Ultracold interacting gases represent a new and exciting frontier for technological applications, such as quantum information processing, and they also offer an ideal test bench for condensed matter systems. \nThis work examines the case of atoms in the alkaline earth metal family. These atoms can exhibit long-range dipolar interactions, generated via coherent exchange of photons on the 3P0 ! 3D1 transition. In particular, the progress in realising an experiment to study this coherent exchange of atoms in bosonic strontium is discussed. A review of the experimental techniques developed over the last 50 years to cool, manipulate and study atoms and molecules used in long-range interaction experiments is given from a historical viewpoint. Techniques to laser cool and trap atomic strontium are described, and a novel study of different geometries for magneto-optical traps (MOTs) is presented. \nThis thesis describes the long-range interaction strontium experiment under development at the University of Birmingham. In particular, the characterisation of a self assembled Zeeman slower is presented, along with a novel repump scheme for the first stage of cooling using the 3P0 ! 3D1 transition. \nThis work also reports the use of the 3P1 ! 3S1 transition to populate the 3P0 level, and the realisation of a monolithic (Interference Filter External \nCavity Diode Laser) IFECDL. \nThe new techniques that I present here have the potential to facilitate future studies of long-range interaction in strontium and other cold atoms experiments.
Ultracold interacting gases represent a new and exciting frontier for technological applications, such as quantum information processing, and they also offer an ideal test bench for condensed matter systems. \nThis work examines the case of atoms in the alkaline earth metal family. These atoms can exhibit long-range dipolar interactions, generated via coherent exchange of photons on the 3P0 ! 3D1 transition. In particular, the progress in realising an experiment to study this coherent exchange of atoms in bosonic strontium is discussed. A review of the experimental techniques developed over the last 50 years to cool, manipulate and study atoms and molecules used in long-range interaction experiments is given from a historical viewpoint. Techniques to laser cool and trap atomic strontium are described, and a novel study of different geometries for magneto-optical traps (MOTs) is presented. \nThis thesis describes the long-range interaction strontium experiment under development at the University of Birmingham. In particular, the characterisation of a self assembled Zeeman slower is presented, along with a novel repump scheme for the first stage of cooling using the 3P0 ! 3D1 transition. \nThis work also reports the use of the 3P1 ! 3S1 transition to populate the 3P0 level, and the realisation of a monolithic (Interference Filter External \nCavity Diode Laser) IFECDL. \nThe new techniques that I present here have the potential to facilitate future studies of long-range interaction in strontium and other cold atoms experiments.
Alkaline-earth-metal atoms can exhibit long-range dipolar interactions, which are generated via the coherent exchange of photons on the (3)P(0) - (3)D(1) transition of the triplet manifold. In the case of bosonic strontium, which we discuss here, this transition has a wavelength of 2.6 μm and a dipole moment of 4.03 D, and there exists a magic wavelength permitting the creation of optical lattices that are identical for the states (3)P(0) and (3)D(1). This interaction enables the realization and study of mixtures of hard-core lattice bosons featuring long-range hopping, with tunable disorder and anisotropy. We derive the many-body master equation, investigate the dynamics of excitation transport, and analyze spectroscopic signatures stemming from coherent long-range interactions and collective dissipation. Our results show that lattice gases of alkaline-earth-metal atoms permit the creation of long-lived collective atomic states and constitute a simple and versatile platform for the exploration of many-body systems with long-range interactions. As such, they represent an alternative to current related efforts employing Rydberg gases, atoms with large magnetic moment, or polar molecules.
We describe the operation and performance of an ultracold strontium apparatus that is capable of generating quantum degenerate gases. The experiment has produced Bose-Einstein condensates (BECs) of 84Sr and 86Sr as well as degenerate Fermi gases (DFGs) of 87Sr with a reduced temperature of T/TF = 0.2 at a Fermi temperature of TF = 55 nK. Straightforward modifications could be made to allow for isotopic mixtures and BECs of the fourth stable isotope, 88Sr. We also report on a technique to improve the continuous loading of a magnetic trap by adding a laser tuned to the 3P1 - 3S1 transition. The method increases atom number in the magnetic trap and subsequent cooling stages by up to 65% for the bosonic isotopes and up to 30% for the fermionic isotope of strontium. We optimize this trap loading strategy with respect to laser detuning, intensity, and beam size. To understand the results, we develop a one-dimensional rate equation model of the system, which is in good agreement with the data. We discuss the use of other transitions in strontium for accelerated trap loading and the application of the technique to other alkaline-earth-like atoms. Finally, we also report on an updated investigation of photoassociation resonances relative to the 1S0 + 3P1 dissassociation limit in bosonic strontium. Multiple new resonances for 84Sr and 86Sr were measured out to binding energies of -5 GHz and several discrepancies in earlier measurements were resolved. These measurements will allow for the development of a more accurate mass-scaled model and a better theoretical understanding of the molecular potentials near the 3P1 state. We also measure the strength of the 84Sr 0u transitions in order to characterize their use as optical Feshbach resonances.
