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Coherent multiple scattering: from atomic matter waves to light and vice versa

Nicolas Cherroret

Published Nov 14, 2018• 1 citation
OpenAlex

Abstract

This manuscript presents a selection of works on the coherent evolution of atomic matter waves in random potentials. In this context, a number of interference, « mesoscopic » phenomena surviving a disorder average are discussed, in particular in the regime where Anderson localization shows up: coherent backscattering, coherent forward scattering, mesoscopic echo and quantum boomerang effect. The interplay between weak atomic interactions and Anderson localization is also touched upon for spreading wave packets, a scenario frequently considered in experiments. The last chapter, finally, gives an overview of recent works by the author on multiple scattering of light in media of dimension « (2+1) ». These peculiar systems, originally introduced to demonstrate Anderson localization of light in 2D, have sparked a growing interest in the recent years, for light propagation is governed by an effective Schrödinger equation and thus mimics the behavior of a matter wave. We here show that when the vector character of light is properly taken into account, these systems in fact display a physics much richer than the one pertained to this sole analogy.

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arXiv:quant-ph/0107030•Physical Review A•Oct 2, 2001•62 citations
This manuscript presents a selection of works on the coherent evolution of atomic matter waves in random potentials. In this context, a number of interference, « mesoscopic » phenomena surviving a disorder average are discussed, in particular in the regime where Anderson localization shows up: coherent backscattering, coherent forward scattering, mesoscopic echo and quantum boomerang effect. The interplay between weak atomic interactions and Anderson localization is also touched upon for spreading wave packets, a scenario frequently considered in experiments. The last chapter, finally, gives an overview of recent works by the author on multiple scattering of light in media of dimension « (2+1) ». These peculiar systems, originally introduced to demonstrate Anderson localization of light in 2D, have sparked a growing interest in the recent years, for light propagation is governed by an effective Schrödinger equation and thus mimics the behavior of a matter wave. We here show that when the vector character of light is properly taken into account, these systems in fact display a physics much richer than the one pertained to this sole analogy.
Propagation in a random medium is often described by a random walk and a diffusion coefficient. However in the mesoscopic regime, where wave properties cannot be neglected, interferences alter the diffusion process leading in extreme situations to strong (Anderson) localisation. The recent observation of coherent backscattering of light by laser cooled atoms has opened the way to new studies in previously not accessible regimes. Here we present some of the questions addressed by these experiments, allowing for a more complete understanding of the physical processes involved in this quantum mesoscopic regime
Propagation in a random medium is often described by a random walk and a diffusion coefficient. However in the mesoscopic regime, where wave properties cannot be neglected, interferences alter the diffusion process leading in extreme situations to strong (Anderson) localisation. The recent observation of coherent backscattering of light by laser cooled atoms has opened the way to new studies in previously not accessible regimes. In this paper we present some of the questions addressed by these experiments, allowing for a more complete understanding of the physical processes involved in this quantum mesoscopic regime
This thesis presents the author's work on multiple scattering of intense laser light by cold atoms in chapter 2 and nonlinear coherent backscattering in chapter 3. The basic concepts and most important results should be understandable from reading these chapters on their own, whereas we refer to the subsequent collection of articles (P1-P11) for more detailed treatments. In chapter 2.1, we review scattering of light by a single two-level atom, with special emphasis on the fact that the atoms are nonlinear and inelastic scatterers, which will be relevant for multiple scattering. In chapter 2.2, we treat double scattering by two distant atoms, before we generalize this technique to a dilute disordered sample of many atoms in chapter 2.3. Both 2.2 and 2.3 apply in the perturbative regime of low laser intensity, where, by analyzing scattering of two photons, we clarify the different roles of nonlinearity and inelasticity concerning the coherent backscattering interference. Chapter 2.4 discusses the master equation as a complementary approach, applicable at arbitrarily high laser intensity, but only for a small number of atoms. In addition, we present an equivalent new approach, which explicitly takes advantage of the large distance between the atoms, and thereby combines the advantages of the master equation and the scattering approach. As discussed in chapter 2.5, this new approach opens the way to a non-perturbative theory for