Quantum networks are a rapidly developing field of quantum information processing that have the potential to enable long-range entanglement between future quantum computers as well as the implementation of secure communication through quantum key distribution. Two key components of such networks are quantum memories to store entangled photon pairs for use in the quantum repeater protocol and quantum light-matter interfaces to efficiently interconvert between stationary qubits and flying qubits in the form of photons. Rare-earth ion-doped crystals are a promising solid-state platform that show promise for both of these applications due to their long optical and spin coherence times. Due to their relatively weak optical transitions, rare-earth ions have been coupled with nanophotonic resonators to enhance their transition strengths, with past work in the Faraon group utilizing focused ion beam milled photonic crystal resonators with 45-degree angled couplers to couple light in and out. Such resonators have the disadvantage of requiring manual alignment to fabricate, and the couplers are also relatively inefficient which limits the performance of such devices. It is therefore desirable to move towards silicon photonics, where mature techniques such as electron-beam lithography can allow for scalable fabrication of nanophotonic cavities together with high coupling efficiencies. In this thesis, we demonstrate significant progress towards the usage of acid-etched tapered optical fibers as an efficient interface for coupling light into tapered silicon nanophotonic waveguides. We show comprehensive simulations of the taper geometries required to achieve adiabatic coupling with theoretical efficiencies of more than 99%, and design a silicon photonic crystal mirror to be used in the measurement of the fiber-waveguide coupling efficiency. We then optimize the hydrofluoric acid fiber etching process and demonstrate the ability to make tapered fibers which are 200 microns long with a taper half-angle of 2 degrees and a tip diameter of 50 nm. Using these tapered fibers to couple light into tapered silicon waveguides fabricated using electron-beam lithography shows a moderately high coupling efficiency of 11.4% with the potential for improvement. This method of tapered fiber coupling shows promise to be integrated into silicon nanophotonic resonators on rare-earth ion doped crystals and allow for highly efficient quantum memories and quantum light-matter interfaces in the solid-state.
Quantum networks are a rapidly developing field of quantum information processing that have the potential to enable long-range entanglement between future quantum computers as well as the implementation of secure communication through quantum key distribution. Two key components of such networks are quantum memories to store entangled photon pairs for use in the quantum repeater protocol and quantum light-matter interfaces to efficiently interconvert between stationary qubits and flying qubits in the form of photons. Rare-earth ion-doped crystals are a promising solid-state platform that show promise for both of these applications due to their long optical and spin coherence times. Due to their relatively weak optical transitions, rare-earth ions have been coupled with nanophotonic resonators to enhance their transition strengths, with past work in the Faraon group utilizing focused ion beam milled photonic crystal resonators with 45-degree angled couplers to couple light in and out. Such resonators have the disadvantage of requiring manual alignment to fabricate, and the couplers are also relatively inefficient which limits the performance of such devices. It is therefore desirable to move towards silicon photonics, where mature techniques such as electron-beam lithography can allow for scalable fabrication of nanophotonic cavities together with high coupling efficiencies. In this thesis, we demonstrate significant progress towards the usage of acid-etched tapered optical fibers as an efficient interface for coupling light into tapered silicon nanophotonic waveguides. We show comprehensive simulations of the taper geometries required to achieve adiabatic coupling with theoretical efficiencies of more than 99%, and design a silicon photonic crystal mirror to be used in the measurement of the fiber-waveguide coupling efficiency. We then optimize the hydrofluoric acid fiber etching process and demonstrate the ability to make tapered fibers which are 200 microns long with a taper half-angle of 2 degrees and a tip diameter of 50 nm. Using these tapered fibers to couple light into tapered silicon waveguides fabricated using electron-beam lithography shows a moderately high coupling efficiency of 11.4% with the potential for improvement. This method of tapered fiber coupling shows promise to be integrated into silicon nanophotonic resonators on rare-earth ion doped crystals and allow for highly efficient quantum memories and quantum light-matter interfaces in the solid-state.
With an assortment of narrow line-width transitions spanning the visible and IR spectrum and long spin coherence times, rare-earth doped crystals are the leading material system for solid-state quantum memories. Integrating these materials in an on-chip optical platform would create opportunities for highly integrated light-matter interfaces for quantum communication and quantum computing. Nano-photonic resonators with high quality factors and small mode volumes are required for efficient on-chip coupling to the small dipole moment of rare-earth ion transitions. However, direct fabrication of optical cavities in these crystals with current nanofabrication techniques is difficult and unparallelized, as either exotic etch chemistries or physical milling processes are required. We fabricated hybrid devices by mechanically transferring a nanoscale membrane of gallium arsenide (GaAs) onto a neodymium-doped yttrium silicon oxide (Y2SiO5) crystal and then using electron beam lithography and standard III-V dry etching to pattern nanobeam photonic crystal cavities and ring resonator cavities, a technique that is easily adapted to other frequency ranges for arbitrary dopants in any rare earth host system. Single crystalline GaAs was chosen for its low loss and high refractive index at the transition wavelength. We demonstrated the potential to evanescently couple between the cavity field and the 883 nm 4I9/2- 4F3/2 transition of nearby neodymium impurities in the host crystal by examining transmission spectra through a waveguide coupled to the resonator with a custom-built confocal microscope. The prospects and requirements for using this system for scalable quantum networks are discussed.
