Over the last few decades, quantum cryptography has been one of the most important quantum technologies developed. It holds the promise of communicating secure information over untrusted channels. In particular, quantum cryptography is immune to the eventual threats posed by large-scale quantum computers, which is not the case for our current classical cryptography infrastructures. In a world where information, communication and privacy are of paramount importance, the development of secure quantum communication infrastructures becomes imperative. So far, most of the quantum cryptographic systems developed to date are based on two-dimensional encoding schemes, analogous to classical bits, known as qubits. Nevertheless, other than for the polarization of light, photonic degrees of freedom, i.e. position, momentum, time and frequency, naturally occur as high-dimensional quantum systems. Moreover, by considering high-dimensional encoding schemes beyond qubits, advantages in terms of information capacity and noise tolerance are predicted in theory. In this thesis, the basic components of a high-dimensional quantum cryptographic system are investigated. We begin by reviewing important developments in quantum cryptography and high-dimensional quantum information. As a starting point, two different quantum information tasks, i.e. optimal quantum cloning and quantum metrology, are experimentally investigated for high-dimensional quantum systems in order to demonstrate the numerous advantages of performing quantum tasks beyond qubits. The photonic degree of freedom used in these experiments, known as transverse spatial modes, is obtained by combining the position and momentum photonics degrees of freedom. Thus, we develop a novel method to measure high-dimensional quantum states encoded in arbitrary spatial modes. Using a similar characterization technique, several high-dimensional quantum communication channels are characterized to perform high-dimensional quantum cryptography. The tools developed in the laboratory are then brought to realistic conditions in order to test the feasibility of high-dimensional quantum cryptography. Two different types of quantum channels are experimentally investigated, namely an intra-city 300 m long free-space link and a short 3 m outdoor underwater link. Finally, we investigate and compare novel high-dimensional protocols to overcome current limitations.
Over the last few decades, quantum cryptography has been one of the most important quantum technologies developed. It holds the promise of communicating secure information over untrusted channels. In particular, quantum cryptography is immune to the eventual threats posed by large-scale quantum computers, which is not the case for our current classical cryptography infrastructures. In a world where information, communication and privacy are of paramount importance, the development of secure quantum communication infrastructures becomes imperative. So far, most of the quantum cryptographic systems developed to date are based on two-dimensional encoding schemes, analogous to classical bits, known as qubits. Nevertheless, other than for the polarization of light, photonic degrees of freedom, i.e. position, momentum, time and frequency, naturally occur as high-dimensional quantum systems. Moreover, by considering high-dimensional encoding schemes beyond qubits, advantages in terms of information capacity and noise tolerance are predicted in theory. In this thesis, the basic components of a high-dimensional quantum cryptographic system are investigated. We begin by reviewing important developments in quantum cryptography and high-dimensional quantum information. As a starting point, two different quantum information tasks, i.e. optimal quantum cloning and quantum metrology, are experimentally investigated for high-dimensional quantum systems in order to demonstrate the numerous advantages of performing quantum tasks beyond qubits. The photonic degree of freedom used in these experiments, known as transverse spatial modes, is obtained by combining the position and momentum photonics degrees of freedom. Thus, we develop a novel method to measure high-dimensional quantum states encoded in arbitrary spatial modes. Using a similar characterization technique, several high-dimensional quantum communication channels are characterized to perform high-dimensional quantum cryptography. The tools developed in the laboratory are then brought to realistic conditions in order to test the feasibility of high-dimensional quantum cryptography. Two different types of quantum channels are experimentally investigated, namely an intra-city 300 m long free-space link and a short 3 m outdoor underwater link. Finally, we investigate and compare novel high-dimensional protocols to overcome current limitations.
In this thesis, Quantum Key Distribution and quantum communication methods based on high-dimensional spatial coding of light are developed. Their security is based on the fundamental quantum nature of light and profits from the highdimensional Hilbert spaces offered intrinsically by imaging optics. An overview of classical information theory and quantum information is given to introduce the field of quantum cryptography. The advantages of larger dimensional alphabets and the security of the standard two-bases BB84 protocol is shown. The spatial states used for encoding are introduced. An analytic expression for the upper bound on the mutual information for these states is derived, including multiphoton states, detector noise and beam broadening. High-dimensional encoding of single photons is experimentally realized, reaching 10.5 bit per received photon. The dependence of the mutual information on the number of detector pixels is discussed and the experimental values are compared with the theoretical upper bound. It was shown that a standard error-correcting LDPC code is sufficient to achieve practically error-free communication. By adding a second mutually unbiased basis, a large-alphabet QKD system is experimentally realized and characterized. The security of this BB84-like protocol is analyzed in terms of intercept-resend and collective attacks. The key rate after postprocessing is analyzed under realistic circumstances, including finite key length. Finally, a new quantum communication method is demonstrated, which is based on encoding information into wavefronts decomposed over guided modes of a multimode fiber. At the end a step back is made and the similarities and differences of several quantum authentication and quantum cryptography schemes as well as Quantum Data Locking are discussed. This involves comparison of the characteristics of the classical channel, the quantum channel and the necessary dimension of the Hilbert space.
