We investigate, both experimentally and theoretically, the interpretation of the free-electron wave function using spontaneous emission. We use a transversely wide single-electron wave function to describe the spatial extent of transverse coherence of an electron beam in a standard transmission electron microscope. When the electron beam passes next to a metallic grating, spontaneous Smith-Purcell radiation is emitted. We then examine the effect of the electron wave function transversal size on the emitted radiation. Two interpretations widely used in the literature are considered: (1) radiation by a continuous current density attributed to the quantum probability current, equivalent to the spreading of the electron charge continuously over space; and (2) interpreting the square modulus of the wave function as a probability distribution of finding a point particle at a certain location, wherein the electron charge is always localized in space. We discuss how these two interpretations give contradictory predictions for the radiation pattern in our experiment, comparing the emission from narrow and wide wave functions with respect to the emitted radiation's wavelength. Matching our experiment with a new quantum-electrodynamics derivation, we conclude that the measurements can be explained by the probability distribution approach wherein the electron interacts with the grating as a classical point charge. Our findings clarify the transition between the classical and quantum regimes and shed light on the mechanisms that take part in general light-matter interactions.
We investigate, both experimentally and theoretically, the interpretation of the free-electron wave function using spontaneous emission. We use a transversely wide single-electron wave function to describe the spatial extent of transverse coherence of an electron beam in a standard transmission electron microscope. When the electron beam passes next to a metallic grating, spontaneous Smith-Purcell radiation is emitted. We then examine the effect of the electron wave function transversal size on the emitted radiation. Two interpretations widely used in the literature are considered: (1) radiation by a continuous current density attributed to the quantum probability current, equivalent to the spreading of the electron charge continuously over space; and (2) interpreting the square modulus of the wave function as a probability distribution of finding a point particle at a certain location, wherein the electron charge is always localized in space. We discuss how these two interpretations give contradictory predictions for the radiation pattern in our experiment, comparing the emission from narrow and wide wave functions with respect to the emitted radiation's wavelength. Matching our experiment with a new quantum-electrodynamics derivation, we conclude that the measurements can be explained by the probability distribution approach wherein the electron interacts with the grating as a classical point charge. Our findings clarify the transition between the classical and quantum regimes and shed light on the mechanisms that take part in general light-matter interactions.
Do the prior history and the wave-packet size and form of a free electron have a physical effect in its interaction with light? Here we answer these fundamental questions on the interpretation of the electron quantum wave function by analyzing spontaneous and stimulated emissions of a quantum electron wave packet, interacting with a general, quantized radiation field. For coherent radiation (Glauber state), we confirm that stimulated emission and absorption of photons depends on the preinteraction-history-dependent size, exhibiting spectral cutoff when it exceeds the interacting radiation wavelength. Furthermore, stimulated emission of an optically modulated electron wave packet has a characteristic harmonic emission spectrum beyond the cutoff, which depends on the modulation features. In either case, there is no wave-packet-dependent radiation of the Fock state, and particularly the vacuum state spontaneous emission is wave-packet independent. The classical-to-quantum transition of radiation from the point-particle to the plane-wave limits, and the effects of wave-packet modulation indicate a way of measuring the wave-packet size of a single electron wave function, and suggest an alternative direction for exploring light-matter interaction.
Spontaneous light emission is central to a vast range of physical systems and is a founding pillar for the theory of light–matter interactions. In the presence of complex photonic media, the description of spontaneous light emission usually requires advanced theoretical quantum optics tools such as macroscopic quantum electrodynamics, involving quantized electromagnetic fields. Although rigorous and comprehensive, the complexity of such models can obscure the intuitive understanding of many quantum-optical phenomena. Here, we review a method for calculating spontaneous emission and other quantum-optical processes without making explicit use of quantized electromagnetic fields. Instead, we introduce the concept of transition currents, comprising charges in matter that undergo transitions between initial and final quantum states. We show how predictions that usually demand advanced methods in quantum electrodynamics or quantum optics can be reproduced by feeding these transition currents as sources to the classical Maxwell equations. One then obtains the relevant quantum observables from the resulting classical field amplitudes, without washing out quantum optical effects. We show that this procedure allows for a straightforward description of quantum phenomena, even when going beyond the dipole approximation and single emitters. As illustrative examples, we calculate emission patterns and Purcell-enhanced emission rates in both bound-electron and free-electron systems. For the latter, we derive cathodoluminescence emission and energy-loss probabilities of free electrons interacting with nanostructured samples. In addition, we calculate quantum-beat phenomena in bound-electron systems and wave function-dependent optical coherence in free-electron systems. Remarkably, the transition-current formalism captures more complex phenomena, such as many-body interference effects and super-radiance of both bound- and free-electron systems, second-order processes such as two-photon emission, and quantum recoil corrections to free-electron radiation. We review a variety of light–matter interactions in fields ranging from electron microscopy to nanophotonics and quantum optics, for which the transition-current theoretical formalism facilitates practical simulations and a deeper understanding of novel applications.
