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Bulletin of the American Physical Society

Electric dipole matrix elements for the $6p\ ^2P_J \rightarrow 7s\ ^2S_{1/2}$ transitions in atomic cesium

George Toh, Amy Damitz, Nathan Glotzbach, Jonah Quirk, Ian Stevenson, Jungu Choi, Marianna S. Safronova, Daniel S. Elliott

Published May 29, 2019• 0 citations
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Matrix-element spectroscopy of the 5s $^{2}S_{1/2}$ $\rightarrow$ 5p $^{2}P_{j}$ $\rightarrow$ 5d $^{2}D_{j'}$ transitions in $^{87}$Rb

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Electric dipole matrix elements for the 6p2PJ→7s2S1/2 transition in atomic cesium

George Toh, Amy Damitz, Nathan Glotzbach +5 more

We report a measurement of the ratio of electric dipole transition matrix elements of cesium for the $6p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rightarrow}7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ and $6p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rightarrow}7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ transitions. We determine this ratio of matrix elements through comparisons of two-color, two-photon excitation rates of the $7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ state using laser beams with polarizations parallel to one another vs perpendicular to one another. Our result of $R\ensuremath{\equiv}\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rangle}/\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rangle}=1.5272(17)$ is in excellent agreement with a theoretical prediction of $R=1.5270(27)$. Moreover, the accuracy of the experimental ratio is sufficiently high to differentiate between various theoretical approaches. To our knowledge, there are no prior experimental measurements of $R$. Combined with our recent determination of the lifetime of the $7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ state, we determine reduced matrix elements for these two transitions, $\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rangle}=\ensuremath{-}6.489(5)\phantom{\rule{4pt}{0ex}}{a}_{0}$ and $\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rangle}=\ensuremath{-}4.249(4)\phantom{\rule{4pt}{0ex}}{a}_{0}$. These matrix elements are also in excellent agreement with theoretical calculations. These measurements improve knowledge of Cs properties needed for parity violation studies and provide benchmarks for tests of high-precision theory.

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Measurement of the Stark shift of the 6s$^{2}$S$_{1/2}$ $\to$ 7p$^{2}$P$_{\mathrm{J}}$ transitions in atomic cesium

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Experimental and Theoretical Study of Dynamic Polarizabilities in the 5S1/2 – 5D5/2 Clock Transition in Rubidium-87 and Determination of Electric Dipole Matrix Elements

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The interaction between light and an atom causes perturbations in the atom's energy levels, known as the light shift. These light shifts are a key source of inaccuracy in atomic clocks, and can also deteriorate their precision. We present a study of light shifts and associated dynamic polarizabilities for a two-photon atomic clock based on the $5{S}_{1/2}$--$5{D}_{5/2}$ transition in rubidium-87 over the range 770--800 nm. We determine experimental and theoretical values for a magic wavelength in this range and the electric dipole (E1) matrix element for the $5{P}_{3/2}$--$5{D}_{5/2}$ transition. We find a magic wavelength of 776.179(5) nm (experimental) and 776.21 nm (theoretical) in the vicinity of the $5{P}_{3/2}$--$5{D}_{5/2}$ resonance, and the corresponding reduced E1 matrix element $1.80(6)e{a}_{0}$ (experimental) and $1.96(15)e{a}_{0}$ (theoretical). These values resolve a previous discrepancy between theory and experiment.

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Measurement of the ratio of the 6P$_{\mathrm{j}}\to $ 7S $_{\mathrm{\raise.5ex\hbox{$\scriptstyle 1$}\kern-.1em/ \kern-.15em\lower.25ex\hbox{$\scriptstyle 2$} }}$ matrix elements in atomic cesium

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Magnetic Sublevel Independent Magic and Tune-Out Wavelengths of the Alkaline-Earth Ions

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Light shift in a state due to the applied laser in an atomic system vanishes at tune-out wavelengths (λTs). Similarly, differential light shift in a transition vanishes at the magic wavelengths (λmagics). In many of the earlier studies, values of the electric dipole (E1) matrix elements were inferred precisely by combining measurements and calculations of λmagic. Similarly, the λT values of an atomic state can be used to infer the E1 matrix element, as it involves dynamic electric dipole (α) values of only one state whereas the λmagic values require evaluation of α values for two states. However, both the λmagic and λT values depend on angular momenta and their magnetic components (M) of states. Here, we report the λmagic and λT values of many S1/2 and D3/2,5/2 states, and transitions among these states of the Mg+, Ca+, Sr+ and Ba+ ions that are independent of M values. It is possible to infer a large number of E1 matrix elements of the above ions accurately by measuring these values and combining with our calculations.

