Starting with the first experimental generation of a Greenberger-Horne-Zeilinger entangled state in three dimensions we show how to describe photonic quantum experiments using graph theory. This novel link promises exciting new applications ranging from multi-photon high-dimensionally entangled states to special purpose quantum simulation.
Starting with the first experimental generation of a Greenberger-Horne-Zeilinger entangled state in three dimensions we show how to describe photonic quantum experiments using graph theory. This novel link promises exciting new applications ranging from multi-photon high-dimensionally entangled states to special purpose quantum simulation.
Quantum entanglement plays an important role in quantum information processes, such as quantum computation and quantum communication. Experiments in laboratories are unquestionably crucial to increase our understanding of quantum systems and inspire new insights into future applications. However, there are no general recipes for the creation of arbitrary quantum states with many particles entangled in high dimensions. Here we exploit a recent connection between quantum experiments and graph theory and answer this question for a plethora of classes of entangled states. We find experimental setups for Greenberger-Horne-Zeilinger states, W states, general Dicke states, and asymmetrically high-dimensional multipartite entangled states. This result sheds light on the producibility of arbitrary quantum states using photonic technology with probabilistic pair sources and allows us to understand the underlying technological and fundamental properties of entanglement.
Quantum nonlocality gives us deeper insight into quantum physics. In addition, quantum nonlocality has been further recognized as an essential resource for device-independent quantum information processing in recent years. Most experiments of nonlocality are performed using a photonic system. However, until now, photonic experiments of nonlocality have involved at most four photons. Here, for the first time, we experimentally demonstrate the six-photon quantum nonlocality in an all-versus-nothing manner based on a high-fidelity (88.4%) six-photon Greenberger-Horne-Zeilinger state. Our experiment pushes multiphoton nonlocality studies forward to the six-photon region and might provide a larger photonic system for device-independent quantum information protocols.
Greenberger-Horne-Zeilinger (GHZ) states are multipartite entangled quantum states that play a central role in quantum information theory, with applications in quantum communication, cryptography, and distributed quantum computing. A major experimental goal is to create high-dimensional GHZ states using multiple entangled parties. Krenn, Gu and Zeilinger discovered a surprising bridge between these quantum-optical experiments and graph theory: certain photonic experiments can be represented by edge-coloured, edge-weighted graphs, and the dimension of the produced GHZ state equals the number of feasible monochromatic inherited vertex colourings. This led Krenn and Gu to conjecture that every GHZ graph with more than four vertices has dimension at most 2. A counterexample would give a new high-dimensional multipartite GHZ construction, while a proof would clarify fundamental resource limitations in quantum optics. It is known that the conjecture holds for graphs of vertex connectivity at most 2 [MFCS 2024], and that simple GHZ graphs with n>4 vertices have dimension less than n/2 [Quantum 2024]. However, no general upper bound depending only on vertex connectivity was known. We prove that every simple connected GHZ graph G with at least four vertices has dimension at most 2κ(G)−1+(2κ(G)), where κ(G) is the vertex connectivity of G. We also prove new bounds in terms of edge connectivity and maximum degree.
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Multi-party quantum steering is an important concept in quantum information theory and quantum mechanics, typically related to quantum entanglement and quantum nonlocality. It enables precise manipulation of large quantum systems, which is essential for large-scale quantum computing, simulations, and quantum communication. Recently, a quantum steering certification for any three-qubit generalized Greenberger-Horne-Zeilinger (GGHZ) states based on the fine-grained steering inequality was proved [Quantum Studies: Mathematics and Foundations, 2022, 9(2): 175-198]. Here we provide an experimental proposal to prepare the GGHZ states in photon system. The measurement observalbes in each party can be realized by different polarization optical elements. By choosing the angles of the waveplates, our experiment proposal can observe the maximum quantum violation for any three-qubit GGHZ states. Our proposal can be easily extended to high-dimensional qubits and multi-photon GHZ states, which provides a method to study the complex multi-party quantum protocols.