Spin Noise and Spin Relaxation in Spin Squeezed Alkali-Metal Vapors

Spin noise sets fundamental limits to the precision of measurements using spin-polarized atomic vapors, such as performed with sensitive atomic magnetometers. Spin squeezing offers the possibility to extend the measurement precision beyond the standard quantum limit of uncorrelated atoms. Contrary to current understanding, we show that, even in the presence of spin relaxation, spin squeezing can lead to a significant reduction of spin noise, and hence an increase in magnetometric sensitivity, for a long measurement time. This is the case when correlated spin relaxation due to binary alkali-atom collisions dominates independently acting decoherence processes, a situation realized in thermal high atom-density magnetometers and clocks.Spin noise sets fundamental limits to the precision of measurements using spin-polarized atomic vapors, such as performed with sensitive atomic magnetometers. Spin squeezing offers the possibility to extend the measurement precision beyond the standard quantum limit of uncorrelated atoms. Contrary to current understanding, we show that, even in the presence of spin relaxation, spin squeezing can lead to a significant reduction of spin noise, and hence an increase in magnetometric sensitivity, for a long measurement time. This is the case when correlated spin relaxation due to binary alkali-atom collisions dominates independently acting decoherence processes, a situation realized in thermal high atom-density magnetometers and clocks.

arXiv:0708.0330Physical Review LettersFeb 19, 200830 citations

Quantum sensitivity limits and dynamical correlations in alkali-vapor sensors

K. Mouloudakis, V. Koutrouli, I.K. Kominis +2 more

For spin-polarized ensembles of alkali-metal atoms with hyperfine structure and spin greater than 1/2, the interplay between spin dynamics and quantum noise mechanisms remains largely unexplored, especially in the spin-exchange-relaxation-free (SERF) regime. In particular, the theoretical understanding of the dynamics for the mean values of the spin operators was established shortly after the advent of optical pumping. In contrast, a corresponding theory for spin fluctuations has not yet been developed, and is addressed in this work. Here, we develop such a first-principles theory of spin fluctuations in alkalimetal vapors. The nonlinearity bottleneck of spin-exchange collisions, which dominate the physics of such vapors, is overcome by linearizing the dynamics around the equilibrium density matrix. The result is a precise calculation of the absolute magnetic sensing limit of optically pumped atomic magnetometers, which can precisely benchmark quantum limited and quantum enhanced protocols, in contrast to the traditional approach shown to be adequate only within a factor of 2. Further, we elucidate how signal and noise in atomic magnetometers are distributed among the spin eigenmodes defined under continuous optical pumping and probing via the paramagnetic Faraday rotation. Notably, in the SERF regime, alongside the magnetic resonance narrowing, we find a reduction of spin noise at the spin-precession frequency as a consequence of strong hyperfine correlations redistributing spin noise, when both hyperfine manifolds are simultaneously probed. These insights can lead to improved quantum devices utilizing alkali-metal atoms or similar spin-based sensing platforms.For spin-polarized ensembles of alkali-metal atoms with hyperfine structure and spin greater than 1/2, the interplay between spin dynamics and quantum noise mechanisms remains largely unexplored, especially in the spin-exchange-relaxation-free (SERF) regime. In particular, the theoretical understanding of the dynamics for the mean values of the spin operators was established shortly after the advent of optical pumping. In contrast, a corresponding theory for spin fluctuations has not yet been developed, and is addressed in this work. Here, we develop such a first-principles theory of spin fluctuations in alkalimetal vapors. The nonlinearity bottleneck of spin-exchange collisions, which dominate the physics of such vapors, is overcome by linearizing the dynamics around the equilibrium density matrix. The result is a precise calculation of the absolute magnetic sensing limit of optically pumped atomic magnetometers, which can precisely benchmark quantum limited and quantum enhanced protocols, in contrast to the traditional approach shown to be adequate only within a factor of 2. Further, we elucidate how signal and noise in atomic magnetometers are distributed among the spin eigenmodes defined under continuous optical pumping and probing via the paramagnetic Faraday rotation. Notably, in the SERF regime, alongside the magnetic resonance narrowing, we find a reduction of spin noise at the spin-precession frequency as a consequence of strong hyperfine correlations redistributing spin noise, when both hyperfine manifolds are simultaneously probed. These insights can lead to improved quantum devices utilizing alkali-metal atoms or similar spin-based sensing platforms.

Physical Review AppliedDec 11, 20253 citations

Spin-exchange narrowing of the atomic ground-state resonances

Witold Chałupczak, Patrick Josephs-Franks, Brian Patton +1 more

At the most fundamental level, the performance of atomic sensors is limited by quantum decoherence. The problem of decoherence has been addressed at low magnetic fields with atomic samples, where the limiting factor of the coherence lifetime arises from spin-exchange collisions. In this paper, we demonstrate the complex role of the collisions in the relaxation of quantum states of alkali-metal atoms. The detailed understanding of the collision role allows us to reduce the ground-state relaxation in stronger magnetic fields (tens $\ensuremath{\mu}\mathrm{T}$). Reduction of the relaxation rate enables improvement of the performance of atomic sensors. In particular, enhancement of the sensitivity of optical magnetometers in the detection of stronger magnetic fields may be obtained. Reduced transverse relaxation also enables increasing quantum-information storage time in atomic vapor.At the most fundamental level, the performance of atomic sensors is limited by quantum decoherence. The problem of decoherence has been addressed at low magnetic fields with atomic samples, where the limiting factor of the coherence lifetime arises from spin-exchange collisions. In this paper, we demonstrate the complex role of the collisions in the relaxation of quantum states of alkali-metal atoms. The detailed understanding of the collision role allows us to reduce the ground-state relaxation in stronger magnetic fields (tens $\ensuremath{\mu}\mathrm{T}$). Reduction of the relaxation rate enables improvement of the performance of atomic sensors. In particular, enhancement of the sensitivity of optical magnetometers in the detection of stronger magnetic fields may be obtained. Reduced transverse relaxation also enables increasing quantum-information storage time in atomic vapor.

