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Experimental demonstration of a passive temperature stabilized quantum memory for storage of polarization qubits in a cold atomic ensemble

Thomas G. Akin, John F. Reintjes, Michał Piotrowicz, Adam T. Black, A. Kuzmich, Mark Bashkansky

Published May 13, 2019• 0 citations
Publisher

Abstract

Interferometric stability of polarization-entangled photons in quantum repeaters for long time intervals is an important capability for future scalable quantum networks linked over distances greater than hundreds of kilometers. A quantum memory node is a necessary component of the quantum repeater, where entanglement is prepared and swapped to extend entangled states from remote to distant nodes. Room temperature fluctuations can have significant effects on phase stability of the polarization states stored in the quantum memory. Although common-path stabilization in a quantum memory has been demonstrated, passive stabilization to room temperature variations has not been realized. Our approach to the quantum memory uses a single collective excitation encoded in two separate spatial modes in a cold ensemble of rubidium atoms. The two spatial modes are combined into a single path using the birefringence of two calcite crystals. However, normal lab temperature changes introduces a phase shift between the ordinary and extraordinary pathways on the order of 2π. We demonstrate passive temperature stabilization by alignment of the ordinary path in one crystal to the extraordinary path in the second crystal and vice versa. We show a phase stability on the order of ten hours by homodyne detection of classical light modes exiting the interferometer. We corroborate the phase stability of the quantum memory with a correlation measurement between polarization states of a signal photon generated at the formation of the collective atomic excitation and a retrieved idler photon during the destruction of the atomic excitation. We measure a Bell-CHSH parameter for both the unstable configuration and for the stable configuration. For an unstable calcite crystal configuration, we do not measure a violation of the Bell-CHSH inequality1 (S≤2) with S = 1.42 ± 0.087. For the stable calcite crystal configuration, we measure a violation of Bell-CHSH inequality (S>2) with S = 2.48±0.099.

