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Two-level Gas Laser with Coherent Optical Pumping

Nicolai G. Basov, Vladilen S Letokhov

Published Jun 1, 1969• 0 citations
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We report magneto-optical rotation due to the interaction of atoms with a resonance laser beam. Our experiment is performed on the excited He states, 23P-33D transition, (lambda) equals 587,56nm. Two processes are responsible for the magneto-optical activity: the Zeeman coherences, induced in the absorbing level, and the optical pumping processes, each of them due to the laser beam excitation. The Zeeman coherence creates peaks with a width determined by the coherence relaxation rate, while the optical pumping creates a structure with a width in the order of the natural width of the transition. Due to the difference between the relaxation rates of the 2P and 3D He levels, the two parts of signal are well resolved and depend on the He pressure in different ways. The narrow coherence signal disappears at high He pressure, unless the amplitude of the optical pumping signal increases. The optical pumping signals saturates as He pressure increased and changes its sign. At high gas pressures, such that only the optical pumping signal exists, an increase of the He pressure leads to the narrowing of both the 'classical parabolic dependence' and the optical pumping signal.

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Atomic coherence gives rise to a series of interesting phenomena in quantum optics.1 In this work we investigate coherence effects within the Na Dl line, demonstrating coherent trapping and lasing without inversion, and study the dependence of these phenomena on buffer gas pressure. Two pump laser beams (I, and I2) are tuned to the frequencies υ1 and υ2 that correspond to the 3S1/2 (F=1, 2) → 3P1/2 transition and are right circularly polarized. Pockels cells are used to turn on or/and off the beams within approximately one nanosecond. To demonstrate lasing without inversion, a weak pulse of left polarized light tuned to t)2 was used to create a small population in the upper level (3P1/2) and the amplification of I, was observed. We found a significant gain in the absence of population inversion, which was verified by a direct experimental observation. These results were observed as a function of buffer gas pressure. The atomic coherence effects are shown to disappear in the presence of a helium buffer gas at a pressure of ≈ 1 Torr; whereas, complete optical pumping is only achieved at helium buffer gas pressures >10 Torr.

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Possibility of inversionless amplification and generation of radiation by a two-level system in the ‘red’ wing of its spectral line under resonant diode pumping

А. И. Пархоменко, Anatolii M. Shalagin

We report a theoretical study on the possibility of amplification and generation of radiation by an inversionless two-level system in the ‘red’ wing of its spectral line under resonant diode pumping. The two-level system is used to simulate atoms of an active gas, while it is in the atmosphere of a high-pressure buffer gas. The effect results from the fact that the probability of stimulated emission in the ‘red’ wing of the spectral line exceeds the probability of absorption if the homogeneous broadening due to the interaction of particles with the buffer gas significantly exceeds the natural one (at high pressures of the buffer gas). It is found that the higher the buffer gas pressure and the higher the pump radiation intensity, the greater the inversionless amplification. It is shown that the gain in a two-level system in the ‘red’ wing of its spectral line can reach 0.011 cm −1 when the radiation intensity and the width of the radiation spectrum of pump diodes are 5 kW cm −2 and 4 cm −1 , respectively. The use of transverse diode pumping of an active medium placed in an optical cavity will make it possible to obtain lasing with frequency tuning and thereby solve the problem of converting incoherent broadband radiation into a coherent laser light in a gas of two-level active particles.

Quantum Electronics•Sep 27, 2021•3 citations
We report magneto-optical rotation due to the interaction of atoms with a resonance laser beam. Our experiment is performed on the excited He states, 23P-33D transition, (lambda) equals 587,56nm. Two processes are responsible for the magneto-optical activity: the Zeeman coherences, induced in the absorbing level, and the optical pumping processes, each of them due to the laser beam excitation. The Zeeman coherence creates peaks with a width determined by the coherence relaxation rate, while the optical pumping creates a structure with a width in the order of the natural width of the transition. Due to the difference between the relaxation rates of the 2P and 3D He levels, the two parts of signal are well resolved and depend on the He pressure in different ways. The narrow coherence signal disappears at high He pressure, unless the amplitude of the optical pumping signal increases. The optical pumping signals saturates as He pressure increased and changes its sign. At high gas pressures, such that only the optical pumping signal exists, an increase of the He pressure leads to the narrowing of both the 'classical parabolic dependence' and the optical pumping signal.
Atomic coherence gives rise to a series of interesting phenomena in quantum optics.1 In this work we investigate coherence effects within the Na Dl line, demonstrating coherent trapping and lasing without inversion, and study the dependence of these phenomena on buffer gas pressure. Two pump laser beams (I, and I2) are tuned to the frequencies υ1 and υ2 that correspond to the 3S1/2 (F=1, 2) → 3P1/2 transition and are right circularly polarized. Pockels cells are used to turn on or/and off the beams within approximately one nanosecond. To demonstrate lasing without inversion, a weak pulse of left polarized light tuned to t)2 was used to create a small population in the upper level (3P1/2) and the amplification of I, was observed. We found a significant gain in the absence of population inversion, which was verified by a direct experimental observation. These results were observed as a function of buffer gas pressure. The atomic coherence effects are shown to disappear in the presence of a helium buffer gas at a pressure of ≈ 1 Torr; whereas, complete optical pumping is only achieved at helium buffer gas pressures >10 Torr.
We report a theoretical study on the possibility of amplification and generation of radiation by an inversionless two-level system in the ‘red’ wing of its spectral line under resonant diode pumping. The two-level system is used to simulate atoms of an active gas, while it is in the atmosphere of a high-pressure buffer gas. The effect results from the fact that the probability of stimulated emission in the ‘red’ wing of the spectral line exceeds the probability of absorption if the homogeneous broadening due to the interaction of particles with the buffer gas significantly exceeds the natural one (at high pressures of the buffer gas). It is found that the higher the buffer gas pressure and the higher the pump radiation intensity, the greater the inversionless amplification. It is shown that the gain in a two-level system in the ‘red’ wing of its spectral line can reach 0.011 cm −1 when the radiation intensity and the width of the radiation spectrum of pump diodes are 5 kW cm −2 and 4 cm −1 , respectively. The use of transverse diode pumping of an active medium placed in an optical cavity will make it possible to obtain lasing with frequency tuning and thereby solve the problem of converting incoherent broadband radiation into a coherent laser light in a gas of two-level active particles.