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Exciton condensation with spontaneous time-reversal symmetry breaking

Congjun Wu, Ian Mondragon-Shem

Published Sep 20, 2008• 2 citations
OpenAlex

Abstract

According to the no-node theorem, many-body ground state wavefunctions of conventional Bose-Einstein condensations (BEC) are positive-definite, thus time-reversal symmetry cannot be spontaneously broken. We find that multi-component bosons with spin-orbit coupling provide an unconventional type of BECs beyond this paradigm. We focus on the subtle case of isotropic Rashba spin-orbit coupling and the spin-independent interaction. In the limit of the weak confining potential, the condensate wavefunctions are frustrated at the Hartree-Fock level due to the degeneracy of the Rashba ring. Quantum zero-point energy selects the spin-spiral type condensate through the order-from-disorder mechanism. In a strong harmonic confining trap, the condensate spontaneously generates a half-quantum vortex combined with the skyrmion type of spin texture. In both cases, time-reversal symmetry is spontaneously broken. These phenomena can be realized in both cold atom systems with artificial spin-orbit couplings generated from atom-laser interactions and exciton condensates in semi-conductor systems.

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We theoretically investigate the condensate state and collective excitations of a two-component Bose gas in a two-dimensional harmonic trap subject to isotropic Rashba spin-orbit coupling. In the weakly interacting regime when the interspecies interaction is larger than the intraspecies interaction (${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}>g$), we find that the condensate ground state has a half-quantum angular momentum vortex configuration with spatial rotational symmetry and skyrmion-type spin texture. Upon increasing the interatomic interaction beyond a threshold ${g}_{c}$, the ground state starts to involve higher-order angular momentum components and thus breaks rotational symmetry. In the case of ${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}<g$, the condensate becomes unstable toward the superposition of two degenerate half-quantum vortex states. Both instabilities (at $g>{g}_{c}$ and ${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}<g$) can be determined by solving the Bogoliubov equations for collective density oscillations of the half-quantum vortex state and by analyzing the softening of mode frequencies. We obtain the phase diagram as a function of the interatomic interactions and the spin-orbit coupling. In addition, we directly simulate the time-dependent Gross-Pitaevskii equation to examine the dynamical properties of the system. Finally, we investigate the stability of the half-quantum vortex state against both trap anisotropy and anisotropy in the spin-orbit coupling.

