An accurate theoretical treatment of periodically driven quantum systems is crucial for various fields in the exact sciences, for instance Nuclear Magnetic Resonance (NMR) spectroscopy. Conventionally, either average Hamiltonian theory or Floquet theory is used to predict or describe experimental outcomes, such as the time evolution or the spectra yielding the information of the sample under study. A detailed analysis of the equivalence of these two approaches with an emphasis on applications in NMR will help to improve the theoretical understanding of NMR experiments.
In this work, we identify the Floquet-Magnus expansion as essential to prove the mathematical equivalence of Floquet theory and average Hamiltonian theory. We advocate a calculation scheme which is less prone to algebraic mistakes because explicit integration is avoided. On this basis, we provide the first four orders of both theories. We further examine their applicability to some experiments in NMR. As examples, we investigate the Bloch-Siegert shift and dipolar coupled spin systems under magic-angle spinning.
Based on our analysis, we recommend the use of the Floquet-Van Vleck approach including both the effective Hamiltonian and the kick operator. The consistent separation of secular and non-secular contributions appears to be especially advantageous for numerical robustness. Its accuracy is about three times better than the one provided by average Hamiltonian theory despite their formal equivalence.
Our findings provide important insights into the theoretical background of Floquet theory and average Hamiltonian theory. This includes the extent of their algebraic and perturbative equivalence, with an emphasis on how these findings are of relevance in the analysis of solid-state NMR experiments.
The realization of synthetic gauge fields has attracted a lot of attention recently in relation to periodically driven systems and the Floquet theory. In ultracold atom systems in optical lattices and photonic networks, this allows one to simulate exotic phases of matter such as quantum Hall phases, anomalous quantum Hall phases, and analogs of topological insulators. In this paper, we apply the Floquet theory to engineer anisotropic Haldane models on the honeycomb lattice and two-leg ladder systems. We show that these anisotropic Haldane models still possess a topologically nontrivial band structure associated with chiral edge modes. Focusing on (interacting) boson systems in
s-wave bands of the lattice, we show how to engineer through the Floquet theory, a quantum phase transition (QPT) between a uniform superfluid and a Bose-Einstein condensate analog of Fulde-Ferrell-Larkin-Ovchinnikov states, where bosons condense at nonzero wave vectors. We perform a Ginzburg-Landau analysis of the QPT on the graphene lattice, and compute observables such as chiral currents and the momentum distribution. The results are supported by exact diagonalization calculations and compared with those of the isotropic situation. The validity of high-frequency expansion in the Floquet theory is also tested using time-dependent simulations for various parameters of the model. Last, we show that the anisotropic choice for the effective vector potential allows a bosonization approach in equivalent ladder (strip) geometries.