Although the quantum theory of the optical response of individual atoms to coherent light with frequencies close to electronic transitions and the fluid equations for a gas are well known and understood from first principles, they are developed independently of each other and therefore cannot be applied directly to describe many of the quantum collective and transport phenomena that occur in cold atomic gases, especially in what regards their interaction with optical pulses and beams. Few attempts have been made to derive a consistent formalism and theory that are capable to model this type of systems, and those which exist rely on the adaptation of several ad-hoc hypothesis and simplifications, such as space and time dependent density operators. In this paper we provide the theoretical foundations and establish a formalism capable of paving the way for the development of new simulation tools and to explore new problems in nonlinear optics out of equilibrium.
Although the quantum theory of the optical response of individual atoms to coherent light with frequencies close to electronic transitions and the fluid equations for a gas are well known and understood from first principles, they are developed independently of each other and therefore cannot be applied directly to describe many of the quantum collective and transport phenomena that occur in cold atomic gases, especially in what regards their interaction with optical pulses and beams. Few attempts have been made to derive a consistent formalism and theory that are capable to model this type of systems, and those which exist rely on the adaptation of several ad-hoc hypothesis and simplifications, such as space and time dependent density operators. In this paper we provide the theoretical foundations and establish a formalism capable of paving the way for the development of new simulation tools and to explore new problems in nonlinear optics out of equilibrium.
We present the rigorous microscopic quantum theory of the interaction of ultracold Bose and Fermi gases with the electromagnetic field of vacuum and laser photons. The main attention has been paid to the consistent consideration of dynamical dipole-dipole interactions. The theory developed is shown to be consistent with the general principles of the canonical quantization of electromagnetic field in a medium. Starting from the first principles of QED we have derived the general system of Maxwell-Bloch equations for atomic creation and annihilation operators and the propagation equation for the laser field which can be used for the self-consistent analysis of various linear and nonlinear phenomena in atom optics at high densities of the atomic system. All known equations which are used for the description of the behaviour of an ultracold atomic ensemble in a radiation field can be obtained from our general system of equations in a low-density limit.
Starting from the first principles of nonrelativistic QED we have derived the system of Maxwell-Schr\"odinger equations which can be used for theoretical description of atom optical phenomena at high densities of atoms and high intensities of the laser radiation. The role of multiple atomic transitions between ground and excited states in atom optics has been investigated. Nonlinear optical properties of interacting Bose gases are studied and an equation for the refractive index has been derived. We have investigated the role of light-induced and collisional nonlinearities in the diffraction of an ultracold atomic beam from an intense standing laser wave in the Raman-Nath and in the Bragg regimes.
The study of out-of-equilibrium dynamics in ultra-cold gases is a new and exciting field, driven largely by the recent experimental advances in controlling and imaging cold clouds. The experimental and theoretical work thus far has been somewhat exploratory and largely numerical in nature, as the very paradigms for thinking about these systems are not well established. In this thesis I consider several different scenarios of ultra-cold bosonic and fermionic gases driven out of equilibrium and study their properties. In Chapter 1, I provide an overview of the phenomenology of ultra-cold gases, highlighting the timescales governing these systems and how the experimentalist can tune them. I discuss how cold gases can be cooled and trapped and discuss the basic physics behind optical lattices. I also discuss experimental probes of these gases, in particular the new high resolution imaging techniques developed recently at Chicago, Munich and Harvard. In Chapter 2, I discuss an early experiment (circa. 2008) which observed long lived spin dynamics in a thermal spin-1/2 Fermi gas. This experiment is an nice illustration of interesting physics resulting from the separation of timescales between spin and collisional dynamics. In my opinion, it is an excellent example of why cold gases are naturally suited to studying non-equilibrium dynamics. I simulate the experiment numerically using a collisionless Boltzmann equation and explain the observed spin dynamics both qualitatively and quantitively. In Chapter 3, I continue the discussion of spin waves in thermal gases by extending previous works on spin-1/2 gases to spin-1 Bose gases. In contrast to Chapter 2, the bulk of the work in this Chapter is analytic in nature. In particular, I find a spin wave instability in the thermal spin-1 Bose gas, which is the high temperature analog of the polar to ferromagnetic transition in a spin-1 Bose Einstein condensate. In Chapter 3, I turn my attention to bosonic systems and briefly review the the Bogoliubov mean-field theory. I calculate the momentum distribution and density-density correlation function of an interacting Bose gas within the Bogoliubov framework. Then I consider bosons in an optical lattice, and introduce the Bose Hubbard model. I calculate the mean-field phase diagram of the Bose Hubbard model and then consider fluctuations about the mean field, and derive the excitation spectrum of the lattice gas in the superfluid and insulating regimes. In Chapter 4, I ask what we learn by studying the dynamics of correlation functions following a sudden change in the interactions in a superfluid. Using the Bogoliubov theory developed in Chapter 3, I will show how the underlying excitation spectrum influences the long and short time behavior of the correlation functions. By considering a lattice dispersion, I study the analogous problem in a weak optical lattice and discuss how the lattice dispersion leads to additional features in the correlation functions. I will also discuss the timescale governing the revival of the condensate fraction in a quantum depleted gas. In Chapter 5, I derive equations of motion governing the dynamics of one and two body correlation functions in the single-band Bose Hubbard model, applicable to bosons in deep lattices. I then consider a simple quench from a Mott insulating initial state to a weakly interacting final state and produce analytic expressions describing the dynamics of correlations following such a quench. I discuss the timescale for the development of long range order following such a quench. I study the problem of chapter 4 using an equations of motion approach. This approach complements the Bogoliubov approach of Chapter 4. First, I derive exact expressions for a quench to a non-interacting state. I then consider how interactions redistribute quasi-momentum to first order in perturbation theory in different dimensions. In Chapter 6, I calculate the relevant timescales for local and global dynamics in trapped lattice Bose gases, a work done in collaboration with Dr. Kaden R. A Hazzard. Using a time-dependent Gutzwiller mean-field theory, I show that the timescale for local equilibration in these systems is fast in experimental terms. I then show that due to the spatial inhomogeneities inherent to cold gases, achieving global equilibrium can be quite complicated, sometimes taking longer than the lifetime of the experiment, an issue of practical importance to current day experiments. I continue this discussion in Chapter 7 which is a collaborative work with experimentalists David McKay and Prof. Brian DeMarco from the University of Toronto and the University of Illinois, Urbana Champaign. Using experimental and numerical methods, we show that the rapid timescales for local dynamics in interacting systems invalidates a frequently used cold atom technique for mapping out the momentum distribution of atoms in an optical lattice.