This thesis describes Rydberg spectroscopy and dressing experiments in an ultracold strontium gas. The strontium atoms are cooled to sub-uK temperatures in a narrowline magneto-optical trap, where Rydberg atoms are created using a two-photon excitation scheme. This required the development of a high-power ultraviolet laser system at 319 nm. The laser has a large tuning range for access to triplet Rydberg states from principal quantum numbers of 35 to > 300. By performing Rydberg spectroscopy in a magneto-optical trap, we show that narrow spectra can be obtained where the line centre is determined to ~ 10 kHz. A frequency comb is then employed to make absolute frequency measurements of optical transitions to accuracies of < 2 MHz. Techniques are outlined for improving the accuracy further, showing that overall uncertainties on the order of 10 kHz can be obtained. The reliable measurement of Rydberg levels is important for studying the variation in quantum defect across Rydberg series, and hence improving the accuracy of atomic models. In this work we also develop a novel system in which to realise Rydberg dressing. By resonantly coupling the excited state of the cooling transition to a high lying Rydberg state, we create a Rydberg-dressed magneto-optical trap. We demonstrate that the atoms acquire Rydberg properties, while undergoing continuous cooling at ~ 1 uK. The lifetime of the trap is proved to be sufficiently long to observe interactions, however the interaction strength is currently limited by the non-uniform spatial profile of the dressing beam. Straightforward methods to overcome this limitation are presented. As such this work should lead to future experiments, whereby tuneable long-range interactions can be observed in the dynamics of the dressed magneto-optical trap.
We describe the construction and characterization of a new apparatus that can produce degenerate quantum gases of strontium. The realization of degenerate gases is an important first step toward future studies of quantum magnetism. Three of the four stable isotopes of strontium have been cooled into the degenerate regime. The experiment can make nearly pure Bose-Einstein condensates containing approximately 1x10^4 atoms, for strontium-86, and approximately 4x10^5 atoms, for strontium-84. We have also created degenerate Fermi gases of strontium-87 with a reduced temperature, T/T_F of approximately 0.2. The apparatus will be able to produce Bose-Einstein condensates of strontium-88 with straightforward modifications. We also report the first experimental and theoretical results from the strontium project. We have developed a technique to accelerate the continuous loading of strontium atoms into a magnetic trap. By applying a laser addressing the 3P1 to 3S1 transition in our magneto-optical trap, the rate at which atoms populate the magnetically-trapped 3P2 state can be increased by up to 65%. Quantum degenerate gases of atoms in the metastable 3P0 and 3P2 states are a promising platform for quantum simulation of systems with long-range interactions. We have performed an initial numerical study of a method to transfer the ground state degenerate gases that we can currently produce into one of the metastable states via a three-photon transition. Numerical simulations of the Optical Bloch equations governing the three-photon transition indicate that >90% of a ground state degenerate gas can be transferred into a metastable state.
Ultracold polar molecules have emerged as promising platforms for quantum simulation, quantum information science, precision measurements of fundamental symmetry violations, and quantum chemistry. Over the past decade, rapid progress in direct laser cooling of molecules has enabled new capabilities such as magneto-optical traps (MOTs), sub-Doppler cooling, and optical dipole traps (ODTs), expanding the quantum toolbox with ultracold molecules of complex internal structures and strong dipolar interactions. This thesis presents the design, construction, and operation of an experiment on ultracold strontium monofluoride (88Sr19F) molecules, demonstrating state-of-the-art techniques for molecular laser cooling and trapping. The apparatus integrates a broad range of technical sub-systems, including cryogenics, ultra-high vacuum, optics, electronics, and automated laboratory control software. SrF molecules produced in a slowed cryogenic buffer gas beam are captured into a dual-frequency MOT. Subsequent Λ-enhanced gray molasses cooling reduces the molecule temperature to as low as 5 μK. A novel blue-detuned MOT is also implemented to further compress the molecular cloud, increasing the density by a factor of ∼ 400. At this high density, SrF molecules are efficiently loaded into an ODT, a tight, conservative trap with long lifetimes. Population transfer between different rotational levels is achieved via optical pumping and coherent microwave control, yielding ∼ 0.8 ms coherence time in Rabi oscillation and ∼ 90 % transfer efficiency. This thesis also describes the development of an ultracold rubidium (87Rb) atom experiment, in which a loading rate of ∼ 10^10 atoms/s into a radio-frequency (RF) MOT is demonstrated. A modular two-dimensional MOT serves as the Rb source and can be seamlessly integrated into the SrF apparatus, opening the possibility for future studies of co-trapping and sympathetic cooling of SrF molecules with atoms. The results presented in this thesis establish an experimental foundation for exploring new frontiers in ultracold molecular physics.
The optical lattice clock with neutral atoms occupies an outstanding position in the research field of atomic clocks, demonstrating the great potential of its performance (like the uncertainty and the stability). At present, the optical lattice clock has realized a 10-18 level of its uncertainty. In this paper, we present the realization of loading bosonic atoms 88Sr (strontium, alkaline-earth metals) into a one-dimensional (1D) optical lattice in our laboratory. The optical lattice where the atoms are trapped can make the energy level shift, called Stark shift. But there is the special optical lattice operating at the “magic” wavelength for clock transitions (5s2) 1S0-(5s5p) 3P0, which can make the same Stark light-shift for both of them, indicating a zero light-shift relative to the clock. In our experiment, Sr atoms are cooled in a two-stage cooling and its temperature can be as low as 2 μK. Then these cold atoms are confined in the Lamb-Dicke region by the lattice laser output from an amplified diode laser operating at the “magic” wavelength, 813 nm. Experimentally, it is straightforward to provide 850 mW of lattice power focused to a 38 μm beam radius. After the cold atoms have trapped in the optical lattice, the lifetime of atoms in 1D optical lattice is measured to be 270 ms. The temperature and the number are about 3.5 μK and 1.2×105 respectively. Besides, effects of the power of the lattice laser on both the number and temperature are analyzed. The number changes linearly with the laser power, while there is no obvious influence on the temperature by the power. This original and special approach for atoms trapped in the optical lattice can provide a long interrogation time for probing the clock transition. Furthermore, it may be the foundation for developing our optical lattice clock of strontium atoms.