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Optica

Experimental observation of the geometric phase in nonlinear frequency conversion

Aviv Karnieli, Sivan Trajtenberg‐Mills, Giuseppe Di Domenico, Ady Arie

Published Oct 29, 2019• 37 citations
Publisher

Abstract

The geometric phase is a common phenomenon in a variety of physical systems, with significant applications in optics. We report the first experimental demonstration of the adiabatic geometric phase in nonlinear frequency conversion, wherein the coupling between the signal and idler frequencies constitutes the intrinsic two-level dynamics of the system. We observe a variety of effects associated with the geometric phase, including the adiabatic broadening of bandwidth, asymmetric transmission for opposite propagation directions, conjugation of the phase for orthogonal eigenstates, and the nonreciprocity associated with the pump field bias. Our work paves the way towards all-optically controlled geometric phase elements for wavefront shaping, isolation, guiding, and quantum optical applications, harnessing spectral and spatial correlations.

DOI
10.1364/optica.6.001401

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The geometric phase is a common phenomenon in a variety of physical systems, with significant applications in optics. We report the first experimental demonstration of the adiabatic geometric phase in nonlinear frequency conversion, wherein the coupling between the signal and idler frequencies constitutes the intrinsic two-level dynamics of the system. We observe a variety of effects associated with the geometric phase, including the adiabatic broadening of bandwidth, asymmetric transmission for opposite propagation directions, conjugation of the phase for orthogonal eigenstates, and the nonreciprocity associated with the pump field bias. Our work paves the way towards all-optically controlled geometric phase elements for wavefront shaping, isolation, guiding, and quantum optical applications, harnessing spectral and spatial correlations.
nonlinear crystal rotate along a closed path, geometric phase will be generated in the signal and idler waves that participate in the nonlinear frequency conversion. In this paper, we study two rotation schemes, full-wedge rotation and half-wedge rotation, of the QPM parameters in the process of fully nonlinear three-wave mixing. These two schemes can effectively suppress the uncertainty in creating the geometric phase in the nonlinear frequency conversion process when the intensity of the pump is depleted. The finding of this paper provides an avenue toward constant control of the geometric phase in nonlinear optics applications and quantum information processing.
The application of the adiabatic geometric phase (AGP) to nonlinear frequency conversion may help to develop new types of all-optical devices, which leads to all-optical modulation of the phase front of one wave by the intensity of other waves. In this paper, we develop the canonical Hamilton equation and a corresponding geometric representation for two schemes of four-wave mixing (FWM) processes (ω1 + ω2 = ω3 + ω4 and ω1 + ω2 + ω3 = ω4), which can precisely describe and calculate the AGP controlled by the quasi-phase matching technique. The AGPs of the idler (ω1) and signal (ω4) waves for these two schemes of FWM are studied systematically when the two pump waves (ω2 and ω3) are in either the undepleted or in the depleted pump cases, respectively. The analysis reveals that the proposed methods for calculating the AGP are universal in both cases. We expect that the analysis of AGP in FWM processes can be applied to all-optically shaping or encoding of ultrafast light pulse.
Adiabatic evolution, an important dynamical process in a variety of classical and quantum systems providing a robust way of steering a system into a desired state 1-5, was introduced only recently to frequency conversion 6-9. Adiabatic frequency conversion allowed the achievement of efficient scalable broadband frequency conversion 8, 9 and was applied successfully to the conversion of ultrashort pulses, demonstrating near-100% efficiency for ultrabroadband spectrum 10-16. The underlying analogy between undepleted pump nonlinear processes and coherently excited quantum systems was extended in the past few years to multi-level quantum systems, demonstrating new concepts in frequency conversion, such as complete frequency conversion through an absorption band 17-20. Additionally, the undepleted pump restriction was removed, enabling the exploration of adiabatic processes in the fully nonlinear dynamics regime of nonlinear optics 21-26. In this article, the basic concept of adiabatic frequency conversion is introduced, and recent advances in ultrashort physics, multi-process systems, and the fully nonlinear dynamics regime are reviewed.
Quantum eigenstates undergoing cyclic changes acquire a phase factor of geometric origin. This phase, known as the Berry phase, or the geometric phase, has found applications in a wide range of disciplines throughout physics, including atomic and molecular physics, condensed matter physics, optics, and classical dynamics. In this article, the basic theory of the geometric phase is presented along with a number of representative applications. The article begins with an account of the geometric phase for cyclic adiabatic evolutions. An elementary derivation is given along with a worked example for two-state systems. The implications of time-reversal are explained, as is the fundamental connection between the geometric phase and energy level degeneracies. We also discuss methods of experimental observation. A brief account is given of geometric magnetism; this is a Lorenz-like force of geometric origin which appears in the dynamics of slow systems coupled to fast ones. A number of theoretical developments of the geometric phase are presented. These include an informal discussion of fibre bundles, and generalizations of the geometric phase to degenerate eigenstates (the nonabelian case) and to nonadiabatic evolution. There follows an account of applications. Manifestations in classical physics include the Hannay angle and kinematic geometric phases. Applications in optics concern polarization dynamics, including the theory and observation of Pancharatnam's phase. Applications in molecular physics include the molecular Aharonov-Bohm effect and nuclear magnetic resonance studies. In condensed matter physics, we discuss the role of the geometric phase in the theory of the quantum Hall effect.
A comprehensive study of two simultaneous three wave mixing processes, a second harmonic generation followed by difference frequency generation, under nonlinear stimulated Raman adiabatic passage (STIRAP) is presented. An input pump is up-converted to its second harmonic, which then gets down-converted to a signal and idler pair with frequencies lying very close to the input pump in such a manner that complete conversion from the pump to the signal and idler takes place without exciting the second harmonic under counterintuitive adiabatic passage. This process involves nonlinear STIRAP with a nonlinear dark state similar to atomic population transfers, and we bring an analogy from atomic systems to our nonlinear dynamics to linearize the problem and analytically obtain the adiabaticity condition required for complete conversion. We also show that the nonlinear STIRAP mechanism results in a large bandwidth of about 380 nm with almost complete conversion of the pump to the signal and idler.
The geometrical Berry phase is key to understanding the behaviour of quantum states under cyclic adiabatic evolution. When generalised to non-Hermitian systems with gain and loss, the Berry phase can become complex, and should modify not only the phase but also the amplitude of the state. Here, we perform the first experimental measurements of the adiabatic non-Hermitian Berry phase, exploring a minimal two-site PT\mathcal{PT}PT-symmetric Hamiltonian that is inspired by the Hatano-Nelson model. We realise this non-Hermitian model experimentally by mapping its dynamics to that of a pair of classical oscillators coupled by real-time measurement-based feedback. As we verify experimentally, the adiabatic non-Hermitian Berry phase is a purely geometrical effect that leads to significant amplification and damping of the amplitude also for non-cyclical paths within the parameter space even when all eigenenergies are real. We further observe a non-Hermitian analog of the Aharonov--Bohm solenoid effect, observing amplification and attenuation when encircling a region of broken PT\mathcal{PT}PT symmetry that serves as a source of imaginary flux. This experiment demonstrates the importance of geometrical effects that are unique to non-Hermitian systems and paves the way towards the further studies of non-Hermitian and topological physics in synthetic metamaterials.