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Physical Review Letters

Accurate and Robust Unitary Transformations of a High-Dimensional Quantum System

Brian E. Anderson, Hector Sosa Martinez, Carlos A. Riofrío, Ivan Deutsch, Poul Jessen

Published Jun 16, 2015• 93 citations
Publisher

Abstract

Unitary transformations are the most general input-output maps available in closed quantum systems. Good control protocols have been developed for qubits, but questions remain about the use of optimal control theory to design unitary maps in high-dimensional Hilbert spaces, and about the feasibility of their robust implementation in the laboratory. Here we design and implement unitary maps in a 16-dimensional Hilbert space associated with the 6S(1/2) ground state of (133)Cs, achieving fidelities >0.98 with built-in robustness to static and dynamic perturbations. Our work has relevance for quantum information processing and provides a template for similar advances on other physical platforms.

DOI
10.1103/physrevlett.114.240401

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Unitary transformations are the most general input-output maps available in closed quantum systems. Good control protocols have been developed for qubits, but questions remain about the use of optimal control theory to design unitary maps in high-dimensional Hilbert spaces, and about the feasibility of their robust implementation in the laboratory. Here we design and implement unitary maps in a 16-dimensional Hilbert space associated with the 6S(1/2) ground state of (133)Cs, achieving fidelities >0.98 with built-in robustness to static and dynamic perturbations. Our work has relevance for quantum information processing and provides a template for similar advances on other physical platforms.
Quantum control in large dimensional Hilbert spaces is essential for realizing the power of quantum information processing. For closed quantum systems the relevant input/output maps are unitary transformations, and the fundamental challenge becomes how to implement these with high fidelity in the presence of experimental imperfections and decoherence. For two-level systems (qubits) most aspects of unitary control are well understood, but for systems with Hilbert space dimension d>2 (qudits), many questions remain regarding the optimal design of control Hamiltonians and the feasibility of robust implementation. Here we show that arbitrary, randomly chosen unitary transformations can be efficiently designed and implemented in a large dimensional Hilbert space (d=16) associated with the electronic ground state of atomic 133Cs, achieving fidelities above 0.98 as measured by randomized benchmarking. Generalizing the concepts of inhomogeneous control and dynamical decoupling to d>2 systems, we further demonstrate that these qudit unitary maps can be made robust to both static and dynamic perturbations. Potential applications include improved fault-tolerance in universal quantum computation, nonclassical state preparation for high-precision metrology, implementation of quantum simulations, and the study of fundamental physics related to open quantum systems and quantum chaos.
Neutral atom systems are an appealing platform for the development and testing of quantum control and measurement techniques. This dissertation presents experimental investigations of control and measurement tools using as a testbed the 16-dimensional hyperfine manifold associated with the electronic ground state of 133^{133}133Cs atoms. On the control side, we present an experimental realization of a protocol to implement robust unitary transformations in the presence of static and dynamic perturbations. We also present an experimental realization of inhomogeneous quantum control. Specifically, we demonstrate our ability to perform two different unitary transformations on atoms that see different light shifts from an optical addressing field. On the measurement side, we present experimental realizations of quantum state and process tomography. The state tomography project encompasses a comprehensive evaluation of several measurement strategies and state estimation algorithms. Our experimental results show that in the presence of experimental imperfections, there is a clear tradeoff between accuracy, efficiency and robustness in the reconstruction. The process tomography project involves an experimental demonstration of efficient reconstruction by using a set of intelligent probe states. Experimental results show that we are able to reconstruct unitary maps in Hilbert spaces with dimension ranging from d=4d = 4d=4 to d=16d = 16d=16. To the best of our knowledge, this is the first time that a unitary process in d=16d = 16d=16 is successfully reconstructed in the laboratory.
The optimal control of unitary transformations is a fundamental problem in quantum control theory and quantum information processing. The feasibility of performing such optimizations is determined by the computational and control resources required, particularly for systems with large Hilbert spaces. Prior work on unitary transformation control indicates that (i) for controllable systems, local extrema in the search landscape for optimal control of quantum gates have null measure, facilitating the convergence of local search algorithms, but (ii) the required time for convergence to optimal controls can scale exponentially with the Hilbert space dimension. Depending on the control-system Hamiltonian, the landscape structure and scaling may vary. This work introduces methods for quantifying Hamiltonian-dependent and kinematic effects on control optimization dynamics in order to classify quantum systems according to the search effort and control resources required to implement arbitrary unitary transformations.
Neutral atom systems are an appealing platform for the development and testing of quantum control and measurement techniques. This dissertation presents experimental investigations of control and measurement tools using as a testbed the 16-dimensional hyperfine manifold associated with the electronic ground state of 133^{133}133Cs atoms. On the control side, we present an experimental realization of a protocol to implement robust unitary transformations in the presence of static and dynamic perturbations. We also present an experimental realization of inhomogeneous quantum control. Specifically, we demonstrate our ability to perform two different unitary transformations on atoms that see different light shifts from an optical addressing field. On the measurement side, we present experimental realizations of quantum state and process tomography. The state tomography project encompasses a comprehensive evaluation of several measurement strategies and state estimation algorithms. Our experimental results show that in the presence of experimental imperfections, there is a clear tradeoff between accuracy, efficiency and robustness in the reconstruction. The process tomography project involves an experimental demonstration of efficient reconstruction by using a set of intelligent probe states. Experimental results show that we are able to reconstruct unitary maps in Hilbert spaces with dimension ranging from d=4d = 4d=4 to d=16d = 16d=16. To the best of our knowledge, this is the first time that a unitary process in d=16d = 16d=16 is successfully reconstructed in the laboratory.
Quantum systems with Hilbert space dimension greater than two (qudits) provide an alternative to qubits as carriers of quantum information, and may prove advantageous for quantum information tasks if good laboratory tools for qudit manipulation and readout can be developed. We have implemented a protocol for arbitrary unitary transformations in the 16 dimensional hyperfine ground manifold of Cesium 133 atoms, using phase modulated rf and microwave magnetic fields to drive the atomic evolution. Our phase modulation waveforms are designed numerically using a variant of the highly efficient GRAPE algorithm. The fidelity of the resulting transformations is verified experimentally through randomized benchmarking, which indicates an average fidelity better than 97% across a sample of random unitaries.
Robust control design for quantum unitary transformations has been recognized as a fundamental and challenging task in the development of quantum information processing due to unavoidable decoherence or operational errors in the experimental implementation of quantum operations. In this paper, we extend the systematic methodology of sampling-based learning control (SLC) approach with a gradient flow algorithm for the design of robust quantum unitary transformations. The SLC approach first uses a "training" process to find an optimal control strategy robust against certain ranges of uncertainties. Then a number of randomly selected samples are tested and the performance is evaluated according to their average fidelity. The approach is applied to three typical examples of robust quantum transformation problems including robust quantum transformations in a three-level quantum system, in a superconducting quantum circuit, and in a spin chain system. Numerical results demonstrate the effectiveness of the SLC approach and show its potential applications in various implementation of quantum unitary transformations.