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According to the no-node theorem, many-body ground state wavefunctions of conventional Bose-Einstein condensations (BEC) are positive-definite, thus time-reversal symmetry cannot be spontaneously broken. We find that multi-component bosons with spin-orbit coupling provide an unconventional type of BECs beyond this paradigm. We focus on the subtle case of isotropic Rashba spin-orbit coupling and the spin-independent interaction. In the limit of the weak confining potential, the condensate wavefunctions are frustrated at the Hartree-Fock level due to the degeneracy of the Rashba ring. Quantum zero-point energy selects the spin-spiral type condensate through the order-from-disorder mechanism. In a strong harmonic confining trap, the condensate spontaneously generates a half-quantum vortex combined with the skyrmion type of spin texture. In both cases, time-reversal symmetry is spontaneously broken. These phenomena can be realized in both cold atom systems with artificial spin-orbit couplings generated from atom-laser interactions and exciton condensates in semi-conductor systems.
According to the “no-node" theorem, the many-body ground state wavefunctions of conventional Bose—Einstein condensations (BEC) are positive-definite, thus time-reversal symmetry cannot be spontaneously broken. We find that multi-component bosons with spin-orbit coupling provide an unconventional type of BECs beyond this paradigm. We focus on a subtle case of isotropic Rashba spin-orbit coupling and the spin-independent interaction. In the limit of the weak confining potential, the condensate wavefunctions are frustrated at the Hartree—Fock level due to the degeneracy of the Rashba ring. Quantum zero-point energy selects the spin-spiral type condensate through the “order-from-disorder" mechanism. In a strong harmonic confining trap, the condensate spontaneously generates a half-quantum vortex combined with the skyrmion type of spin texture. In both cases, time-reversal symmetry is spontaneously broken. These phenomena can be realized in both cold atom systems with artificial spin-orbit couplings generated from atom-laser interactions and exciton condensates in semi-conductor systems.
According to the no-node theorem, many-body ground state wavefunctions of conventional Bose-Einstein condensations (BEC) are positive-definite, thus time-reversal symmetry cannot be spontaneously broken. We find that multi-component bosons with spin-orbit coupling provide an unconventional type of BECs beyond this paradigm. We focus on the subtle case of isotropic Rashba spin-orbit coupling and the spin-independent interaction. In the limit of the weak confining potential, the condensate wavefunctions are frustrated at the Hartree-Fock level due to the degeneracy of the Rashba ring. Quantum zero-point energy selects the spin-spiral type condensate through the order-from-disorder mechanism. In a strong harmonic confining trap, the condensate spontaneously generates a half-quantum vortex combined with the skyrmion type of spin texture. In both cases, time-reversal symmetry is spontaneously broken. These phenomena can be realized in both cold atom systems with artificial spin-orbit couplings generated from atom-laser interactions and exciton condensates in semi-conductor systems.
Feynman's "no-node" theorem states that the conventional many-body ground state wavefunctions of bosons in the coordinate representation are positive definite. This implies that time-reversal symmetry cannot be spontaneously broken. In this article, we review our progress in studying a class of new states of unconventional Bose–Einstein condensations beyond this paradigm. These states can either be the long-lived metastable states of ultracold bosons in high orbital bands in optical lattices as a result of the "orbital Hund's rule" interaction, or the ground states of spinful bosons with spin-orbit coupling linearly dependent on momentum. In both cases, Feynman's argument does not apply. The resultant many-body wavefunctions are complex-valued and thus break time-reversal symmetry spontaneously. Exotic phenomena in these states include the Bose–Einstein condensation at nonzero momentum, the ordering of orbital angular momentum moments, the half-quantum vortex, and the spin texture of skyrmions.
The spin–orbit coupling with bosons gives rise to novel properties that are absent in usual bosonic systems. Under very general conditions, the conventional ground state wavefunctions of bosons are constrained by the ‘no-node’ theorem to be positive definite. In contrast, the linear dependence of the spin–orbit coupling leads to complex-valued condensate wavefunctions beyond this theorem. In this paper, we review the study of this class of unconventional Bose–Einstein condensations focusing on their topological properties. Both the 2D Rashba and 3D -type Weyl spin–orbit couplings give rise to Landau-level-like quantization of single-particle levels in the harmonic trap. Interacting condensates develop the half-quantum vortex structure spontaneously breaking the time-reversal symmetry and exhibit topological spin textures of the skyrmion type. In particular, the 3D Weyl coupling generates topological defects in the quaternionic phase space as an SU(2) generalization of the usual U(1) vortices. Rotating spin–orbit-coupled condensates exhibit rich vortex structures due to the interplay between vorticity and spin texture. In the Mott-insulating states in optical lattices, quantum magnetism is characterized by the Dzyaloshinskii–Moriya-type exchange interactions.
Motivated by the goal of realizing spin-orbit coupling (SOC) beyond one dimension, we propose and analyze a method to generate effective two-dimensional SOC in bilayer BECs with laser-assisted interlayer tunneling. We show that interplay among the interlayer tunneling, SOC, and intralayer atomic interaction can give rise to diverse ground-state configurations. In particular, the system undergoes a transition to a different type of stripe phase which spontaneously breaks the time-reversal symmetry. Different from the ordinary Rashba-type SOC, a fractionalized skyrmion lattice emerges spontaneously in the bilayer system without external traps. Furthermore, we predict the occurrence of a tetracritical point in the phase diagram of the bilayer BECs, where four phases merge. The origin of the different emerging phases is elucidated.
We theoretically investigate the condensate state and collective excitations of a two-component Bose gas in a two-dimensional harmonic trap subject to isotropic Rashba spin-orbit coupling. In the weakly interacting regime when the interspecies interaction is larger than the intraspecies interaction (${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}>g$), we find that the condensate ground state has a half-quantum angular momentum vortex configuration with spatial rotational symmetry and skyrmion-type spin texture. Upon increasing the interatomic interaction beyond a threshold gc{g}_{c}gc​, the ground state starts to involve higher-order angular momentum components and thus breaks rotational symmetry. In the case of ${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}<g$, the condensate becomes unstable toward the superposition of two degenerate half-quantum vortex states. Both instabilities (at g>gcg>{g}_{c}g>gc​ and ${g}_{\ensuremath{\uparrow}\ensuremath{\downarrow}}<g$) can be determined by solving the Bogoliubov equations for collective density oscillations of the half-quantum vortex state and by analyzing the softening of mode frequencies. We obtain the phase diagram as a function of the interatomic interactions and the spin-orbit coupling. In addition, we directly simulate the time-dependent Gross-Pitaevskii equation to examine the dynamical properties of the system. Finally, we investigate the stability of the half-quantum vortex state against both trap anisotropy and anisotropy in the spin-orbit coupling.