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QUANTUM MONTE CARLO STUDY OF BOSONIC LATTICE SYSTEMS IN THE PRESENCE OF DISORDER

Chao Zhang

Published Aug 30, 2018• 0 citations
OpenAlex

Abstract

Disorder is ubiquitous in condensed matter systems, but a thorough understanding of these systems is hindered by poor control over the nature of disorder and competing interactions. Ultracold gases trapped in optical lattices, on the other hand, offer an unprecedented level of control over interactions and disorder, and are ideal candidates to test theoretical predictions and study fascinating phenomena resulting from the interplay between disorder, interaction, and quantum degeneracy. In this dissertation, I present my research on strongly correlated many-body lattice bosons in the presence of disordered potentials. My results are based on quantum Monte Carlo simulations by the Worm algorithm. Experimentally, lattice bosons can be realized by ultracold gases in optical lattices. I studied the ground state phase diagram of the above systems in the presence of diagonal (quasi-periodic disordered potential or random disordered potential) and off-diagonal disorder (in the form of site dilution). First, I will discuss the ground state phase diagram of two-dimensional bosons in quasi-periodic lattices. Then, I will discuss the phase diagram as well as finite temperature thermodynamic properties of two-dimensional dipolar lattice bosons in the presence of random diagonal disordered potentials. Finally, I will discuss the phase diagram of two-dimensional hard-core lattice bosons system in the presence of long-range hopping and long-range two-body interactions both in the absence of disorder and in the presence of site dilution (equivalent to off-diagonal disorder). This system is equivalent to the long-range XXZ model as realized by polar molecules trapped in a deep optical lattice. These results provide theoretical guidance for experimentalists to find quantum phase transitions as well as exotic quantum phases in strongly correlated bosonic lattice systems.

Related papers

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This dissertation serves as a summary of my Ph.D. work numerically studying equilibrium and non-equilibrium properties of strongly-interacting one-dimensional (1D) boson systems. This work is motivated by the fact that 1D systems are realizable and highly controllable with ultracold atoms in optical lattice and atom chip experiments. We apply a recent worm algorithmic Monte Carlo approach developed for 1D continuous systems to study their equilibrium properties, both with and without an underlying lattice. We also apply an exact lattice approach based on the Bose-Fermi mapping to check our Monte Carlo results in the Tonks-Girardeau limit, and more importantly, to study far-from-equilibrium expansion dynamics of the systems. We first study the scaling of one-particle correlations of the harmonically trapped Lieb-Liniger gas with changing temperature and interaction strength. Based on the universal behaviors of the density and momentum profiles, we are able to determine the effective parameters needed to fully characterize the system. We also find that the Tonks-Girardeau limit at low temperatures is the ideal regime for the experimental observation of the $1/k^4$ momentum tail. An extra periodic lattice can drive the transition from superfluid to Mott insulator states. Exact and complete phase diagrams for such transitions are available only in the weak interacting and deep lattice limit, in which the system can be described using one-band Bose-Hubbard model. Beyond this limit, we use the worm algorithm in continuous space to map out the phase diagrams at various interaction strengths. We compare our phase diagrams with one-band Bose-Hubbard predictions and identify the regime where the one-band description breaks down. We introduce an inverse confined scattering solution to obtain effective Hubbard parameters, with which the Bose-Hubbard model provides correct results for strong interactions and deep lattices at unit filling. In addition to the equilibrium properties, we also study the expansion dynamics of ultracold atoms in the hard-core limit. Experimentally, this is usually achieved by turning off confining potentials and letting atoms expand in optical lattices. Theoretical studies from initial ground states predicted the occurrence of fermionization of the momentum distribution after long expansion times. In addition, quasicondensation at finite momenta emerges when expanding from Mott insulating domains. Here, we develop a finite-temperature extension of the lattice approach for dynamics. We find the dynamical ferminoization of the momentum distributions at all temperatures. For expansion from initial Mott domains, we observe enhanced correlations reminiscent of dynamical quasicondensation. Surprisingly, we find the systems appear to cool down during the melting of the Mott domains. We use an emergent local Hamiltonian to understand these emergent phenomena.

