Long-lived Stark states detected at a positive energy

В. В. Колосов

M. H. Rayment, S. D. Hogan

Nitric oxide (NO) molecules in pulsed supersonic beams have been excited to long-lived Rydberg-Stark states in series converging to the lowest vibrational level in the ground electronic state of NO+ with rotational quantum numbers N+ = 2, 4, and 6. The molecules in these excited states were then guided, or decelerated and trapped in a chip-based Rydberg-Stark decelerator, and detected in situ by pulsed electric field ionization. Time constants, reflecting the decay of molecules in N+ = 2 Rydberg-Stark states, with principal quantum numbers n between 38 and 44, from the electrostatic traps were measured to be ∼300μs. Molecules in Rydberg-Stark states with N+ = 4 and 6, and the same range of values of n were too short-lived to be trapped, but their decay time constants could be determined from complementary sets of delayed pulsed electric field ionization measurements to be ∼100 and ∼25 μs, respectively.

Stefan G. Fischer, Yigal Meir, Yuval Gefen +1 more

Ergodic many-body systems are expected to reach thermal equilibrium. Here, we demonstrate that, surprisingly, high-energy electrons, which are injected into a quantum Hall edge mode with finite-range interactions, stabilize at a far-from-thermalized state over a long timescale. To detect this nonequilibrium state, one positions an energy-resolved detector downstream of the injection point. So far, nonequilibrium distributions in integrable systems were either found not to display relaxation at all, or generically relax to near-thermal asymptotic states. In stark contrast, the here-obtained many-body state comprises fast-decaying transient components, followed by a nearly frozen distribution with a peak near the injection energy.

В. В. Колосов

Thomas E. Wall, A. Alonso, B. S. Cooper +3 more

Rydberg positronium (Ps) atoms have been prepared in selected Stark states via two-step (1s→2p→nd/ns) optical excitation. Two methods have been used to achieve Stark-state selection: a field ionization filter that transmits the outermost states with positive Stark shifts, and state-selected photoexcitation in a strong electric field. The former is demonstrated for n=17 and 18 while the latter is performed for n=11 in a homogeneous electric field of 1.9 kV/cm. The observed spectral intensities and their dependence on the polarization of the laser radiation are in agreement with calculations that include the perturbations of the intermediate n=2 manifold. Our results pave the way for the generation of Rydberg Ps atoms with large electric dipole moments that are required for the realization of schemes to control their motion using inhomogeneous electric fields, an essential feature of some proposed Ps free-fall measurements requiring focused beams of long-lived atoms.

Dominique Delande