DOI
10.1117/12.2518484

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Interferometric stability of polarization-entangled photons in quantum repeaters for long time intervals is an important capability for future scalable quantum networks linked over distances greater than hundreds of kilometers. A quantum memory node is a necessary component of the quantum repeater, where entanglement is prepared and swapped to extend entangled states from remote to distant nodes. Room temperature fluctuations can have significant effects on phase stability of the polarization states stored in the quantum memory. Although common-path stabilization in a quantum memory has been demonstrated, passive stabilization to room temperature variations has not been realized. Our approach to the quantum memory uses a single collective excitation encoded in two separate spatial modes in a cold ensemble of rubidium atoms. The two spatial modes are combined into a single path using the birefringence of two calcite crystals. However, normal lab temperature changes introduces a phase shift between the ordinary and extraordinary pathways on the order of 2π. We demonstrate passive temperature stabilization by alignment of the ordinary path in one crystal to the extraordinary path in the second crystal and vice versa. We show a phase stability on the order of ten hours by homodyne detection of classical light modes exiting the interferometer. We corroborate the phase stability of the quantum memory with a correlation measurement between polarization states of a signal photon generated at the formation of the collective atomic excitation and a retrieved idler photon during the destruction of the atomic excitation. We measure a Bell-CHSH parameter for both the unstable configuration and for the stable configuration. For an unstable calcite crystal configuration, we do not measure a violation of the Bell-CHSH inequality1 (S≤2) with S = 1.42 ± 0.087. For the stable calcite crystal configuration, we measure a violation of Bell-CHSH inequality (S>2) with S = 2.48±0.099.
First generation quantum repeater networks require independent quantum memories capable of storing and retrieving indistinguishable photons to perform quantum-interference-mediated high-repetition entanglement swapping operations. The ability to perform these coherent operations at room temperature is of prime importance in order to realize large scalable quantum networks. Here we address these significant challenges by observing Hong-Ou-Mandel (HOM) interference between indistinguishable photons carrying polarization qubits retrieved from two independent room-temperature quantum memories. Our elementary quantum network configuration includes: (i) two independent sources generating polarization-encoded qubits; (ii) two atomic-vapor dual-rail quantum memories; and (iii) a HOM interference node. We obtained interference visibilities after quantum memory retrieval of V=(41.9±2.0)%\rm \boldsymbol{V=(41.9\pm2.0)\%}V=(41.9±2.0)% for few-photon level inputs and V=(25.9±2.5)%\rm \boldsymbol{V=(25.9\pm2.5)\%}V=(25.9±2.5)% for single-photon level inputs. Our prototype network lays the groundwork for future large-scale memory-assisted quantum cryptography and distributed quantum networks.
Quantum memory is an essential building block for quantum communication and scalable linear quantum computation. Storing two-color entangled photons with one photon being at the telecommunication (telecom) wavelength while the other photon is compatible with quantum memory has great advantages toward the realization of the fiber-based long-distance quantum communication with the aid of quantum repeaters. Here, we report an experimental realization of storing a photon entangled with a telecom photon in polarization as an atomic spin wave in a cold atomic ensemble, thus establishing the entanglement between the telecom-band photon and the atomic-ensemble memory in a polarization degree of freedom. The reconstructed density matrix and the violation of the Clauser-Horne-Shimony-Holt inequality clearly show the preservation of quantum entanglement during storage. Our result is very promising for establishing a long-distance quantum network based on cold atomic ensembles.
First generation quantum repeater networks require independent quantum memories capable of storing and retrieving indistinguishable photons to perform quantum-interference-mediated high-repetition entanglement swapping operations. The ability to perform these coherent operations at room temperature is of prime importance in order to realize large scalable quantum networks. Here we address these significant challenges by observing Hong-Ou-Mandel (HOM) interference between indistinguishable photons carrying polarization qubits retrieved from two independent room-temperature quantum memories. Our elementary quantum network configuration includes: (i) two independent sources generating polarization-encoded qubits; (ii) two atomic-vapor dual-rail quantum memories; and (iii) a HOM interference node. We obtained interference visibilities after quantum memory retrieval of V=(41.9±2.0)%\rm \boldsymbol{V=(41.9\pm2.0)\%}V=(41.9±2.0)% for few-photon level inputs and V=(25.9±2.5)%\rm \boldsymbol{V=(25.9\pm2.5)\%}V=(25.9±2.5)% for single-photon level inputs. Our prototype network lays the groundwork for future large-scale memory-assisted quantum cryptography and distributed quantum networks.
Quantum memory capable of storage and retrieval of flying photons on demand is crucial for developing quantum information technologies. However, the devices needed for long-distance links are different from those envisioned for local processing. We present the first hybrid quantum memory-enabled network by demonstrating the interconnection and simultaneous operation of two types of quantum memory: an atomic ensemble-based memory and an all-optical Loop memory. Interfacing the quantum memories at room temperature, we observe a well-preserved quantum correlation and a violation of Cauchy-Schwarz inequality. Furthermore, we demonstrate the creation and storage of a fully-operable heralded photon chain state that can achieve memory-built-in combining, swapping, splitting, tuning, and chopping single photons in a chain temporally. Such a quantum network allows atomic excitations to be generated, stored, and converted to broadband photons, which are then transferred to the next node, stored, and faithfully retrieved, all at high speed and in a programmable fashion.
Abstract Quantum interfaces (QIs) that generate entanglement between photonic and spin-wave (atomic memory) qubits are basic building block for quantum repeaters. Realizing ensemble-based repeaters in practice requires quantum memory providing long lifetimes and multimode capacity. Significant progress has been achieved on these separate goals. The remaining challenge is to combine the two attributes into a single QI. Here, by establishing spatial multimode, magnetic-field-insensitive and long-wavelength spin-wave storage in laser-cooled atoms inside a phase-passively-stabilized polarization interferometer, we constructed a multiplexed QI that stores up to three long-lived spin-wave qubits. Using a feed-forward-controlled system, we demonstrated that a multiplexed QI gives rise to a 3-fold increase in the atom–photon (photon–photon) entanglement-generation probability compared with single-mode QIs. For our multiplexed QI, the measured Bell parameter is 2.51±0.01 combined with a memory lifetime of up to 1 ms. This work represents a key step forward in realizing fiber-based long-distance quantum communications.
Single photons are the best carriers of quantum information for long-distance transmission. Nevertheless, maximal achievable distance is limited by the exponential decay of photons as a function of link length. The protocol of quantum repeater provides a promising solution by replacing direction transmission with segmented entanglement distribution and entanglement connection via swapping. The quantum repeater necessitates a key element of quantum memory for making efficient interconnections. An atomic ensemble is very suitable for this purpose due to the collective enhanced interaction. Single photons are stored as collective excitations in an atomic ensemble. Thus a comprehensive study of the physics relating to collective excitations is crucially important for improving the quantum memory performance and its reachable applications in quantum repeater and quantum network. In this article, we review our experimental work on cold atomic ensembles in recent years, focusing on the coherent manipulation of collective excitations. We first briefly introduce the general concept of collective excitations and the preparation process through spontaneous Raman scattering, and we review our experimental work on extending the coherence time, such as suppressing motional dephasing by increasing the spin-wave wavelength, by confining atoms with a three-dimensional optical lattice. Afterwards, we discuss about the retrieval process of collective excitations and review our experiments on using a ring-cavity enhanced setup to improve the retrieval efficiency. The coherent qubit operation in a quantum memory is very useful for enabling new functionalities for a quantum network, in a subsequent section, we thus review our work on developing Raman-based coherent operations for single excitations. Afterwards, we mention our experiments on creating a pair of atom-photon entanglement by interfering two modes of a collective excitation. Improving the entanglement preparation efficiency is crucially important, and Rydberg-based interaction provides a promising solution. Our experimental work in this direction is also reviewed. Additionally, as an application in coherent manipulation with collective excitations, we show several experiments on using excitations in remote atomic memories and demonstrating basic functionality of quantum repeater and quantum network. In short, significant progress has been made in the coherent manipulation of single collective excitations in cold atomic ensembles, and further improvement will be accelerated by the Rydberg-enabled interactions; practical applications in quantum repeater and quantum network is foreseeable in the near future.