•Jan 1, 2018•0 citations

Equilibrium phases of dipolar lattice bosons in the presence of random diagonal disorder

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Ultracold gases offer an unprecedented opportunity to engineer disorder and interactions in a controlled manner. In an effort to understand the interplay between disorder, dipolar interactions, and quantum degeneracy, we study two-dimensional hard-core dipolar lattice bosons in the presence of on-site bound disorder. Our results are based on large-scale path-integral quantum Monte Carlo simulations by the worm algorithm. We study the ground-state phase diagram at a fixed half-integer filling factor for which the clean system is either a superfluid at a lower dipolar interaction strength or a checkerboard solid at a larger dipolar interaction strength. We find that, even for weak dipolar interactions, superfluidity is destroyed in favor of a Bose glass at a relatively low disorder strength. Interestingly, in the presence of disorder, superfluidity persists for values of the dipolar interaction strength for which the clean system is a checkerboard solid. At a fixed disorder strength, as the dipolar interaction is increased, superfluidity is destroyed in favor of a Bose glass. As the interaction is further increased, the system eventually develops extended checkerboard patterns in the density distribution. Due to the presence of disorder, though, grain boundaries and defects, responsible for a finite residual compressibility, are present in the density distribution. Finally, we study the robustness of the superfluid phase against thermal fluctuations.

arXiv:1711.04879•Physical Review A•Jan 16, 2018•8 citations

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"This thesis presents research on a variety of dynamical phenomena in strongly correlated systems. We use 87Rb atoms trapped in a disordered optical lattice to realize the 3D Bose Hubbard model, with independently, dynamically tunable lattice depth and disorder strength. The equilibrium behavior of the Bose Hubbard and disordered Bose Hubbard models are understood, but there are many outstanding questions about dynamics. One area of interest is in dynamical behavior near quantum phase boundaries, such as the generation of quench-induced excitations in the presence of disorder. Another area concerns heat flow, relaxation, and thermalization. The primary focus of this thesis is driving a gas across a disorder-induced quantum phase transition from the Bose glass to the superfluid phase via quenching the disorder. We measured excitations generated during the quench and related them to crossing the equilibrium phase transition determined by quantum Monte Carlo simulations of the trapped system. The behavior we observe is reminiscent of the quantum Kibble Zurek mechanism, where the relaxation timescale diverges and local fluctuations are ""frozen"" into the system near the phase boundary. Understanding how disorder impacts the Kibble Zurek paradigm about behavior near a phase boundary provides insight into the dynamics of strongly interacting, disordered systems. The three other works discussed in this thesis concern relaxation and energy transfer in clean optical lattices. Understanding these dynamical properties of lattice gases is key to developing tools such as cooling in a lattice. In the first result, a gas comprised of two spin states was loaded into a spin-dependent optical lattice, such that one spin state experienced the lattice, and the other did not. We found that when the lattice gas was heated, energy transfer to the non-lattice gas did not occur at higher lattice depths due to the mismatch in the dispersion relations. In the second result, lattice atoms were excited to a higher band and found to decay to the ground state via two mechanisms. One decay channel involved generating excitations in the non-lattice atoms, while the other channel involved collisions between lattice atoms, where one atom decayed to the ground state and the other was excited to a higher band. The final result measured relaxation timescales by removing atoms with low quasimomentum and measuring rethermalization. The observed timescales are faster than the tunneling time and interaction time of the lattice. Proof-of-principle cooling was also demonstrated by removing atoms with higher quasimomentum and allowing the remaining atoms rethermalize to a cooler temperature."

