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APS

A study of adiabatic population transfer for the production of heavy Rydberg systems

Jeffrey N. Philippson, Ralph C. Shiell

Published Jun 1, 2007• 0 citations
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The light-induced adiabatic population transfer of holes from the heavy-hole ( $\mathrm{hh}$) to the light-hole ( $\mathrm{lh}$) band in p-doped semiconductor quantum wells is investigated theoretically. The exact analog to the population-trapped state (PTS) used in atomic and molecular adiabatic population transfer does not exist in a semiconductor due to the continuum of transition energies and the dynamic light-induced shifts thereof. However, it is found that the population transfer only requires an approximate PTS condition to be fulfilled. As for a possible observation of the effect, the transient creation of a $\mathrm{hh}$ exciton resonance at the expense of the $\mathrm{lh}$ exciton is predicted.

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Multiphoton population transfer in a kicked Rydberg atom: adiabatic rapid passage by separatrix crossing

Türker Topçu, F. Robicheaux

Following an experimental observation, a recent simulation has shown that efficient population transfer can be achieved through adiabatic chirping of a microwave pulse through a 10-photon resonance connecting two Rydberg states with n = 72, ℓ = 1 and n ∼ 82. These simulations have revealed that this population transfer is essentially a classical transition caused by separatrix crossing in the classical phase space. Here, we present the results of our fully three-dimensional quantum and classical simulations of coherent multiphoton population transfer in a kicked Li atom in a Rydberg state. We were able to achieve ∼76% population transfer from the 40p to 46p state in Li through a 6-photon resonance and contrast our results with those when the transition is driven by microwaves. We further discuss the case when the atom starts out from a Stark state in conjunction with the ℓ-distribution of the transferred population. We use a one-dimensional classical model to investigate the classical processes taking place in the phase space and find that the same separatrix crossing mechanism observed in microwave transitions is also responsible for the transition when the atom is kicked.

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Production of Rydberg Atoms

Thomas F. Gallagher

Experimental methods in the physical sciences•Jan 1, 1996•3 citations
The light-induced adiabatic population transfer of holes from the heavy-hole ( hh\mathrm{hh}hh) to the light-hole ( lh\mathrm{lh}lh) band in p-doped semiconductor quantum wells is investigated theoretically. The exact analog to the population-trapped state (PTS) used in atomic and molecular adiabatic population transfer does not exist in a semiconductor due to the continuum of transition energies and the dynamic light-induced shifts thereof. However, it is found that the population transfer only requires an approximate PTS condition to be fulfilled. As for a possible observation of the effect, the transient creation of a hh\mathrm{hh}hh exciton resonance at the expense of the lh\mathrm{lh}lh exciton is predicted.
Following an experimental observation, a recent simulation has shown that efficient population transfer can be achieved through adiabatic chirping of a microwave pulse through a 10-photon resonance connecting two Rydberg states with n = 72, ℓ = 1 and n ∼ 82. These simulations have revealed that this population transfer is essentially a classical transition caused by separatrix crossing in the classical phase space. Here, we present the results of our fully three-dimensional quantum and classical simulations of coherent multiphoton population transfer in a kicked Li atom in a Rydberg state. We were able to achieve ∼76% population transfer from the 40p to 46p state in Li through a 6-photon resonance and contrast our results with those when the transition is driven by microwaves. We further discuss the case when the atom starts out from a Stark state in conjunction with the ℓ-distribution of the transferred population. We use a one-dimensional classical model to investigate the classical processes taking place in the phase space and find that the same separatrix crossing mechanism observed in microwave transitions is also responsible for the transition when the atom is kicked.