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Quantum dynamics of a single, mobile spin impurity

Takeshi Fukuhara, Adrian Kantian, Manuel Endres, Marc Cheneau, Peter Schauß, Sebastian J. Hild, David Bellem, Ulrich Schollwöck, Thierry Giamarchi, Christian Groß, Immanuel Bloch, Stefan Kuhr

Published Jan 1, 2013• 1 citation
Publisher

Abstract

One of the elementary processes in quantum magnetism is the propagation of spin excitations. Here we study the quantum dynamics of a deterministically created spin-impurity atom, as it propagates in a one-dimensional lattice system [1]. We probe the spatial probability distribution of the impurity at different times using single-site-resolved imaging of bosonic atoms in an optical lattice. In the Mott-insulating regime, the quantum-coherent propagation of a magnetic excitation in the Heisenberg model can be observed using a post-selection technique. Extending the study to the superfluid regime of the bath, we quantitatively determine how the bath affects the motion of the impurity, showing evidence of polaronic behaviour. The experimental data agree with theoretical predictions, allowing us to determine the effect of temperature on the impurity motion. Our results provide a new approach to studying quantum magnetism, mobile impurities in quantum fluids and polarons in lattice systems.

DOI
10.1364/cleo_qels.2013.qw3c.2

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One of the elementary processes in quantum magnetism is the propagation of spin excitations. Here we study the quantum dynamics of a deterministically created spin-impurity atom, as it propagates in a one-dimensional lattice system [1]. We probe the spatial probability distribution of the impurity at different times using single-site-resolved imaging of bosonic atoms in an optical lattice. In the Mott-insulating regime, the quantum-coherent propagation of a magnetic excitation in the Heisenberg model can be observed using a post-selection technique. Extending the study to the superfluid regime of the bath, we quantitatively determine how the bath affects the motion of the impurity, showing evidence of polaronic behaviour. The experimental data agree with theoretical predictions, allowing us to determine the effect of temperature on the impurity motion. Our results provide a new approach to studying quantum magnetism, mobile impurities in quantum fluids and polarons in lattice systems.
We consider bosonic atoms in an optical lattice at integer filling, tuned to the superfluid--Mott-insulator critical point, and coupled to a single, mobile impurity atom of a different species. This setup is inspired by current experiments with quantum gas microscopes, which enable tracking of the impurity motion. We describe the evolution of the impurity motion from the quantum wave packet spread at short times, to Brownian diffusion at long times. This dynamics is controlled by the interplay between dangerously irrelevant perturbations at the strongly interacting field theory describing the superfluid-insulator transition in two spatial dimensions.
The most recent advances in the ultracold atoms experimental techniques allowed the production of the ultracold gases mixtures in the laboratory.Motivated by these developments, in this project we study systems involving two ultracold atoms mixtures.In the first part, we consider a Bose-Einstein condensate (BEC) with a vortex lattice weakly interacting with another utracold dilute bosonic gas.We apply the Bose-Hubbard (BH) model to describe the atoms of the minority species trapped in the vortex lattice.As occurs in a static optical lattice, we predict the quantum phase transition between the Mott insulator to superfluid phases, which now can be controlled by changing the intra and inter-species scattering length.Considering the intrinsic lattice dynamics, the Tkachenko modes of the vortex lattice, we derive an extended BH Hamiltonian and analyzed new properties in the phase diagram that arise from a long-range attractive potential and density-dependent hopping.In the second part, we study the properties of a mobile impurity living in two dimensions and interacting with a 2 and 3 BEC cloud.The resulting impurity-bath interaction leads to the formation of a polaron (particle "dressed" by the phonon excitations of the BEC), which is characterized by its spectral function.We determine the energy dispersion, spectral weight, effective mass and lifetime of the polaron.These analysis allowed us to identify a dissipative regime for higher impurity velocities, with an increasing scattering rate of phonons.In addition, we observe a self-localization regime for lower impurity velocities which may be a signature for molecular formation.In spite of qualitatively similar results obtained for the 2 and 3 bath, we had differences related to the self-localization and dissipation limits, that allowed us to conclude that a 2 BEC bath would be a better candidate to observe stable quasi-particle properties.
We study the physics of a mobile impurity confined in a two-dimensional lattice, moving within a Bose-Hubbard bath at zero temperature. Exploiting the quantum Gutzwiller formalism, we develop a beyond-Fröhlich model of the bath-impurity interaction to describe the properties of the polaronic quasiparticle formed by the dressing of the impurity by quantum fluctuations of the bath. We find a stable and well-defined polaron throughout the entire phase diagram of the bath, except for the very low tunneling limit of the hard-core superfluid. The polaron properties are highly sensitive to the different universality classes of the quantum phase transition between the superfluid and Mott insulating phases, providing an unambiguous probe of correlations and collective modes in a quantum critical many-body environment.
We study the non-equilibrium dynamics of an impurity in a harmonic trap that is kicked with a well-defined quasi-momentum, and interacts with a bath of free fermions or interacting bosons in a one-dimensional lattice configuration. Using numerical and analytical techniques we investigate the full dynamics beyond linear response, which allows us to quantitatively characterize states of the impurity in the bath for different parameter regimes. These vary from a tightly bound molecular state in a strongly interacting limit to a polaron (dressed impurity) and a free particle for weak interactions, with composite behaviour in the intermediate regime. These dynamics and different parameter regimes should be readily realizable in systems of cold atoms in optical lattices.
We study the non-equilibrium dynamics of an impurity in a harmonic trap that is kicked with a well-defined quasi-momentum, and interacts with a bath of free fermions or interacting bosons in a one-dimensional lattice configuration. Using numerical and analytical techniques we investigate the full dynamics beyond linear response, which allows us to quantitatively characterize states of the impurity in the bath for different parameter regimes. These vary from a tightly bound molecular state in a strongly interacting limit to a polaron (dressed impurity) and a free particle for weak interactions, with composite behaviour in the intermediate regime. These dynamics and different parameter regimes should be readily realizable in systems of cold atoms in optical lattices.
A mobile impurity particle immersed in a quantum degenerate gas leads to the formation of a quasiparticle, which can serve as a sensor for its environment. Here, we develop a unified wave function description of an impurity in a two-dimensional Bose-Hubbard model across the Mott-insulator to superfluid transition. Using a multi-mode variational ansatz based on the quantum Gutzwiller approach, we show that the impurity can form several kinds of polaronic and molecular states. In addition to their spectral properties, the wave function provides direct access to the microscopic structure of these states, and we demonstrate that strong correlations in the critical regime of the quantum phase transition give rise to several non-analytic features in the polaron properties. Increasing the impurity-boson interaction leads to transitions between polaron and molecular ground states, and the number of bosons in the impurity dressing cloud grows rapidly at the quantum critical point as the bath modes soften. We furthermore reveal qualitatively distinct non-equilibrium many-body dynamics after the injection of the impurity in the different phases of the Bose-Hubbard model. Our spectral, real space, and dynamical predictions describe complementary properties of polarons in a strongly correlated bosonic bath, which can be observed using current techniques with atoms in optical lattices.