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Springer theses

Two-Photon Rydberg Excitation

Gerard T. Higgins

Published Jan 1, 2019• 1 citation
Publisher
DOI
10.1007/978-3-030-33770-4_4

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Two-photon bound states in Rydberg gases

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We propose a scheme for a deterministic controlled-phase gate between two photons that is based on the strong interaction between two stationary collective Rydberg excitations in an atomic ensemble outside the regime of Rydberg blockade. The distance-dependent character of the interaction causes both a momentum displacement of the collective excitations and unwanted entanglement between them. We show that these effects can be overcome by swapping the collective excitations in space and by optimizing the geometry, resulting in a photon-photon gate with high fidelity and efficiency.
Mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons enables the realization of optical nonlinearities which can modify light on the level of individual photons.This novel approach forms the basis of a growing Rydberg quantum optics toolbox, which already contains photonic logic building-blocks such as single-photon sources, switches, transistors, and conditional π-phase shifts.This thesis reports on two experiments investigating strong photon-photon interactions mediated by Rydberg interactions.First, applying a ladder-type EIT scheme to Rydberg atoms in D-states with high principal quantum number results in the Rydberg interaction mediated nonlinearity accompanied by a time-dependent decay of transmission of probe light through the medium.In a joint experimental and theoretical analysis, this effect is attributed to the dephasing of propagating polaritons into stationary Rydberg excitations caused by the state mixing interaction occurring with Rydberg D-state atoms.Second, via a two-photon Raman excitation scheme Rydberg atoms are efficiently excited in a small atomic cloud.As the size of the Rydberg blockade exceeds the dimension of the medium, only a single Rydberg excitation can be present at a time.By fast engineered dephasing this Rydberg excitation is decoupled from the light field.Measurement of the transmitted light and the amount of excited Rydberg atoms gives evidence for the realization of a deterministic single-photon absorber.