Physical Review AOct 21, 201419 citations

High-Sensitivity Atomic Magnetometer Unaffected by Spin-Exchange Relaxation

J. C. Allred, ROBERT LYMAN, Thomas W. Kornack +1 more

Alkali-metal magnetometers compete with SQUID detectors as the most sensitive magnetic field sensors. Their sensitivity is limited by relaxation due to spin-exchange collisions. We demonstrate a K magnetometer in which spin-exchange relaxation is completely eliminated by operating at high K density and low magnetic field. Direct measurements of the signal-to-noise ratio give a magnetometer sensitivity of $10\text{ }\mathrm{f}\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$, limited by magnetic noise produced by Johnson currents in the magnetic shields. We extend a previous theoretical analysis of spin exchange in low magnetic fields to arbitrary spin polarizations and estimate the shot-noise limit of the magnetometer to be $2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}18}\text{ }\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$.Alkali-metal magnetometers compete with SQUID detectors as the most sensitive magnetic field sensors. Their sensitivity is limited by relaxation due to spin-exchange collisions. We demonstrate a K magnetometer in which spin-exchange relaxation is completely eliminated by operating at high K density and low magnetic field. Direct measurements of the signal-to-noise ratio give a magnetometer sensitivity of $10\text{ }\mathrm{f}\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$, limited by magnetic noise produced by Johnson currents in the magnetic shields. We extend a previous theoretical analysis of spin exchange in low magnetic fields to arbitrary spin polarizations and estimate the shot-noise limit of the magnetometer to be $2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}18}\text{ }\mathrm{T}\text{ }\mathrm{H}{\mathrm{z}}^{\mathrm{\ensuremath{-}}\mathrm{1}\mathrm{/}\mathrm{2}}$.

Physical Review LettersSep 9, 20021,050 citations

Can a Quantum Nondemolition Measurement Improve the Sensitivity of an Atomic Magnetometer?

Marcis P. Auzinsh, Dmitry Budker, Derek F. Jackson Kimball +4 more

We consider the limitations due to noise (e.g., quantum projection noise and photon shot-noise) on the sensitivity of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of $N$ atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as ${N}^{\ensuremath{-}3/4}$; if strongly squeezed probe light is used, the Heisenberg limit of ${N}^{\ensuremath{-}1}$ scaling can be achieved. However, if the measurement time exceeds ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/{N}^{1/2}$ in the former case, or ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/N$ in the latter, where ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}$ is the spin relaxation time, the scaling becomes ${N}^{\ensuremath{-}1/2}$, as for a standard shot-noise-limited magnetometer.We consider the limitations due to noise (e.g., quantum projection noise and photon shot-noise) on the sensitivity of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of $N$ atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as ${N}^{\ensuremath{-}3/4}$; if strongly squeezed probe light is used, the Heisenberg limit of ${N}^{\ensuremath{-}1}$ scaling can be achieved. However, if the measurement time exceeds ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/{N}^{1/2}$ in the former case, or ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/N$ in the latter, where ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}$ is the spin relaxation time, the scaling becomes ${N}^{\ensuremath{-}1/2}$, as for a standard shot-noise-limited magnetometer.

arXiv:physics/0403097Physical Review LettersOct 19, 2004149 citations

Can a quantum nondemolition measurement improve the sensitivity of an atomic magnetometer? - eScholarship

Marcis P. Auzinsh, Dmitry Budker, Derek F. Jackson Kimball +4 more

We consider the limitations due to noise (e.g., quantum projection noise and photon shot-noise) on the sensitivity of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of N atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as N-3/4; if strongly squeezed probe light is used, the Heisenberg limit of N-1 scaling can be achieved. However, if the measurement time exceeds tau(rel)/N-1/2 in the former case, or tau(rel)/N in the latter, where tau(rel) is the spin relaxation time, the scaling becomes N-1/2, as for a standard shot-noise-limited magnetometer.We consider the limitations due to noise (e.g., quantum projection noise and photon shot-noise) on the sensitivity of an idealized atomic magnetometer that utilizes spin squeezing induced by a continuous quantum nondemolition measurement. Such a magnetometer measures spin precession of N atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as N-3/4; if strongly squeezed probe light is used, the Heisenberg limit of N-1 scaling can be achieved. However, if the measurement time exceeds tau(rel)/N-1/2 in the former case, or tau(rel)/N in the latter, where tau(rel) is the spin relaxation time, the scaling becomes N-1/2, as for a standard shot-noise-limited magnetometer.

Oct 1, 20040 citations

N

atomic spins by detecting optical rotation of far-detuned light. We show that for very short measurement times, the optimal sensitivity scales as ${N}^{\ensuremath{-}3/4}$; if strongly squeezed probe light is used, the Heisenberg limit of ${N}^{\ensuremath{-}1}$ scaling can be achieved. However, if the measurement time exceeds ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/{N}^{1/2}$ in the former case, or ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}/N$ in the latter, where ${\ensuremath{\tau}}_{\mathrm{r}\mathrm{e}\mathrm{l}}$ is the spin relaxation time, the scaling becomes ${N}^{\ensuremath{-}1/2}$, as for a standard shot-noise-limited magnetometer.