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Scientific Reports

Velocity-dependent optical forces and Maxwell’s demon

J. D. Franson

Published Sep 24, 2019• 2 citations
Publisher

Abstract

An atom placed in a focused laser beam will experience a dipole force due to the gradient in the interaction energy, which is analogous to the well-known optical tweezers effect. This force will be dependent on the velocity of the atom due to the Doppler effect, which could potentially be used to implement a Maxwell's demon. Photon scattering and other forms of dissipation can be negligibly small, which would seem to contradict quantum information proofs that a Maxwell's demon must dissipate a minimum amount of energy. We show that the velocity dependence of the dipole force is cancelled out by another force that is related to the gradient in the phase of the laser beam. As a result, a Maxwell's demon cannot be implemented in this way.

DOI
10.1038/s41598-019-50284-z

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An atom placed in a focused laser beam will experience a dipole force due to the gradient in the interaction energy, which is analogous to the well-known optical tweezers effect. This force will be dependent on the velocity of the atom due to the Doppler effect, which could potentially be used to implement a Maxwell's demon. Photon scattering and other forms of dissipation can be negligibly small, which would seem to contradict quantum information proofs that a Maxwell's demon must dissipate a minimum amount of energy. We show that the velocity dependence of the dipole force is cancelled out by another force that is related to the gradient in the phase of the laser beam. As a result, a Maxwell's demon cannot be implemented in this way.
An atom moving in a focused laser beam will experience a velocity-dependent dipole force due to the Doppler effect, which allows the operation of a Maxwell's demon. Photon scattering and other forms of dissipation can be negligibly small, which appears to contradict quantum information proofs that a Maxwell's demon must dissipate a minimum amount of energy. We resolve this 'paradox' by showing that Schrodinger's equation does not predict a velocity-dependent dipole force. Forces of that kind have been observed experimentally, however, and we show that Heisenberg's equation does predict a velocity-dependent dipole force in agreement with experiment, provided that the total time derivative of an operator is evaluated along the trajectory of an atom.
We propose an optical Maxwell demon which efficiently captures, concentrates, and damps the kinetic motion of sodium atoms in a gas cell. A bath of radiation tuned just below resonance can prove to be a very viscous medium for atoms. We propose to use this effect to produce and concentrate very slow atoms in a vapor cell. Our bath of radiation consists of three orthogonally intersecting pairs of counterpropagating laser beams. Each beam is tuned about half of the natural linewidth below the resonance transition frequency. (Because of the hyperfine splitting of the Na ground state, two separate frequencies are used.) Atoms which enter the intersection region with velocities less than ~15 m/s (for 1-cm diam beams) are quickly damped to ~0.5 m/s. Thereafter, the velocity is randomized in a characteristic time of ~10 μs. The atoms will then execute diffusive motion in this photon bath, escaping only after many seconds. Since the effusion time for atoms to enter the intersecting beam demon is much shorter than the diffusion time out of it, the demon acts to collect and concentrate the slow atoms into a cold, dense, central gas superposed on the hot, rarified, background gas.
It is shown that a circular dipole can deflect the focused laser beam that induces it and will experience a corresponding transverse force. Quantitative expressions are derived for Gaussian and angular top hat beams, while the effects vanish in the plane wave limit. The phenomena are analogous to the Magnus effect, pushing a spinning ball onto a curved trajectory. The optical case originates in the coupling of spin and orbital angular momentum of the dipole and the light. In optical tweezers the force causes off-axis displacement of the trapping position of an atom by a spin-dependent amount up to λ/2π, set by the direction of a magnetic field. This suggests direct methods to demonstrate and explore these effects, for instance, to induce spin-dependent motion.
The theory of a method to measure electric-dipole polarizabilities is presented. The method uses two-stage laser ablation to produce a pulsed beam of atoms from a solid target. A pair of slits makes the velocity distribution of the atomic beam nonuniform in a way that is well characterized. The light-force technique uses the polarization forces experienced by an atom in the intense, inhomogeneous electromagnetic field of a standing-wave laser to change the velocity distribution of the atomic beam. The large forces cause measurable Doppler shifts in the resonant frequency of the atoms. These frequency shifts change the amount of absorption of resonant light, yielding information about the change in the velocity distribution of the atoms. The detailed shape of the final absorption distribution is polarizability dependent. In the classical picture of the light force, the standing-wave electric field induces a time-varying dipole moment in each atom. Each atom then experiences a Lorentz force due to coherent interaction of the oscillating dipole moment with the time-varying magnetic field. The quantum-mechanical picture corresponds to the Kapitza-Dirac effect for atoms: an atom absorbs a photon from one of the two beams which form the standing wave, and is then stimulated to emit this photon by the other, counterpropagating beam. This paper provides a classical treatment of the light force experienced by an atom in a standing-wave light field; the polarizability is treated quantum mechanically. The theory presented here can be applied to atoms with a scalar polarizability, such as rubidium, and to atoms with significant tensor components, such as uranium. Experimental results from application of the light-force technique to a measurement of the polarizability of rubidium are also presented.
We present a simple review of the basic physical processes allowing one to control, with laser beams, the velocity and the position of neutral atoms. The control of the velocity corresponds to a cooling of atoms, that is, a reduction of the atomic velocity spread around a given value. The control of the position means a trapping of atoms in real space. The best present performances will be given, in terms of the lowest temperatures and the highest densities. The corresponding highest quantum degeneracy will also be estimated. It is imposed by fundamental limits, which will be described briefly. We also give the general trends in this field of research and outline the new directions which look promising for observing quantum statistical effects in laser cooled atomic samples, but which are for the moment restricted by unsolved problems. Introducing the Simple Schemes The radiative forces acting on atoms in a light field can be split into two parts, a reactive one and a dissipative one. The dissipative force (radiation pressure), which basically involves scattering processes, is velocity dependent. We will see that this dependence leads to the Doppler cooling scheme and to the concept of optical molasses, and we will give the corresponding minimal achievable temperature. The dissipative force can be made position dependent, through a gradient of the magnetic field, so that the atoms are also trapped in the so-called magneto-optical trap.
We implemented an optical one-way potential barrier that allows ultracold 87Rb^{87}\text{R}\text{b}87Rb atoms to transmit through when incident on one side of the barrier but reflect from the other. This asymmetric barrier is a realization of Maxwell's demon, which can be employed to produce phase-space compression and has implications for cooling atoms and molecules not amenable to standard laser-cooling techniques. The barrier comprises two focused Gaussian laser beams that intersect the focus of a far-off-resonant single-beam optical dipole trap that holds the atoms. The main barrier beam presents a state-dependent potential to incident atoms, while the repumping barrier beam optically pumps atoms to a trapped state. We investigated the robustness of the barrier asymmetry to changes in the barrier-beam separation, the initial atomic potential energy, the intensity of the second beam, and the detuning of the first beam. We performed simulations of the atomic dynamics in the presence of the barrier, showing that the initial three-dimensional momentum distribution plays a significant role, and that light-assisted collisions are likely the dominant loss mechanism. We also carefully examined the relationship to Maxwell's demon and explicitly accounted for the apparent decrease in entropy for our particular system.