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Quantum catalysis of multi-photon nonclassical states

Tim J. Bartley, Gaia Donati, Justin B. Spring, Xian‐Min Jin, Marco Barbieri, Animesh Datta, Brian J. Smith, Ian A. Walmsley

Published May 2, 2012• 0 citations
OpenAlex

Abstract

We develop a technique for generating multi-photon nonclassical states via interference between coherent and Fock states using quantum catalysis. By modulating the coherent field strength, the number of catalyst photons and the ratio of the beam splitter upon which they interfere, a wide range of nonclassical phenomena can be created, including squeezing of up to 1.25 dB, anti- and super-bunched photon statistics and states exhibiting over 90% fidelity to displaced coherent superposition states. We perform quantum catalysis experimentally, showing tunability into the nonclassical regime. Our protocol is not limited by weak nonlinearities that underlie most known strategies of preparing multi-photon nonclassical states. Successive iterations of this protocol can lead to direct control over the weights of higher-order terms in the Fock basis, paving the way towards conditional preparation of designer multi-photon states for applications in quantum computation, communication and metrology.

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We develop a technique for generating multi-photon nonclassical states via interference between coherent and Fock states using quantum catalysis. By modulating the coherent field strength, the number of catalyst photons and the ratio of the beam splitter upon which they interfere, a wide range of nonclassical phenomena can be created, including squeezing of up to 1.25 dB, anti- and super-bunched photon statistics and states exhibiting over 90% fidelity to displaced coherent superposition states. We perform quantum catalysis experimentally, showing tunability into the nonclassical regime. Our protocol is not limited by weak nonlinearities that underlie most known strategies of preparing multi-photon nonclassical states. Successive iterations of this protocol can lead to direct control over the weights of higher-order terms in the Fock basis, paving the way towards conditional preparation of designer multi-photon states for applications in quantum computation, communication and metrology.
We develop a technique for generating multiphoton nonclassical states via interference between coherent and Fock states using quantum catalysis. By modulating the coherent field strength, the number of catalyst photons, and the ratio of the beam splitter upon which they interfere, a wide range of nonclassical phenomena can be created, including squeezing of up to 1.25 dB, antibunched and superbunched photon statistics, and states exhibiting over 90% fidelity to displaced coherent superposition states. We perform quantum catalysis experimentally, showing tunability into the nonclassical regime. Our protocol is not limited by weak nonlinearities that underlie most known strategies of preparing multiphoton nonclassical states. Successive iterations of this protocol can lead to direct control over the weights of higher-order terms in the Fock basis, paving the way towards conditional preparation of ``designer'' multiphoton states for applications in quantum computation, communication, and metrology.
We report preparation and characterization of coherent superposition states t[0>+alpha]1> of the electromagnetic field by conditional measurements on a beam splitter. This state is generated in one of the beam splitter output channels if a coherent state [alpha> and a single-photon Fock state [1> are present in the two input ports and a single photon is registered in the other beam splitter output. The single photon thus plays a role of a "catalyst:" it is explicitly present in both the input and the output channels of the interaction yet facilitates generation of a nonclassical state of light.
Based on heralded interference on a six-port Mach-Zehnder interferometer, we propose protocols to generate a series of multiphoton states in primary output port, by injecting a coherent state in primary input port and two Fock states in two ancillary input ports, and measuring two Fock states in two ancillary output ports. Only manipulating at the single-photon level (i.e, |0> or |1>) in all ancillary ports, we generate sixteen types (six categories) of multiphoton nonclassical states, whose state vectors are unified as superposition of a new coherent state, a single-photon added coherent state, and a two-photon added coherent state. Indeed, a wide range of nonclassical phenomena can be created by modulating the interaction parameters (including coherent field strength and shift phase). We mainly analyze quadrature-squeezing effects for all our considered states. Of particular interest is maximum squeezing of up to 2.57dB, with success probability 6.7%, at least in our present cases.
Non-Gaussian quantum states and operations constitute essential resources for achieving quantum computational advantage and enabling quantum error correction in bosonic platforms. However, their generation in optical settings remains a challenging experimental task, often relying on probabilistic heralded protocols. Here, we present an in-depth analysis of the suitability of photon catalysis between low number Fock states and squeezed states for the generation of squeezed coherent state superpositions. We employ the stellar rank formalism to characterize the non-Gaussian complexity of input resources (including both states and measurements) and the generated states. This enables a systematic comparison of the fidelity between the catalyzed output and the target states to the maximum fidelity achievable by any protocol with the same non-Gaussian input resources. In this sense, we identify instances where the catalysis protocols considered here are provably optimal. We identify parameter regimes in which high-fidelity approximations of the target states can be achieved with minimal resources. Furthermore, we benchmark the performance of photon catalysis against Gaussian boson sampling-inspired protocols in terms of success probability and state quality, highlighting the advantages of deterministic Fock state sources. We also investigate the generation of related non-Gaussian resources including squeezed Fock states, relevant for quantum error correction. To account for experimental imperfections, we model losses across all optical modes using a Hilbert space truncation approach in the Fock basis and analyze the robustness of the generated states under realistic conditions. Our results quantify the trade-offs between non-Gaussian resource complexity, achievable fidelity, and losses in photon catalysis protocols, providing practical guidelines for near-term photonic implementations.
Abstract We propose a scheme to generate a new kind of non-Gaussian state—the Laguerre polynomial excited coherent state (LPECS)—by using multiphoton catalysis with coherent state input. The nonclassical properties of the LPECS are studied in terms of nonclassical depth, Mandel’s parameter, second-order correlation, quadrature squeezing, and the negativity of the Wigner function (WF). It is found that the LPECS is highly nonclassical and its nonclassicality depends on the amplitude of the coherent state, the catalysis photon number, and the parameters of the unbalanced beam splitter (BS). In particular, the maximum degree of squeezing can be enhanced by increasing the catalysis photon number. In addition, we examine the effect of decoherence using the WF, which shows that the negative region, the characteristic time of decoherence, and the structure of the WF are affected by catalysis photon number and the parameters of the unbalanced BS. Our work provides general analysis on how to prepare polynomial quantum states, which may be useful in the fields of quantum information and quantum computation.
We theoretically introduce a new kind of non-Gaussian state, namely, the mixture of multiphoton added thermal states, achieved through multiphoton measurements at one output port of the beam splitter (termed multiphoton catalysis) for thermal state input. We discuss the success probabilities of detection (the normalization factors). Furthermore, we investigate their nonclassical properties based on the nonclassical depth, photon number distribution, and photocount distribution. It is shown that the multiphoton catalysis presents a better nonclassical performance by controlling the thermal parameter, catalyzed photon number and the transmissivity of the beam splitter. In addition, the nonclassicality is further examined through the partial negativity of the Wigner function, which reveals that multiphoton catalysis operation can prepare highly nonclassical quantum states. These results indicate that the preparation of a non-Gaussian states may have potential applications in the realms of quantum information processing and quantum metrology.