Light with a complex amplitude structure invokes interesting fundamental properties such as phase and polarization singularities, which also enables novel applications in classical and quantum optical experiments [1]. One feature, namely a twisted phase front and its orbital angular momentum, attracted a lot of attention due its broad range of applications. In the quantum domain, structured photons are highly beneficial since they serve as a physical realizations of high-dimensional states, which allow for example an enlarged information content per single carrier and are known to have a better noise resistance in quantum cryptography applications [2]. At first, I will present a set of laboratory experiments, in which we investigate different quantum cryptographic protocols. Our versatile approach relies on a heralded single photon source, a preparation stage at Alice’s sender, a 1 m-long quantum channel, and a detection stage at Bob’s receiver unit. Because the generation and detection is performed using computer generated, re-programmable holograms displayed on spatial light modulators, the same setup can be used to experimentally survey different quantum key distribution techniques and compare their benefits and deficiencies. The investigated protocols are all based on high-dimensional quantum states and include the seminal protocol of Bennett & Brassard, tomographic protocols, and recently introduced differential phase shift protocols [3,4]. We compare the performance of the different approaches in terms of noise resistance and secret key rates. Our study highlights the benefits of using structured photons and high-dimensional quantum states for different implementations and channel conditions. In a second series of experiments, we get a step closer to real world implementations and investigate long distance and underwater quantum cryptography using high-dimensional quantum information encoded on structured light. We establish an approx. 280m long intra-city quantum link and study the influence of turbulence on achievable key rates [5]. We further test the effect of water turbulences on an underwater quantum channel using twisted photons in an outdoor pool of 3 m length [6]. Although we are able establish a secure channel with three dimensional quantum states, we find mode deformations and vortex splitting due to strong turbulent conditions most probably caused by local variations in temperature. We perform a detailed analysis of the observed turbulence and find that underwater channels may give rise to turbulent conditions that are fundamentally different in terms of temporal and spatial disturbance from those present in a free-space channel. [1] H. Rubinsztein-Dunlop et al. Roadmap on structured light, Journal of Optics 19, 013001 (2017) [2] M. Erhard, R. Fickler, M. Krenn, A. Zeilinger, Twisted Photons: New Quantum Perspectives in High Dimensions, Nature Light: Science & Applications, 7 17146 (2018) [3] F. Bouchard et al. Experimental investigation of quantum key distribution protocols with twisted photons, arXiv:1802.05773 [4] F. Bouchard, A. Sit, K. Heshami, R. Fickler, E. Karimi, Round-Robin Differential Phase-Shift Quantum Key Distribution with Twisted Photons, arXiv:1803.00166 [5] A. Sit et al. High-Dimensional Intra-City Quantum Cryptography with Structured Photons, Optica 4, 1006 (2017) [6] F. Bouchard et al. Underwater Quantum Key Distribution in Outdoor Conditions with Twisted Photons, arXiv:1801.10299
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.
This thesis encompasses a body of experimental work on the use of structured light in quantum cryptographic protocols. In particular, we investigate the ability to perform quantum key distribution through various quantum channels (fibre, free-space, underwater) in laboratory and realistic conditions. We first demonstrate that a special type of optical fibre (vortex fibre) capable of coherently transmitting vector vortex modes is a viable quantum channel. Next, we describe the first demonstration of high-dimensional quantum cryptography using structured photons in an urban setting. In particular, the prevalence of atmospheric turbulence can introduce many errors to a transmitted key; however, we are still able to transmit more information per carrier using a 4-dimensional scheme in comparison to a 2-dimensional one. Lastly, we investigate the possibility of performing secure quantum communication with twisted photons in an uncontrolled underwater channel. We find that though it is possible for low-dimensional schemes, high-dimensional schemes suffer from underwater turbulence without the use of corrective wavefront techniques.
Currently, theoretical and experimental work in the field of quantum cryptography is being carried out in many research centers around the world. Over the past two decades since the start of active research, many quantum cryptographic protocols have been proposed, a significant number of laboratory experiments have been performed on their practical implementation, important work has been done to prove the resistance of the proposed protocols to certain types of attacks, and the first commercial quantum key distribution systems have been developed. However, there are still many tasks and problems in the field of quantum cryptography, the solution of which is of great scientific and technical importance. So, in particular, such a promising direction as quantum protocols for direct secure communication requires further development, allowing, under certain conditions, to transfer secret information without encryption, both between two and between a large number of users. Currently, such protocols have been developed using two-and three-particle entangled states, but there are almost no similar protocols with entangled states of a larger number of qubits that do not require large quantum memory for their implementation and, at the same time, have a large information capacity. Therefore, the development of new quantum direct secure communication protocols with increased information capacity, the analysis of their resistance to attacks, as well as the determination of the best protocols according to the criteria of resistance and information capacity.