multiple scattering of intense laser light by dilute atomic clouds. Chapter 3 presents our diagrammatic theory for nonlinear coherent backscattering of classical (or single-particle quantum) waves. In chapter 3.1, we explain the most important assumptions of the theory: weak disorder and small nonlinearity, in particular existence of a stable, stationary solution of the nonlinear wave equation. In chapter 3.2, we explain why - contrary to seemingly convincing intuitive reasoning - the nonlinearity indeed changes the height of the coherent backscattering interference peak. In order to describe this effect quantitatively, a diagrammatic theory is sketched in chapters 3.3 and 3.4, where the nonlinear Born series and the nonlinear ladder and crossed diagrams are introduced. Chapter 3.5 presents the transport equations which result from the complete summation of ladder and crossed diagrams - non-perturbatively in the strength of the nonlinearity. We discuss the conditions under which the nonlinearity reduces or enhances the coherent backscattering interference, as compared to the linear case. In order to confirm the validity of the diagrammatic analysis, we compare these results with numerical simulations in chapter 3.6. We conclude with a short account of our work on speckle instabilities for nonlinear point scatterers in chapter 3.7. Finally, chapter 4 describes some future perspectives of our work, in particular the application of the diagrammatic theory to describe the impact of nonlinearity on weak localization and Anderson localization, and possible extensions to the quantum many-particle regime.
Cold atoms have emerged as interesting quantum system to study coherent transport properties of light. First experiments have established that dilute samples with large optical thickness allow studying weak localization of light. The present goal of this research is to study coherent transport of photons in dense samples. The quest for Anderson localization of light is among the most interesting questions currently studied. One important aspect in the quest of Anderson localization of light with cold atoms is the relation of Anderson localization and Dicke super- or subradiance. With large and dense samples of cold atoms the interplay between these different phenomena can be studied. During this research one also has to study anomalous diffusion (Lévy flights of photons) and new situations such as a random lasing can arise if one combines gain with multiple scattering. Cold atoms thus continue to allow for new exciting physics to be investigated.
In this thesis, we investigate the coherent scattering of light propagating in a random medium.We are interested in phenomena like the super-and subradiance and Anderson localization that are related to waves interferences and spatial disorder.However, the fundamental difference between subradiance and Anderson localization still needs to be clarified.This thesis gives new elements for the understanding of these phenomena and we present a new method to observe Anderson localization.A mean-field model that does not contain disorder is developed, and we show that super-and subradiance do not require disorder whereas Anderson localization does.In this theoretical work, the coupling between the light and many atoms is reduced to a coupling matrix between the atoms by tracing over the degrees of freedom of the light, which results in a linear problem for the atomic dipoles.The study of the eigenvalues and eigenmodes of this matrix then allows to determine the super-and subradiant modes, and to probe the Anderson localization phase transition with a scaling analysis.Furthermore, the link to the experiment is realized by showing that the intensity fluctuations present an increase at the localization transition.The system is studied in the steady-state regime when the medium is continuously charged by a laser until reaches a stationary regime, and the decay dynamics, when the laser is switched off, so the cloud releases the energy stored.Finally, we present a preliminary work that shows that the diagonal disorder might be a good strategy to reach Anderson localization.
Since the work of Anderson on localization, interference effects for the propagation of a wave in the presence of disorder have been extensively studied, as exemplified in coherent backscattering (CBS) of light. In the multiple scattering of light by a disordered sample of thermal atoms, interference effects are usually washed out by the fast atomic motion. This is no longer true for cold atoms where CBS has recently been observed. However, the internal structure of the atoms strongly influences the interference properties. In this paper, we consider light scattering by an atomic dipole transition with arbitrary degeneracy and study its impact on coherent backscattering. We show that the interference contrast is strongly reduced. Assuming a uniform statistical distribution over internal degrees of freedom, we compute analytically the single- and double-scattering contributions to the intensity in the weak-localization regime. The so-called ladder and crossed diagrams are generalized to the case of atoms and permit to calculate enhancement factors and backscattering intensity profiles for polarized light and any closed atomic dipole transition.