Motivated by rapid experimental progress in the fields of ultracold atoms and quantum optics, I present a series of theoretical studies which explore collective phenomena in quantum gases of atoms and photons. In Chapter 1, I highlight the major developments in the research field and identify the overarching themes and motivations. I also provide a roadmap for the rest of the thesis and summarize the main results. The remaining eight chapters contain original studies, organized along three broad motifs. In Chapters 2 through 5, I investigate how the nature of collective excitations and quasiparticles can be explored in modern experiments. More specifically, I model the dynamics of a spin impurity in a Bose lattice gas, develop a protocol for observing fractionalized excitations or anyons in an optical cavity, and characterize the collective dynamics of Bogoliubov quasiparticles and domain walls in a Fermi superfluid. In Chapters 6 and 7, I examine unconventional superfluid phases in spin-imbalanced Fermi gases. In particular, I propose a novel technique for engineering the long-sought-after Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase and study the relative stability of exotic phases across a dimensional crossover. Finally, Chapters 8 and 9 are devoted to studies of kinetics in out-of-equilibrium systems. I model the formation of a Bose-Einstein condensate in a dimple trap and characterize the approach to thermal equilibrium in quasi-one-dimensional geometries.
In the field of ultracold quantum gases atom optics has been established as a completely
new discipline in the last years. This led to fundmentally new results in the field of research
of atom optical systems. In modern experiments especially strongly interacting
nonlinear systems are of great interest. Such a strongly correlated system consists of a
cold atomic quantum gas and a light field both embedded into a nonlinear medium.
This thesis documents for the first time that a two-dimensional photonic crystal fiber
can be used as a novel nonlinear medium for atom optical experiments. It shows that
cold atoms can be guided optically through this fiber with high efficiency and density.
In order to study this system a new experiment for creating cold optically guided atoms
has been built up. This complex experimental setup consists of high-stable laser sources,
optics and electronics for generating, manipulating and detecting cold atomic rubidium
ensembles as well as further elements for implementing photonic band gap fibers as
matter wave guides. One focal point of the thesis has been the detailed investigation
of the atomic flux through the fiber. This analysis demonstrates that the experimental
parameters governing the atomic flux are in a good agreement with a self-developed
numerical model as well as with other theoretical predictions.
For applying this system as injector for other quantum gas experiments or for atom
interferometry, a continuous, coherent atomic flux is necessary.
Studies demonstrate that such a regime can be reached by using an additional dipole
trap in front of the fiber. By properly chosen trap parameters this trap can be used
as a reservoir of cold atoms. With this optical setup the atomic flux can be kept up
significantly longer than in a pulsed guiding system.
Further the experimental possibilities of this nearly one-dimensional, cold, dense and
tightly embedded atomic system are of great interest. The analysis shows that because
of the generated atomic density and the energetic distribution of the atoms in the
fiber potential a coherent atom optics is feasible with this system. So this experiment
paves the way towards a novel, coherent matter wave guide. By exploiting the strongly
photonic interaction in the fiber other physical regimes especially in the field of nonlinear
optics can be reached. This includes for example the studies of four-wave-mixing
processes in the photonic band gap fiber. In a recent theoretical paper it has been
suggested to use the tunability of the atom-light-interaction to reach a photonic regime
of extremely strong repulsion. This possibly leads to decelerated or even stopped light
forming a so-called Tonks-Girardeau gas.
The experimental realization of correlated quantum phases with ultracold gases in optical lattices and their theoretical understanding has witnessed remarkable progress during the last decade. In this review we introduce basic concepts and tools to describe the many-body physics of quantum gases in optical lattices. This includes the derivation of effective lattice Hamiltonians from first principles and an overview of the emerging quantum phases. Additionally, state-of-the-art numerical tools to quantitatively treat bosons or fermions on different lattices are introduced.