•Apr 1, 2016•1 citation

Exotic quantum phenomena in cold atomic gases : numerical approaches

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The central aim of this thesis is the study of the low-energy and low-temperature properties of strongly correlated systems of bosonic particles interacting via finite- and long-range potentials, and relevant to experimental realization with cold atomic gases. This study is carried out with a combination of state-of-the-art numerical techniques such as Path Integral Monte Carlo and analytical techniques. The main result of my work is the demonstration of the existence of a stripe supersolid phase and of a rare transition between isotropic and anisotropic supersolids in a finite-range interacting model of hard-bosons on a square lattice. I also investigate the out-of-equilibrium scenarios of such models via simulated temperature quenches. Finally, I investigate how restoring energy extensivity in long-range interacting systems can have a profound incidence on the low-energy properties in the thermodynamic limit.

•Dec 6, 2019•0 citations

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•Jan 1, 2023•0 citations

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This thesis is devoted to the study of dipolar lattice gases, i.e. many-body quantum systems of particles with a strong magnetic or electric dipole moment in optical lattices. Such systems are adequately described by the extended Hubbard model, which accounts for inter-site dipole-dipole interactions (DDI). These interactions, due to their long-range and anisotropic character, result in rich groundstate physics and intriguing dynamics as we illustrate in this thesis for the particular case of bosons in one- and quasi-one-dimensional lattices. We start by focusing on the non-trivial role played by the transversal confinement in one-dimensional dipolar lattice gases. We show that weakening the transversal confinement enhances beyond-nearest-neighbor interactions. Then, we analyze how this affects the ground-state physics of hard-core bosons with repulsive dipolar interactions and reveal quantitative differences to the standard case of the DDI falling off as 1/r^3 where r is the inter-particle distance. With attractive interactions, a new quantum liquid phase of self-bound lattice droplets emerges without the need for super-exchange processes. In the soft-core regime, proper consideration of the transversal confinement not only quantitatively shifts phase boundaries, but introduces novel phases with peculiar correlations in the site occupancies that may be either topological or topologically trivial. Furthermore, we study the effect of the transversal confinement on the dynamical properties of one-dimensional hard-core bosons at half-filling. We show in particular that the localization-to-delocalization transition induced by Hilbert space fragmentation resembles that of a system with an effective power-law decay different from 1/r^3 which can be controlled by the transversal confinement. To conclude this thesis, we analyze ground-state properties of hard-core dipolar bosons in a square ladder at unit rung filling with an energy bias between the two legs. We show that the interplay between the energy bias and the dipolar tail results in a peculiar topological quantum floating phase.

