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Physica Scripta

Observation and theoretical simulation of N -resonances in Cs D 2 lines

A. Krasteva, P.N. Gosh, S. Gateva, S. Tsvetkov, David G. Sarkisyan, Armen D. Sargsyan, T. A. Vartanyan, S. Cartaleva

Published Sep 18, 2019• 7 citations
Publisher

Abstract

Abstract N -type resonances in Cs D 2 lines are investigated in optical cell for different detuning of the fixed coupling transition frequency. Using two independent DFB lasers makes it possible to observe high contrast and subnatural-width N -resonances without magnetic field shielding of an optical buffer gas cell with sub-centimeter dimensions. According to the detuning of the coupling laser frequency, an N -resonance with frequency higher or lower than this of the coupling transition frequency is registered. In the first case the N -resonance is in absorption, but in the second case, an inverse N -resonance (enhanced transparency) is measured. A theoretical simulation of the line shape, which is based on solution of optical Bloch equations and considers the interaction of both coupling and probe radiations with the atomic system is done. The simulation leads to N -resonance peaks in agreement with the observed peaks for different positions of the coupling frequency. The presented approach is of importance for further study and optimization of the three-photon and magneto-optical resonances, as well as for miniaturization of optical sensors based on spatially restricted hot alkali vapor.

DOI
10.1088/1402-4896/ab4508

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Abstract N -type resonances in Cs D 2 lines are investigated in optical cell for different detuning of the fixed coupling transition frequency. Using two independent DFB lasers makes it possible to observe high contrast and subnatural-width N -resonances without magnetic field shielding of an optical buffer gas cell with sub-centimeter dimensions. According to the detuning of the coupling laser frequency, an N -resonance with frequency higher or lower than this of the coupling transition frequency is registered. In the first case the N -resonance is in absorption, but in the second case, an inverse N -resonance (enhanced transparency) is measured. A theoretical simulation of the line shape, which is based on solution of optical Bloch equations and considers the interaction of both coupling and probe radiations with the atomic system is done. The simulation leads to N -resonance peaks in agreement with the observed peaks for different positions of the coupling frequency. The presented approach is of importance for further study and optimization of the three-photon and magneto-optical resonances, as well as for miniaturization of optical sensors based on spatially restricted hot alkali vapor.
The narrow-band coherent N-type resonance, promising for the development of advanced atomic clocks, can be considered as a type of three-photon resonance, where a two-photon Raman excitation is combined with a resonant optical pumping field. In this communication, we present an experimental study and a theoretical analysis related to three-photon, bi-chromatic excitation of Cs atomic vapor contained in an 8-mm long cell with 20 Torr of neon. If a coupling laser is fixed at a frequency that is lower by several GHz than the position of the absorption profile of the F g = 4 set of transitions, and a probe laser is tuned over the D 2 line (λ = 852 nm), a narrow high-contrast enhanced absorption N-resonance will be observed in the probe light profile, superimposed on the absorption profile of the F g = 4 set of transitions. We present theoretical modeling aimed to clarify the processes behind the efficiency of the N-resonance preparation for different frequency positions of the coupling laser within the D 2 line of Cs.
Coherent spectroscopy of degenerate two-level systems of the Doppler-broadened D2{D}_{2}D2​ cesium line has been performed in vacuum and in buffer gas cells. Subnatural-width (SNW) electromagnetically induced transparency and electromagnetically induced absorption (EIA) resonances have been observed with single-frequency laser excitation for different light polarizations and collision regimes. SNW-EIA resonances with linearly polarized excitation of the Fg=4{F}_{g}=4Fg​=4 level are observed, and they increase their contrast with power density increase and reach a contrast of 20% at $200 \mathrm{mW}{\mathrm{cm}}^{\ensuremath{-}2}.$ A theoretical model has been elaborated, taking into account the Doppler broadening of the transitions, the linewidth of the laser light, and the experimental conditions for observation of the fluorescence. Here the theoretical results are in agreement with those of the experiment. In a buffer gas cell, the SNW resonances in the fluorescence, in degenerate two-level systems are observed for the first time and they are only obtained with circularly polarized light. A theoretical explanation of this result is proposed. At the expense of contrast, in the presence of a buffer gas the coherent resonances are significantly narrower than in a vacuum cell for the same power density. The observation of SNW resonances in buffer gas is significantly less sensitive to the laser frequency drift than in a vacuum cell, which could be advantageous for applications in metrology and in the measurement of weak magnetic fields.