arXiv:2309.16910•Atoms•Jul 11, 2022•3 citations
Electric dipole matrix elements for the 6p 2PJ→7s 2S1/26p\ ^2P_J \rightarrow 7s\ ^2S_{1/2}6p 2PJ​→7s 2S1/2​ transitions in atomic cesium
Matrix-element spectroscopy of the 5s 2S1/2^{2}S_{1/2}2S1/2​ →\rightarrow→ 5p 2Pj^{2}P_{j}2Pj​ →\rightarrow→ 5d 2Dj′^{2}D_{j'}2Dj′​ transitions in 87^{87}87Rb
We report a measurement of the ratio of electric dipole transition matrix elements of cesium for the $6p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rightarrow}7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ and $6p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rightarrow}7s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}$ transitions. We determine this ratio of matrix elements through comparisons of two-color, two-photon excitation rates of the 7s2S1/27s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}7s2S1/2​ state using laser beams with polarizations parallel to one another vs perpendicular to one another. Our result of $R\ensuremath{\equiv}\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rangle}/\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rangle}=1.5272(17)$ is in excellent agreement with a theoretical prediction of R=1.5270(27)R=1.5270(27)R=1.5270(27). Moreover, the accuracy of the experimental ratio is sufficiently high to differentiate between various theoretical approaches. To our knowledge, there are no prior experimental measurements of RRR. Combined with our recent determination of the lifetime of the 7s2S1/27s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}7s2S1/2​ state, we determine reduced matrix elements for these two transitions, $\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{3/2}\ensuremath{\rangle}=\ensuremath{-}6.489(5)\phantom{\rule{4pt}{0ex}}{a}_{0}$ and $\ensuremath{\langle}7s{\phantom{\rule{4pt}{0ex}}}^{2}{S}_{1/2}||r||6p{\phantom{\rule{4pt}{0ex}}}^{2}{P}_{1/2}\ensuremath{\rangle}=\ensuremath{-}4.249(4)\phantom{\rule{4pt}{0ex}}{a}_{0}$. These matrix elements are also in excellent agreement with theoretical calculations. These measurements improve knowledge of Cs properties needed for parity violation studies and provide benchmarks for tests of high-precision theory.
Measurement of the Stark shift of the 6s2^{2}2S1/2_{1/2}1/2​ →\to→ 7p2^{2}2PJ_{\mathrm{J}}J​ transitions in atomic cesium
The interaction between light and an atom causes perturbations in the atom's energy levels, known as the light shift. These light shifts are a key source of inaccuracy in atomic clocks, and can also deteriorate their precision. We present a study of light shifts and associated dynamic polarizabilities for a two-photon atomic clock based on the 5S1/25{S}_{1/2}5S1/2​--5D5/25{D}_{5/2}5D5/2​ transition in rubidium-87 over the range 770--800 nm. We determine experimental and theoretical values for a magic wavelength in this range and the electric dipole (E1) matrix element for the 5P3/25{P}_{3/2}5P3/2​--5D5/25{D}_{5/2}5D5/2​ transition. We find a magic wavelength of 776.179(5) nm (experimental) and 776.21 nm (theoretical) in the vicinity of the 5P3/25{P}_{3/2}5P3/2​--5D5/25{D}_{5/2}5D5/2​ resonance, and the corresponding reduced E1 matrix element 1.80(6)ea01.80(6)e{a}_{0}1.80(6)ea0​ (experimental) and 1.96(15)ea01.96(15)e{a}_{0}1.96(15)ea0​ (theoretical). These values resolve a previous discrepancy between theory and experiment.
Light shift in a state due to the applied laser in an atomic system vanishes at tune-out wavelengths (λTs). Similarly, differential light shift in a transition vanishes at the magic wavelengths (λmagics). In many of the earlier studies, values of the electric dipole (E1) matrix elements were inferred precisely by combining measurements and calculations of λmagic. Similarly, the λT values of an atomic state can be used to infer the E1 matrix element, as it involves dynamic electric dipole (α) values of only one state whereas the λmagic values require evaluation of α values for two states. However, both the λmagic and λT values depend on angular momenta and their magnetic components (M) of states. Here, we report the λmagic and λT values of many S1/2 and D3/2,5/2 states, and transitions among these states of the Mg+, Ca+, Sr+ and Ba+ ions that are independent of M values. It is possible to infer a large number of E1 matrix elements of the above ions accurately by measuring these values and combining with our calculations.