Bulletin of the American Physical Society

Cold ion-neutral chemistry: Measurement of charge-exchange reaction rates in the $\textrm{Na} + \textrm{Ca}^+$ system using a hybrid atom- ion trap

Jonathan M. Kwolek, Douglas S. Goodman, Benjamin Slayton, R. Blümel, James E. Wells, Frank A. Narducci, W. W. Smith

Published May 31, 2019• 0 citations

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Bulletin of the American Physical Society

Cold ion-neutral chemistry: Measurement of charge-exchange reaction rates in the $\textrm{Na} + \textrm{Ca}^+$ system using a hybrid atom- ion trapCold ion-neutral chemistry: Measurement of charge-exchange reaction rates in the $\textrm{Na} + \textrm{Ca}^+$ system using a hybrid atom- ion trap

Jonathan M. Kwolek, Douglas S. Goodman, Benjamin Slayton, R. Blümel, James E. Wells, Frank A. Narducci, W. W. Smith

Published May 31, 2019• 0 citations

OpenAlex

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Measurements of charge-exchange reaction rate constants between $\textrm{Ca}^+$ and Na in a hybrid atom-ion trapMeasurements of charge-exchange reaction rate constants between $\textrm{Ca}^+$ and Na in a hybrid atom-ion trap

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We present measurements of the charge-exchange reaction rate between neutral sodium (Na) and ionized calcium ( ${\mathrm{Ca}}^{+}$ ) in a hybrid atom-ion trap, which is comprised of a Na magneto-optical trap concentric with a linear Paul trap. Once the Na and ${\mathrm{Ca}}^{+}$ are co-trapped, the reaction rate is measured by continuously quenching the reaction product ${\mathrm{Na}}^{+}$ from the ion trap, and then destructively measuring the decay of the remaining ion population. The reactants' electronic state and temperature are experimentally controlled, allowing us to determine the four individual reaction rates between $\text{Na}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}P]$ and ${\text{Ca}}^{+}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}D]$ at different collision energies. With the exception of the largest reaction-rate channel ( $\text{Na}[P]+{\text{Ca}}^{+}[D]$ ), our rates are consistent with the classical Langevin rate limit. We have also found evidence of reactant collision-energy thresholds associated with two of the four entrance channels.We present measurements of the charge-exchange reaction rate between neutral sodium (Na) and ionized calcium (${\mathrm{Ca}}^{+}$) in a hybrid atom-ion trap, which is comprised of a Na magneto-optical trap concentric with a linear Paul trap. Once the Na and ${\mathrm{Ca}}^{+}$ are co-trapped, the reaction rate is measured by continuously quenching the reaction product ${\mathrm{Na}}^{+}$ from the ion trap, and then destructively measuring the decay of the remaining ion population. The reactants' electronic state and temperature are experimentally controlled, allowing us to determine the four individual reaction rates between $\text{Na}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}P]$ and ${\text{Ca}}^{+}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}D]$ at different collision energies. With the exception of the largest reaction-rate channel ($\text{Na}[P]+{\text{Ca}}^{+}[D]$), our rates are consistent with the classical Langevin rate limit. We have also found evidence of reactant collision-energy thresholds associated with two of the four entrance channels.

arXiv:1812.02810Physical Review AMay 24, 20198 citations

Cold ion-neutral chemistry: Measurement of charge-exchange reaction rates in the

\textrm{Na} + \textrm{Ca}^+

system using a hybrid atom- ion trap

Measurements of charge-exchange reaction rate constants between

\textrm{Ca}^+

and Na in a hybrid atom-ion trap

Light assisted charge exchange interaction between potassium (K) atoms and calcium ions (Ca

^{\mathrm{+}})

ions in an ion-atom hybrid trap

We present measurements of the charge-exchange reaction rate between neutral sodium (Na) and ionized calcium (

{\mathrm{Ca}}^{+}

) in a hybrid atom-ion trap, which is comprised of a Na magneto-optical trap concentric with a linear Paul trap. Once the Na and

{\mathrm{Ca}}^{+}

are co-trapped, the reaction rate is measured by continuously quenching the reaction product

{\mathrm{Na}}^{+}

from the ion trap, and then destructively measuring the decay of the remaining ion population. The reactants' electronic state and temperature are experimentally controlled, allowing us to determine the four individual reaction rates between

\text{Na}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}P]

and

{\text{Ca}}^{+}[S\phantom{\rule{4.pt}{0ex}}\text{or}\phantom{\rule{4.pt}{0ex}}D]

at different collision energies. With the exception of the largest reaction-rate channel (

\text{Na}[P]+{\text{Ca}}^{+}[D]

), our rates are consistent with the classical Langevin rate limit. We have also found evidence of reactant collision-energy thresholds associated with two of the four entrance channels.