency comb with multiple spectrotemporally uncorrelated channels. Parallel fast random bit generation is fulfilled with 31 channels, single-channel bit rate of 35-Gbps and total bit rate of 1.085-Tbps. National Institute of Standards and Technology statistic tests verify the randomness of generated bit streams. This work, in a simple and efficient way, breaks the correlation barrier for utilizing multi-wavelength laser to achieve high-quality spectrotemporally uncorrelated chaotic laser source, opening new avenues for achieving greatly accelerated random bit generation through parallelization and potentially revolutionizing the current architecture of secure communication and high-performance computation.
Coherent control of the multiple wavelength lasing of N2+: coherence transfer and beyond
Nitrogen molecules pumped by intense femtosecond laser pulses give rise to coherent emission in the forward direction at a series of wavelengths, coined “air lasing.” We demonstrate the coherent control of these emissions via a pair of seeding pulses at two different frequencies at low pressures, revealing a coherence transfer through vibrational motion. It is found that the injection of a 427.8 nm (391.4 nm) seeding pulse results in its amplification at the expense of the 391.4 nm (427.8 nm) signal, demonstrating a competition between the two spectral components of the emission from the upper level population. Moreover, when the delay between the seeding and pump pulses is finely tuned, the coherent control of both transitions is observed via the coherence transfer. A microscopic molecular relaxation model reproduces these observations, highlighting the crucial role of electronic and vibrational coherences, as well as their coupling, during the lasing action.
Photon superbunching, distinguished by second-order coherence values far exceeding the Gaussian thermal limit, represents a highly desirable resource for quantum optics and correlation-based imaging technologies. However, existing approaches typically rely on fragile experimental platforms, inefficient nonlinear conversion processes, or mechanically complex optical architectures. Here, we demonstrate a fully fiber-integrated superbunched random fiber laser (SRFL) in which intrinsic Rayleigh scattering cooperatively interacts with cascaded stimulated Brillouin scattering and quasi-phase-matched four-wave mixing to tailor extreme photon statistics. The SRFL generates a multi-wavelength comb, in which individual spectral components exhibit widely tunable photon bunching, with the second-order coherence g(2)(0) continuously controlled from ~1 to ~26 by tuning the pump power, spectral order and diffusion length. Moreover, we establish a direct correlation between photonic phase transitions (quantified by the Parisi overlap order parameter) and the emergence of superbunching, thereby bridging macroscopic disorder physics and microscopic photon statistics. Finally, we employ the superbunched emission for temporal ghost imaging, realizing high-fidelity temporal object reconstruction with a substantial reduction in required ensemble averaging. These findings validate random fiber lasers as a robust, scalable, and integrated platform for generating extreme photon statistics and unlock new avenues for correlation-enhanced photonic sensing and quantum optics investigations in complex photonic systems.
In the first part of this thesis, a detailed analysis of lasing in random multiple-light-scattering media with gain is presented. Random laser emission is analyzed using a time-dependent diffusion model for light propagating in the medium containing active atoms. We demonstrate the effects of scatterers to narrow the emission spectral linewidth and to shorten the emitted pulse duration at a specific threshold pump intensity. This threshold pump intensity decreases with scatterer density and excitation spot diameter, in excellent agreement with experimental results. The coherence properties of the random laser are studied using a generalized master equation. The random laser medium is treated as a collection of low quality-factor cavities, coupled by random photon diffusion. Laser-like coherence, on average, is demonstrated above a specific pumping threshold. We demonstrate that with stronger scattering, the pumping threshold for the transition from chaotic to isotropic coherent light emission decreases and enhanced optical coherence for the emitted light is achieved above threshold. The second part of this thesis presents a study of lasing in photonic crystals (PCs). The emission from an incoherently pumped atomic system in interaction with the electro-magnetic reservoir of a PC is analyzed using a set of generalized semiclassical Maxwell-Bloch equations. We demonstrate that the photonic band edge facilitates the enhancement of stimulated emission and the reduction of internal losses, leading to an important lowering of the laser threshold. In addition, an increase of the laser output at a photonic band edge is demonstrated. We next develop a detailed quantum theory of a coherently pumped two-level atom in a photonic band gap material, coupled to both a multi-mode wave-guide channel and a high-quality micro-cavity embedded within the PC. The cavity field characteristics are highly distinct from that of a corresponding high-Q cavity in ordinary vacuum. We demonstrate enhanced, inversionless, and nearly coherent light generation when the photon density of states (DOS) jump between the Mollow spectral components of atomic resonance fluorescence is large. In the case of a vanishing photon DOS on the lower Mollow sideband and no dipolar dephasing, the emitted photon statistics is Poissonian and the cavity field exhibits quadrature coherence.
Even though sunlight is by far the most abundant renewable energy source available to humanity, its dilute and variable nature has kept efficient ways to collect, store, and distribute this energy tantalisingly out of reach. Turning the incoherent energy supply provided by the Sun into a coherent laser beam would overcome several of the practical limitations inherent in using sunlight as a source of clean energy: laser beams travel nearly losslessly over large distances, and they are effective at driving chemical reactions which convert sunlight into chemical energy. Here we propose a bio-inspired blueprint for a novel type of laser with the aim of upgrading unconcentrated natural sunlight into a coherent laser beam. Our proposed design constitutes a novel and different path towards sunlight-pumped lasers. In order to achieve lasing with the extremely dilute power provided by natural sunlight, we here propose a laser medium comprised of molecular aggregates inspired by the architecture of natural photosynthetic complexes. Such complexes exhibit a very large internal efficiency in harvesting photons from a power source as dilute as natural sunlight. Specifically, we consider a hybrid structure, where photosynthetic complexes in purple bacteria ( Rhodobacter sphaeroides ) surround a suitably engineered molecular dimer composed of two strongly coupled chromophores. We show that if pumped by the surrounding photosynthetic complex, which efficiently collects and concentrates solar energy, the core dimer structure can reach population inversion, and reach the lasing threshold under natural sunlight. The design principles proposed here will also pave the way for developing other bio-inspired quantum devices.