Abstract We review three laser spectroscopy schemes developed recently for observation of high-contrast enhanced-absorption nonlinear resonances in small alkali-vapor cells. In our experiments, optical transitions within the cesium D1 line are involved and a probe beam transmission is analyzed. The first spectroscopy method is based on the configuration with two-frequency counter propagating beams, which are linearly polarized in orthogonal directions. This configuration provides observation of high-contrast natural-linewidth resonances superimposed on broad Doppler profiles when the laser frequency is scanned. These resonances have good prospects for developing a miniature optical frequency reference. The second scheme involves two-frequency counter propagating beams with equal circular polarizations and provides observation of subnatural-linewidth resonances when the Raman frequency detuning is scanned. We use these resonances for stabilizing the microwave frequency of a local oscillator (≈ 4.6 GHz). Frequency stability of around 6 × l0-12 is achieved at 1-s averaging using a 5-mm length cell. This result makes the technique attractive for developing a miniature frequency standard in thr microwave range. The third configuration exploits single-frequency counter-propagating beams with linear orthogonal polarizations. The ultrahigh-contrast subnatural-linewidth resonances can be observed when the longitudinal magnetic field is scanned around zero. The possible application is discussed of these resonances in vector atomic magnetometry.
Electromagnetically induced transparency (EIT) effect in a -system formed by Cs atoms line, enclosed in nanometric-thin cells, is studied both experimentally and theoretically for the first time. The atomic column thickness varies in the range of 50–1500 nm. It is demonstrated that when the coupling laser frequency is in exact resonance with the corresponding atomic transition, the parameters of the EIT resonance (also called dark resonance (DR)) depend weakly on , which allows us to detect DR at nm with the contrast of . The obtained DR parameters are the best as compared with those for Rb and lines and Cs line. The DR contrast and width are studied versus laser frequency detunings, coupling laser power, cell thickness, temperature, and applied external magnetic field. The well-resolved splitting of the DR resonance in a magnetic field for nm can be used for magnetometry with high spatial resolution. The theoretical model describes well the observed results.
Abstract Magneto-optical subnatural-linewidth resonances of electromagnetically-induced absorption (EIA) in an alkali vapour cell have been experimentally studied. The observation configuration includes using two counter-propagating pumps and probe light waves with mutually orthogonal linear polarizations, exciting an open optical transition in the 87 Rb D 1 line in the presence of argon buffer gas. The EIA signals registered in a probe-wave transmission reach an unprecedented contrast of about 135% with respect to the wide ‘Doppler’ absorption pedestal and 29% with respect to the level of background transmission signal. These contrast values correspond to a relatively small resonance full width at half maximum of about 7.2 mG (5.2 kHz). The width of the narrowest EIA resonance observed is about 2.1 mG (1.5 kHz). To our knowledge, such a large relative contrast at the kHz-width is the record result for EIA resonances. In general, the work has experimentally proved that the magneto-optical scheme used has very good prospects for various quantum technologies (quantum sensors of weak magnetic fields, optical switches and other photonic elements).
Abstract High-contrast sub-Doppler resonances observed in alkali-metal atomic vapors in the field of counterpropagating bichromatic laser beams are perspective in quantum metrology for designing a miniature optical frequency standard. Until now, these nonlinear resonances have been investigated only experimentally or using numerical calculations. In our opinion, the development of a simplified theoretical model of the observed resonances, which would provide explicit compact analytic expressions describing the line shape of the resonance, would be extremely important for further evolution of the theory. In this study, we perform such theoretical analysis based on the three-level Λ scheme of the atom. We investigate two regimes, viz., the regime of a low-intensity standing wave with close intensities of counterpropagating beams (I1 ≈ I2) and the regime of a probe wave, in which one of the beams has a noticeably lower intensity than that of the oppositely propagating beam (I2 ≪ I1). The resulting analytic expressions make it possible to determine qualitative differences between these regimes and to separate explicitly the contributions from different nonlinear effects to the light field absorption, including the terms responsible for the formation of a high-contrast sub-Doppler peak. The expressions derived here are in qualitative agreement with experimental data obtained earlier.