•Jan 1, 2025•0 citations
Disorder is ubiquitous in condensed matter systems, but a thorough understanding of these systems is hindered by poor control over the nature of disorder and competing interactions. Ultracold gases trapped in optical lattices, on the other hand, offer an unprecedented level of control over interactions and disorder, and are ideal candidates to test theoretical predictions and study fascinating phenomena resulting from the interplay between disorder, interaction, and quantum degeneracy. In this dissertation, I present my research on strongly correlated many-body lattice bosons in the presence of disordered potentials. My results are based on quantum Monte Carlo simulations by the Worm algorithm. Experimentally, lattice bosons can be realized by ultracold gases in optical lattices. I studied the ground state phase diagram of the above systems in the presence of diagonal (quasi-periodic disordered potential or random disordered potential) and off-diagonal disorder (in the form of site dilution). First, I will discuss the ground state phase diagram of two-dimensional bosons in quasi-periodic lattices. Then, I will discuss the phase diagram as well as finite temperature thermodynamic properties of two-dimensional dipolar lattice bosons in the presence of random diagonal disordered potentials. Finally, I will discuss the phase diagram of two-dimensional hard-core lattice bosons system in the presence of long-range hopping and long-range two-body interactions both in the absence of disorder and in the presence of site dilution (equivalent to off-diagonal disorder). This system is equivalent to the long-range XXZ model as realized by polar molecules trapped in a deep optical lattice. These results provide theoretical guidance for experimentalists to find quantum phase transitions as well as exotic quantum phases in strongly correlated bosonic lattice systems.
This dissertation serves as a summary of my Ph.D. work numerically studying equilibrium and non-equilibrium properties of strongly-interacting one-dimensional (1D) boson systems. This work is motivated by the fact that 1D systems are realizable and highly controllable with ultracold atoms in optical lattice and atom chip experiments. We apply a recent worm algorithmic Monte Carlo approach developed for 1D continuous systems to study their equilibrium properties, both with and without an underlying lattice. We also apply an exact lattice approach based on the Bose-Fermi mapping to check our Monte Carlo results in the Tonks-Girardeau limit, and more importantly, to study far-from-equilibrium expansion dynamics of the systems. We first study the scaling of one-particle correlations of the harmonically trapped Lieb-Liniger gas with changing temperature and interaction strength. Based on the universal behaviors of the density and momentum profiles, we are able to determine the effective parameters needed to fully characterize the system. We also find that the Tonks-Girardeau limit at low temperatures is the ideal regime for the experimental observation of the 1/k41/k^41/k4 momentum tail. An extra periodic lattice can drive the transition from superfluid to Mott insulator states. Exact and complete phase diagrams for such transitions are available only in the weak interacting and deep lattice limit, in which the system can be described using one-band Bose-Hubbard model. Beyond this limit, we use the worm algorithm in continuous space to map out the phase diagrams at various interaction strengths. We compare our phase diagrams with one-band Bose-Hubbard predictions and identify the regime where the one-band description breaks down. We introduce an inverse confined scattering solution to obtain effective Hubbard parameters, with which the Bose-Hubbard model provides correct results for strong interactions and deep lattices at unit filling. In addition to the equilibrium properties, we also study the expansion dynamics of ultracold atoms in the hard-core limit. Experimentally, this is usually achieved by turning off confining potentials and letting atoms expand in optical lattices. Theoretical studies from initial ground states predicted the occurrence of fermionization of the momentum distribution after long expansion times. In addition, quasicondensation at finite momenta emerges when expanding from Mott insulating domains. Here, we develop a finite-temperature extension of the lattice approach for dynamics. We find the dynamical ferminoization of the momentum distributions at all temperatures. For expansion from initial Mott domains, we observe enhanced correlations reminiscent of dynamical quasicondensation. Surprisingly, we find the systems appear to cool down during the melting of the Mott domains. We use an emergent local Hamiltonian to understand these emergent phenomena.
Ultracold gases offer an unprecedented opportunity to engineer disorder and interactions in a controlled manner. In an effort to understand the interplay between disorder, dipolar interactions, and quantum degeneracy, we study two-dimensional hard-core dipolar lattice bosons in the presence of on-site bound disorder. Our results are based on large-scale path-integral quantum Monte Carlo simulations by the worm algorithm. We study the ground-state phase diagram at a fixed half-integer filling factor for which the clean system is either a superfluid at a lower dipolar interaction strength or a checkerboard solid at a larger dipolar interaction strength. We find that, even for weak dipolar interactions, superfluidity is destroyed in favor of a Bose glass at a relatively low disorder strength. Interestingly, in the presence of disorder, superfluidity persists for values of the dipolar interaction strength for which the clean system is a checkerboard solid. At a fixed disorder strength, as the dipolar interaction is increased, superfluidity is destroyed in favor of a Bose glass. As the interaction is further increased, the system eventually develops extended checkerboard patterns in the density distribution. Due to the presence of disorder, though, grain boundaries and defects, responsible for a finite residual compressibility, are present in the density distribution. Finally, we study the robustness of the superfluid phase against thermal fluctuations.
