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Journal of Experimental and Theoretical Physics

Probe-field spectroscopy in atomic media optically oriented in the ground state

A. V. Bezverbnyĭ, Vladimir S. Smirnov, Anatolii M Tumaikin

Published Jan 1, 1994• 0 citations
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The optical magnetic birefringence (Faraday) technique that can be used to study the anisotropy distributions of the angular momenta of photofragments produced in molecular photodissociation is compared theoretically and experimentally with the magnetic dichroism technique. The frame independent tensor form of the general expression describing the difference between an initial and a final polarization matrix of a probe light beam passing through the photofragment vapor is presented and analyzed. The procedure of detection of the photofragment electron orientation and alignment angular distributions by Doppler spectroscopy using each of the techniques is studied theoretically. The angular independent anisotropy orientation and alignment parameters describing photodissociation dynamics that can be determined from these studies are presented. It is shown that in principle each of the techniques can give the same information about the photodissociation dynamics; however, the birefringence technique has an undeniable advantage since it leads to an increase in accuracy of the experimental data. Both magnetic birefringence and magnetic dichroism techniques were used experimentally to study the spin orientation of ground state Rb atoms produced in photodissociation of RbI at 266 nm by circularly polarized laser light. The experiment was not of the Doppler spectroscopy type, but use of different 85 Rb and 87 Rb isotopes in the dissociation cell and in the probe light source allows detection of the oriented atomic photofragments separately by each of the techniques. Obtained experimental results are in agreement with the theoretical predictions. Contribution of the orientation of the Rb hyperfine structure energy states to the observed signals were also studied and treated theoretically. The initial degree of the electron spin orientation of the Rb atoms produced in the reaction was found to be P e = 0.11 ± 0.02.
A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground-state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field for the two-quantum transitions. The absorption or gain of an additional probe field is monitored as a function of its detuning from one of the fields which constitutes the pump field. Although the probe absorption spectrum displays features common to those found in pump-probe spectroscopy of single-quantum transitions, new interference effects are found to modify the spectrum. Many of these features can be explained within the context of a dressed-atom picture.
This article reviews the early investigations of Series on the resonance absorption and fluorescence of light by samples of oriented atoms dagger subjected to static and oscillatory magnetic fields. These investigations include experiments on optical-radiofrequency double resonance, light beats in double resonance, circulation of coherence in optical pumping, and time-biasing in level-crossing spectroscopy. It then describes some selected laser spectroscopy experiments involving the interaction of optically oriented atoms with static magnetic fields that were stimulated by the earlier work of Series, including experiments on hyperfine structure quantum beats, cascade quantum beats, ground-state quantum beats in transmission, and optogalvanic detection of atomic coherences. Finally, it describes some current work which uses static magnetic fields to manipulate the external variables (momentum and position) of laser-cooled oriented atoms, with applications in the rapidly developing field of atom optics and atom interferometry.