The enhanced interaction of quantum states of light and matter within an optical resonator is a powerful tool for both addressing fundamental questions of nature and pursuing quantum technologies. Here, we discuss the impact of cavity birefringence - a lifting of the degeneracy of polarisation modes within the resonator - on both of these challenges. A novel model for such systems is experimentally verified by the cavity emission of single photons with time-dependent polarisation states that evolve along their wavepacket [1]. This model is then used to demonstrate how a tailored birefringence allows for enhanced photon emission beyond previous limitations [2].
The enhanced interaction of quantum states of light and matter within an optical resonator is a powerful tool for both addressing fundamental questions of nature and pursuing quantum technologies. Here, we discuss the impact of cavity birefringence - a lifting of the degeneracy of polarisation modes within the resonator - on both of these challenges. A novel model for such systems is experimentally verified by the cavity emission of single photons with time-dependent polarisation states that evolve along their wavepacket [1]. This model is then used to demonstrate how a tailored birefringence allows for enhanced photon emission beyond previous limitations [2].
We present the effects of resonator birefringence on the cavity-enhanced interfacing of quantum states of light and matter, including the first observation of single photons with a time-dependent polarization state that evolves within their coherence time. A theoretical model is introduced and experimentally verified by the modified polarization of temporally long single photons emitted from a ^{87}Rb atom coupled to a high-finesse optical cavity by a vacuum-stimulated Raman adiabatic passage process. Further theoretical investigation shows how a change in cavity birefringence can both impact the atom-cavity coupling and engender starkly different polarization behavior in the emitted photons. With polarization a key resource for encoding quantum states of light and modern micron-scale cavities particularly prone to birefringence, the consideration of these effects is vital to the faithful realization of efficient and coherent emitter-photon interfaces for distributed quantum networking and communications.
Abstract The generation of entanglement between distant atoms via single photons is the basis for networked quantum computing, a promising route to large-scale trapped-ion and trapped-atom processors. Locating the emitter within an optical cavity provides an efficient matter-light interface, but mirror-induced birefringence within the cavity introduces time-dependence to the polarisation of the photons produced. We show that such ‘polarisation oscillation’ effects can lead to severe loss of fidelity in the context of two-photon, polarisation encoded measurement-based remote entanglement schemes. It is always preferable to suppress these errors at source by minimising mirror ellipticity, but we propose two remedies for systems where this cannot be achieved. We conclude that even modest cavity birefringence can be detrimental to remote entanglement performance, to an extent that may limit the suitability of polarisation-encoded schemes for large-scale quantum networks.
Combining optical cavities with trapped atomic ions is a powerful tool to investigate the interaction of light with matter on the most fundamental scale: a single atom with a single particle of light. Recent advances have not only demonstrated the emission of single photons, ion-photon entanglement and ion-ion entanglement but paved the way to use these systems in modern quantum technologies. Ion-cavity systems are now one of the most promising technologies for realising a scalable quantum computer and quantum networks. While the integration of optical cavities and ion traps is challenging, new techniques and technologies made it possible to demonstrate important building blocks for such systems.
A cavity quantum electrodynamics (cQED) system consisting of a confined single photon and a single quantum emitter serves as a fundamental block for quantum optics and photonic quantum technologies. The canonical optical mode employed in the conventional cavity quantum electrodynamics features a uniform polarization distribution, leading to the scalar light-matter interaction in most existing experiments. Despite the rapid progress in the generation of structured light with spatially varied polarizations, the structured light-matter interaction, especially at the single quanta level, is highly intriguing yet largely unexplored. Here, we present the structured light-matter interaction at the single-photon level in a semiconductor cavity quantum electrodynamics system. Four distinct structured cavity modes that are spectrally close to each other are constructed in a micropillar cavity. By spatially locating a single epitaxial quantum dot (QD) at the periphery of a semiconductor micropillar cavity and spectrally tuning the QD emission wavelength into the resonances of the structured cavity modes, cavity-enhanced single-photon emissions with spin-locked chiral orbital angular momentum (OAM) and engineerable spin-orbit entanglements are achieved within a single wavelength-scale device. Our work opens an unexplored paradigm of structured quantum light-matter interactions and may further advance chiral quantum optics and high-dimensional photonic quantum technology.