Efficient and stable interfaces between quantum devices and optical fibers are a key requirement for realizing large-scale quantum networks and distributed quantum computing. Adiabatic coupling between a diamond waveguide and a tapered fiber provides a promising route to broadband, efficient, and robust optical coupling [*]. In this work, we present the design, fabrication, and characterization of such interface. First, we performed FDTD simulations to optimize the diamond nanobeam geometry. These simulations predict a maximum coupling efficiency of 98% with an optimized design. Next, tapered optical fibers with angles <3° and tips <150 nm were fabricated using an optimized hydrofluoric acid etching process. Finally, we experimentally evaluated the coupling efficiency by measuring photoluminescence from nitrogen-vacancy centers in a diamond nanobeam through the fiber, yielding an efficiency of 14%. These results establish a clear design path for a practical interface. The gap between simulation and experiment highlights the need to improve physical contact and nanobeam fabrication. Future work will target these optimizations to realize a more efficient and robust packaged device, a critical component for quantum networks.
The growing interest in optical quantum systems has led to the exploration of multiple platforms. Though pioneering experiments were performed in trapped atom and trapped ion systems, solid state systems show promise of being scalable and robust. Rare earth dopants in crystalline hosts are an appealing option because they possess a rich spectrum of energy levels that result from a partially filled electron orbital. While level structure varies across the period, all elements possess crystal field splittings corresponding to near infra-red or optical frequencies, as well as Zeeman and often hyperfine levels separated by radio frequency and microwave frequencies. These levels demonstrate long excited-state lifetimes and coherence times and have been used in diverse applications, including demonstrating storage of a photonic state, converting of optical to microwave photons, and manipulating a single ion as a single qubit. The ions' weak interaction with their environment results in low coupling to optical fields, which had previously required measurements with macroscopically large ensembles of ions. Coupling the ions to an optical cavity enables the use of a smaller ensemble, which is required for the development of the aforementioned technologies in an on-chip scalable architecture. This thesis contains recent progress towards fabricating optical micro and nanocavities coupled to ensembles of erbium ions, mainly erbium in yttrium orthosilicate. In one design, focused ion beam milling was used to create a triangular nanobeam photonic crystal cavity in a bulk erbium-doped substrate. A second design leveraged the fabrication capabilities of silicon photonics, defining amorphous silicon ring resonators using electron beam lithography and dry etching. These devices coupled evanescently to erbium ions below the ring, in the bulk substrate. Simulation, design, fabrication, and characterization of both resonators are discussed. Coupling between the ions and the resonator is demonstrated for each, and capabilities offered by these devices are described. Preliminary work implementing coherent control of erbium ions is presented. Lastly, alternative substrates are evaluated for possible future solid-state erbium systems.
This paper presents progress in developing crystalline waveguides to enable efficient and integrated quantum memories for long-distance quantum communications. The primary objective is to overcome low light-matter interaction strength encountered in rare-earth ion (REI) doped crystals, particularly Yttrium Orthosilicate (YSO), which limits optical storage efficiencies. Compared to other strategies toward photonic integration, our novel approach utilizes traditional lithography and dry-etching techniques to retain the beneficial properties of bulk crystals while allowing for design flexibility. Bonding, lapping, polishing, and dry-etching processes were optimized to fabricate the suitable YSO waveguide geometry demonstrated by simulations. This research paves the way toward fully integrated quantum repeaters. It also contributes toward integration for other REI-doped crystals-based quantum technologies such as quantum computing, single photon generation, RF spectral analysis, and microwave-to-optical quantum transduction.
The sub-wavelength optical confinement and low optical loss of nanophotonic devices dramatically enhances the interaction between light and matter within these structures. When nanophotonic devices are combined with an efficient optical coupling channel, nonlinear optical behavior can be observed at low power levels in weakly-nonlinear materials. In a similar vein, when resonant atomic systems interact with nanophotonic devices, atom-photon coupling effects can be observed at a single quanta level. Crucially, the chip based nature of nanophotonics provides a scalable platform from which to study these effects. This thesis addresses the use of nanophotonic devices in nonlinear and quantum optics, including device design, optical coupling, fabrication and testing, modeling, and integration with more complex systems. We present a fiber taper coupling technique that allows efficient power transfer from an optical fiber into a photonic crystal waveguide. Greater than 97% power transfer into a silicon photonic crystal waveguide is demonstrated. This optical channel is then connected to a high-Q (> 40,000), ultra-small mode volume (V 44% of the photons input to a fiber. This permits the observation of optical bistability in silicon for sub-mW input powers at telecommunication wavelengths. To port this technology to cavity QED experiments at near-visible wavelengths, we also study silicon nitride microdisk cavities at wavelengths near 852 nm, and observe resonances with Q > 3 million and V
I present quantum nano-photonic devices based on nanophotonic resonators coupled to rare-earth-ions in crystals. The rare-earth ions exhibit long coherence times on optical transitions, which makes them suitable for optical quantum memories. We demonstrate a high-fidelity nanophotonic quantum memory based on a mesoscopic rare-earth ensemble coupled to a photonic crystal cavity. The nanocavity enables >95% spin polarization for efficient initialization of the atomic frequency comb memory, and time-bin-selective readout via enhanced optical Stark shift of the comb frequencies. Besides ensemble memories, single rare-earth-ions coupled to nano-resonators can be used as single optically addressable quantum bits where the quantum state is mapped on their Zeeman or hyperfine levels with long coherence time. Our solid-state nano-photonic quantum light-matter interfaces can be integrated with other chip-scale photon source and detector devices for multiplexed quantum and classical information processing at the nodes of quantum networks.