Coherent emission of light by free charged particles is believed to be successfully captured by classical electromagnetism in all experimental settings. However, recent advances triggered fundamental questions regarding the role of the particle wave function in these processes. Here, we find that even in seemingly classical experimental regimes, light emission is fundamentally tied to the quantum coherence and correlations of the emitting particle. We use quantum electrodynamics to show how the particle's momentum uncertainty determines the optical coherence of the emitted light. We find that the temporal duration of Cherenkov radiation, envisioned for almost a century as a shock wave of light, is limited by underlying entanglement between the particle and light. Our findings enable new capabilities in electron microscopy for measuring quantum correlations of shaped electrons. Last, we propose new Cherenkov detection schemes, whereby measuring spectral photon autocorrelations can unveil the wave function structure of any charged high-energy particle.
In quantum mechanics, the physical state of an electron is described by a wave function. According to the standard probability interpretation, the wave function of an electron is probability amplitude, and its modulus square gives the probability density of finding the electron in a certain position in space. In this article, we show that this central assumption of quantum mechanics may have an ontological extension. It is argued that microscopic particles such as electrons are indeed particles, but their motion is not continuous but discontinuous and random. On this view, the modulus square of the wave function not only gives the probability density of the particles being found in certain locations, but also gives the probability density of the particles being there. In other words, the wave function in quantum mechanics can be regarded as a representation of the state of random discontinuous motion of particles, and at a deeper level, it may represent the dispositional property of the particles that determines their random discontinuous motion.
When multiple quantum emitters radiate, their emission rate may be enhanced or suppressed due to collective interference in a process known as super- or subradiance. Such processes are well known to occur also in light emission from free electrons, known as coherent cathodoluminescence. Unlike atomic systems, free electrons have an unbounded energy spectrum, and, thus, all their emission mechanisms rely on electron recoil, in addition to the classical properties of the dielectric medium. To date, all experimental and theoretical studies of super- and subradiance from free electrons assumed only classical correlations between particles. However, dependence on quantum correlations, such as entanglement between free electrons, has not been studied. Recent advances in coherent shaping of free-electron wave functions motivate the investigation of such quantum regimes of super- and subradiance. In this Letter, we show how a pair of coincident path-entangled electrons can demonstrate either super- or subradiant light emission, depending on the two-particle wave function. By choosing different free-electron Bell states, the spectrum and emission pattern of the light can be reshaped, in a manner that cannot be accounted for by a classical mixed state. We show these results for light emission in any optical medium and discuss their generalization to many-body quantum states. Our findings suggest that light emission can be sensitive to the explicit quantum state of the emitting matter wave and possibly serve as a nondestructive measurement scheme for measuring the quantum state of many-body systems.
The mainstream quantum mechanics uses “probability wave superposition and single-electron self-interference” to explain electron single-slit and double-slit diffraction. This theory deviates from the essential nature of real particle interactions and has fundamental logical flaws. The electron is a negatively charged real particle with a definite physical size and high-frequency transverse oscillation; a single real particle has no physical basis for self-interference. Abandoning the abstract probability wave hypothesis, this paper establishes a complete real-interaction model including electrostatic repulsion deflection, surface electron exchange, collision scattering, microscopic refraction, and barrier diffraction, based on the three-dimensional random transverse oscillation and charge repulsion of electrons. The model uniformly explains the real formation mechanism of electron single-slit diffraction and double-slit interference fringes. This paper proves that in single-electron sequential emission, each electron passes through only one slit; all bright and dark fringes are the statistical result of multiple microscopic interactions between electrons and slit walls or the central barrier. The disappearance of fringes under observation is caused by external disturbance to the inherent oscillation and wall-interaction equilibrium, not by wave function collapse. This paper further clarifies that whether an electron can pass through a slit is determined by its transverse oscillation amplitude, not by wavelength. Amplitude directly corresponds to slit width and is the core controlling variable of diffraction. Meanwhile, if no slit is placed, electrons flying directly to the screen produce no diffraction or interference fringes, proving that electrons themselves have no self-interference ability. Fringes are generated by slit structures, not by intrinsic wave interference of electrons. This study corrects the century-long misunderstanding of electron diffraction and establishes a new microscopic diffraction mechanism consistent with classical real-particle physics.