Abstract The spin polarization and spatial homogeneity of alkali metal atoms are critical characteristics that determine the performance of spin-exchange relaxation-free magnetometers. In buffer gas cells, these characteristics are influenced by optical broadening and alkali atomic motional restriction imposed by the buffer gas. In coated cells, the protective effect of the coating on atomic spins, combined with rapid atomic diffusion, leads to significantly superior spin polarization characteristics compared to those in high-pressure buffer gas cells. However, due to neglecting the influence of atom-coating interactions on atomic motion, the existing spin polarization and spatial distribution models fail to accurately describe the polarization characteristics in coated cells. In this paper, based on the Langevin–Bloch equation, a dynamic model considering interaction effects between alkali metal atoms and the coating as well as between the pump light and the hyperfine levels of alkali metal atoms is proposed to accurately describe the spin polarization and spatial distribution in coated cells. To validate the proposed model, a series of experiments were carried out. The results demonstrate that coated cells can maintain high spin polarization and spatial homogeneity even under conditions of low pump intensity and high temperature, which are in good agreement with the simulations. This work provides a theoretical reference for the design of high-performance and low-power quantum sensors.Abstract The spin polarization and spatial homogeneity of alkali metal atoms are critical characteristics that determine the performance of spin-exchange relaxation-free magnetometers. In buffer gas cells, these characteristics are influenced by optical broadening and alkali atomic motional restriction imposed by the buffer gas. In coated cells, the protective effect of the coating on atomic spins, combined with rapid atomic diffusion, leads to significantly superior spin polarization characteristics compared to those in high-pressure buffer gas cells. However, due to neglecting the influence of atom-coating interactions on atomic motion, the existing spin polarization and spatial distribution models fail to accurately describe the polarization characteristics in coated cells. In this paper, based on the Langevin–Bloch equation, a dynamic model considering interaction effects between alkali metal atoms and the coating as well as between the pump light and the hyperfine levels of alkali metal atoms is proposed to accurately describe the spin polarization and spatial distribution in coated cells. To validate the proposed model, a series of experiments were carried out. The results demonstrate that coated cells can maintain high spin polarization and spatial homogeneity even under conditions of low pump intensity and high temperature, which are in good agreement with the simulations. This work provides a theoretical reference for the design of high-performance and low-power quantum sensors.

Journal of Physics D Applied PhysicsMar 26, 20261 citation

Motion in Three Dimensions

K. Tamvakis

Undergraduate texts in physicsJan 1, 20190 citations

One-dimensional motion

Alexander I. Lvovsky

Undergraduate lecture notes in physicsJan 1, 20180 citations

Dynamical scaling of correlations generated by short- and long-range dissipation

Kushal Seetharam, Alessio Lerose, Rosario Fazio +1 more

We study the spatiotemporal spreading of correlations in an ensemble of spins due to dissipation characterized by short- and long-range spatial profiles. Such emission channels can be synthesized with tunable spatial profiles in lossy cavity QED experiments using a magnetic field gradient and a Raman drive with multiple sidebands. We consider systems initially in an uncorrelated state, and find that correlations widen and contract in a novel pattern intimately related to both the dissipative nature of the dynamical channel and its spatial profile. Additionally, we make a methodological contribution by generalizing nonequilibrium spin-wave theory to the case of dissipative systems and derive equations of motion for any translationally invariant spin chain whose dynamics can be described by a combination of Hamiltonian interactions and dissipative Lindblad channels. Our work aims at extending the study of correlation dynamics to purely dissipative quantum simulators and compare them with the established paradigm of correlations spreading in Hamiltonian systems.We study the spatiotemporal spreading of correlations in an ensemble of spins due to dissipation characterized by short- and long-range spatial profiles. Such emission channels can be synthesized with tunable spatial profiles in lossy cavity QED experiments using a magnetic field gradient and a Raman drive with multiple sidebands. We consider systems initially in an uncorrelated state, and find that correlations widen and contract in a novel pattern intimately related to both the dissipative nature of the dynamical channel and its spatial profile. Additionally, we make a methodological contribution by generalizing nonequilibrium spin-wave theory to the case of dissipative systems and derive equations of motion for any translationally invariant spin chain whose dynamics can be described by a combination of Hamiltonian interactions and dissipative Lindblad channels. Our work aims at extending the study of correlation dynamics to purely dissipative quantum simulators and compare them with the established paradigm of correlations spreading in Hamiltonian systems.

arXiv:2110.09547Physical review. B./Physical review. BMay 23, 202231 citations

Two-dimensional matter-wave interferometer, rotational dynamics, and spin contrast

Ryan Rizaldy, Shrestha Mishra, Anupam Mazumdar

We investigate a two-dimensional matter-wave interferometer where both spatial and rotational dynamics of a nanoparticle are intertwined in closing the one-loop interferometer in the Stern-Gerlach type setup. We consider the spin-contrast of the nitrogen-vacancy (NV) centred nanodiamond in combination with a two-dimensional magnetic field setup to extend the one-dimensional Stern--Gerlach interferometry. We analyse the dynamical motion along with the rigid rotation under the influence of the external magnetic field. Regarding rotation, we incorporate Euler-angle dynamics to analyse the stability of rotational degrees of freedom and their influence on the spin contrast to address the Humpty-Dumpty problem. We show that by imparting external rotation provides the gyroscopic stability to the liberating mode of the NV-spin and hence helps to improve the contrast. Our scheme creates a tiny spatial superposition of size $\sim 0.21~{\rm μm}$ for mass $m=10^{-17}$ kg in less than $t\sim 0.013$ s.We investigate a two-dimensional matter-wave interferometer where both spatial and rotational dynamics of a nanoparticle are intertwined in closing the one-loop interferometer in the Stern-Gerlach type setup. We consider the spin-contrast of the nitrogen-vacancy (NV) centred nanodiamond in combination with a two-dimensional magnetic field setup to extend the one-dimensional Stern--Gerlach interferometry. We analyse the dynamical motion along with the rigid rotation under the influence of the external magnetic field. Regarding rotation, we incorporate Euler-angle dynamics to analyse the stability of rotational degrees of freedom and their influence on the spin contrast to address the Humpty-Dumpty problem. We show that by imparting external rotation provides the gyroscopic stability to the liberating mode of the NV-spin and hence helps to improve the contrast. Our scheme creates a tiny spatial superposition of size $\sim 0.21~{\rm μm}$ for mass $m=10^{-17}$kg in less than $t\sim 0.013$s.

quant-pharXiv:2603.05595Mar 9, 20260 citations

\sim 0.21~{\rm μm}

for mass

m=10^{-17}

kg in less than

t\sim 0.013