The interaction of light with matter is at the heart of quantum optics, which itself enables insight into the fundamental aspects of quantum mechanics. First experimental access to this research field has been realized by coupling atoms to light. Here, the transition between discrete energy states of the atom is associated with the absorption and emission of a photon, a single quantum of the electromagnetic field. As a central aspect of quantum optics, the light-emitter interaction can be significantly enhanced by placing the emitter in optical cavity that is on resonance with the emitter. In recent years, this has led to a rapidly evolving research field known as cavity quantum electrodynamics (CQED). In CQED two different regimes are distinguished: the strong and the weak coupling regimes. In the strong coupling regime, the emitted photon is reflected from the cavity mirrors and eventually reabsorbed by the emitter. In contrast, the weak coupling regime describes the irreversible emission, where the photon leaks out of the cavity before it can be reabsorbed. Both the weak and strong coupling regimes enabled fundamental experiments for a better understanding of quantum optical phenomena. \n \n \n \nCQED grants access to the quantum world and hence offers potentially revolutionizing applications, particularly in the field of quantum information processing. A central aspect for the successful implementation of quantum applications is the system's scalability. Unfortunately, placing atoms deterministically inside a cavity remains technologically elaborate and hence minimizes the prospect of scaling a atom-CQED system. \n \nA possibility to address this issue is to implement CQED in the solid state, where sophisticated fabrication strategies allow miniaturization and scalability of the system. Particularly the development of self-assembled quantum dots (QD) in semiconductors represent a promising route. QDs can be considered as artificial atoms that mimic the atomic two-level system. These structures interact strongly with light and therefore have the potential for replacing atoms in CQED. As a central advantage, QDs are naturally trapped, which greatly simplifies the deterministic incorporation into the cavity. \n \nIn recent years, many efforts have been made to couple self-assembled QDs to microcavities. Generally, the successful implementation of CQED requires a cavity with a high quality factor Q and a low mode volume. In a majority of the approaches, the high Q/small mode volume cavities were monolithically defined around the QD, embedding the QD at a fixed position inside the cavity. Both the weak and strong coupling regimes have been reached with these systems. However, for future applications they suffer from several disadvantages. The fixed position of the QD inside the cavity minimizes the prospects for spectral tunability and spatial positioning the QD inside the cavity. Furthermore, prospects for further increasing of the cavity Q-factor and minimization of the mode volume remain limited in these systems. \n \nIn this thesis the mentioned disadvantages are addressed by developing a fully tunable miniaturized Fabry-Pérot microcavity with low mode volume. The design enables both spatial positioning of the emitter inside the cavity and spectral tunability. Successful coupling of a single QD to the microcavity is demonstrated including the strong coupling regime. Further a new approach to decrease the cavity mode volume is presented, where we demonstrate weak coupling is achieved
For many contemporary physics experiments, the use of microwave and optical resonators has become a powerful tool for enhancement in detection sensitivities, nonlinear interactions, and quantum dynamics. Most often, the term cavity is used to describe such electromagnetic resonators. This term has been taken over from microwave technology, where resonators really look like closed cavities, whereas optical resonators traditionally have an open kind of setup. That difference in geometry is related to the fact that optical resonators are usually very large compared with the optical wavelength, whereas microwave cavities are often not much longer than a wavelength. As discussed in the course of this book, microwave and optical cavities allow one to extend the interaction length between matter and field, to build up the optical power, to impose a well-defined mode structure on the electromagnetic field, to implement extreme nonlinear optics, and to study manifestly quantum mechanical behavior associated with the modified vacuum structure and/or the large field associated with a single photon confined to a small volume [100].