"This thesis presents research on a variety of dynamical phenomena in strongly correlated systems. We use 87Rb atoms trapped in a disordered optical lattice to realize the 3D Bose Hubbard model, with independently, dynamically tunable lattice depth and disorder strength. The equilibrium behavior of the Bose Hubbard and disordered Bose Hubbard models are understood, but there are many outstanding questions about dynamics. One area of interest is in dynamical behavior near quantum phase boundaries, such as the generation of quench-induced excitations in the presence of disorder. Another area concerns heat flow, relaxation, and thermalization. The primary focus of this thesis is driving a gas across a disorder-induced quantum phase transition from the Bose glass to the superfluid phase via quenching the disorder. We measured excitations generated during the quench and related them to crossing the equilibrium phase transition determined by quantum Monte Carlo simulations of the trapped system. The behavior we observe is reminiscent of the quantum Kibble Zurek mechanism, where the relaxation timescale diverges and local fluctuations are ""frozen"" into the system near the phase boundary. Understanding how disorder impacts the Kibble Zurek paradigm about behavior near a phase boundary provides insight into the dynamics of strongly interacting, disordered systems. The three other works discussed in this thesis concern relaxation and energy transfer in clean optical lattices. Understanding these dynamical properties of lattice gases is key to developing tools such as cooling in a lattice. In the first result, a gas comprised of two spin states was loaded into a spin-dependent optical lattice, such that one spin state experienced the lattice, and the other did not. We found that when the lattice gas was heated, energy transfer to the non-lattice gas did not occur at higher lattice depths due to the mismatch in the dispersion relations. In the second result, lattice atoms were excited to a higher band and found to decay to the ground state via two mechanisms. One decay channel involved generating excitations in the non-lattice atoms, while the other channel involved collisions between lattice atoms, where one atom decayed to the ground state and the other was excited to a higher band. The final result measured relaxation timescales by removing atoms with low quasimomentum and measuring rethermalization. The observed timescales are faster than the tunneling time and interaction time of the lattice. Proof-of-principle cooling was also demonstrated by removing atoms with higher quasimomentum and allowing the remaining atoms rethermalize to a cooler temperature."
The central aim of this thesis is the study of the low-energy and low-temperature properties of strongly correlated systems of bosonic particles interacting via finite- and long-range potentials, and relevant to experimental realization with cold atomic gases. This study is carried out with a combination of state-of-the-art numerical techniques such as Path Integral Monte Carlo and analytical techniques. The main result of my work is the demonstration of the existence of a stripe supersolid phase and of a rare transition between isotropic and anisotropic supersolids in a finite-range interacting model of hard-bosons on a square lattice. I also investigate the out-of-equilibrium scenarios of such models via simulated temperature quenches. Finally, I investigate how restoring energy extensivity in long-range interacting systems can have a profound incidence on the low-energy properties in the thermodynamic limit.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.
This thesis is devoted to the study of dipolar lattice gases, i.e. many-body quantum systems of particles with a strong magnetic or electric dipole moment in optical lattices. Such systems are adequately described by the extended Hubbard model, which accounts for inter-site dipole-dipole interactions (DDI). These interactions, due to their long-range and anisotropic character, result in rich groundstate physics and intriguing dynamics as we illustrate in this thesis for the particular case of bosons in one- and quasi-one-dimensional lattices. We start by focusing on the non-trivial role played by the transversal confinement in one-dimensional dipolar lattice gases. We show that weakening the transversal confinement enhances beyond-nearest-neighbor interactions. Then, we analyze how this affects the ground-state physics of hard-core bosons with repulsive dipolar interactions and reveal quantitative differences to the standard case of the DDI falling off as 1/r^3 where r is the inter-particle distance. With attractive interactions, a new quantum liquid phase of self-bound lattice droplets emerges without the need for super-exchange processes. In the soft-core regime, proper consideration of the transversal confinement not only quantitatively shifts phase boundaries, but introduces novel phases with peculiar correlations in the site occupancies that may be either topological or topologically trivial. Furthermore, we study the effect of the transversal confinement on the dynamical properties of one-dimensional hard-core bosons at half-filling. We show in particular that the localization-to-delocalization transition induced by Hilbert space fragmentation resembles that of a system with an effective power-law decay different from 1/r^3 which can be controlled by the transversal confinement. To conclude this thesis, we analyze ground-state properties of hard-core dipolar bosons in a square ladder at unit rung filling with an energy bias between the two legs. We show that the interplay between the energy bias and the dipolar tail results in a peculiar topological quantum floating phase.