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Advances in Optics and Photonics

Overcoming the diffraction limit by multi-photon interference: a tutorial

Joachim Stohr

Published Mar 28, 2019• 39 citations
Publisher

Abstract

The nature of light, extending from the optical to the x-ray regime, is reviewed from a diffraction point of view by comparing field-based statistical optics and photon-based quantum optics approaches. The topic is introduced by comparing historical diffraction concepts based on wave interference, Dirac’s notion of photon self-interference, Feynman’s interference of space–time photon probability amplitudes, and Glauber’s formulation of coherence functions based on photon detection. The concepts are elucidated by a review of how the semiclassical combination of the disparate photon and wave concepts have been used to describe light creation, diffraction, and detection. The origin of the fundamental diffraction limit is then discussed in both wave and photon pictures. By use of Feynman’s concept of probability amplitudes associated with independent photons, we show that quantum electrodynamics, the complete theory of light, reduces in lowest order to the conventional wave formalism of diffraction. As an introduction to multi-photon effects, we then review fundamental one- and two-photon experiments and detection schemes, in particular the seminal Hanbury Brown–Twiss experiment. The formal discourse of the paper starts with a treatment of first-order coherence theory. In first order, the statistical optics and quantum optics formulations of coherence are shown to be equivalent. This is elucidated by a discussion of Zernike’s powerful theorem of partial coherence propagation, a cornerstone of statistical optics, followed by its quantum derivation based on the interference of single-photon probability amplitudes. The treatment is then extended to second-order coherence theory, where the equivalence of wave and particle descriptions is shown to break down. This is illustrated by considering two photons whose space–time probability amplitudes are correlated through nonlinear birth processes, resulting in entanglement or cloning. In both cases, the two-photon diffraction patterns are shown to exhibit resolution below the conventional diffraction limit, defined by the one-photon diffraction patterns. The origin of the reduction is shown to arise from the interference of two-photon probability amplitudes. By comparing first- and second-order diffraction, it is shown that the conventional first-order concept of partial coherence with its limits of chaoticity and first-order coherence has the second-order analogue of partial entanglement, with its limits corresponding to two entangled photons (“entangled biphotons”) and two cloned photons (“cloned biphotons”), the latter being second-order coherent. The concept of cloned biphotons is extended to the case of $n$ cloned photons, resulting in a $1/n$ reduction of the diffraction limit. In the limit of $n$th-order collective state are shown to propagate on particle like trajectories, reproducing the 0th-order ray-optics picture. These results are discussed in terms of the linearity of quantum mechanics and Heisenberg’s space–momentum uncertainty principle. Finally, a general concept of coherence based on photon density is developed that in first order is equivalent to the conventional wave-based picture.

DOI
10.1364/aop.11.000215

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The nature of light, extending from the optical to the x-ray regime, is reviewed from a diffraction point of view by comparing field-based statistical optics and photon-based quantum optics approaches. The topic is introduced by comparing historical diffraction concepts based on wave interference, Dirac’s notion of photon self-interference, Feynman’s interference of space–time photon probability amplitudes, and Glauber’s formulation of coherence functions based on photon detection. The concepts are elucidated by a review of how the semiclassical combination of the disparate photon and wave concepts have been used to describe light creation, diffraction, and detection. The origin of the fundamental diffraction limit is then discussed in both wave and photon pictures. By use of Feynman’s concept of probability amplitudes associated with independent photons, we show that quantum electrodynamics, the complete theory of light, reduces in lowest order to the conventional wave formalism of diffraction. As an introduction to multi-photon effects, we then review fundamental one- and two-photon experiments and detection schemes, in particular the seminal Hanbury Brown–Twiss experiment. The formal discourse of the paper starts with a treatment of first-order coherence theory. In first order, the statistical optics and quantum optics formulations of coherence are shown to be equivalent. This is elucidated by a discussion of Zernike’s powerful theorem of partial coherence propagation, a cornerstone of statistical optics, followed by its quantum derivation based on the interference of single-photon probability amplitudes. The treatment is then extended to second-order coherence theory, where the equivalence of wave and particle descriptions is shown to break down. This is illustrated by considering two photons whose space–time probability amplitudes are correlated through nonlinear birth processes, resulting in entanglement or cloning. In both cases, the two-photon diffraction patterns are shown to exhibit resolution below the conventional diffraction limit, defined by the one-photon diffraction patterns. The origin of the reduction is shown to arise from the interference of two-photon probability amplitudes. By comparing first- and second-order diffraction, it is shown that the conventional first-order concept of partial coherence with its limits of chaoticity and first-order coherence has the second-order analogue of partial entanglement, with its limits corresponding to two entangled photons (“entangled biphotons”) and two cloned photons (“cloned biphotons”), the latter being second-order coherent. The concept of cloned biphotons is extended to the case of nnn cloned photons, resulting in a 1/n1/n1/n reduction of the diffraction limit. In the limit of nnnth-order collective state are shown to propagate on particle like trajectories, reproducing the 0th-order ray-optics picture. These results are discussed in terms of the linearity of quantum mechanics and Heisenberg’s space–momentum uncertainty principle. Finally, a general concept of coherence based on photon density is developed that in first order is equivalent to the conventional wave-based picture.
In this thesis we discuss an extension of the historical Hanbury Brown and Twiss experiment and investigate spatial intensity correlations of higher-orders in the radiation field of statistically independent light sources. The light sources can be non-classical like single-photon emitters or classical, obeying thermal or coherent statistics. Although the light sources are assumed to emit the photons in an incoherent manner, we find spatial photon correlations in the far field which can be explained by the quantum mechanical concept of multi-photon interferences. We demonstrate that spatial correlation measurements between indistinguishable photons based on linear optical detection techniques can be used to overcome the resolution limit of classical optics (Abbe/Rayleigh limit) and also to manipulate the spatial radiation characteristic of the light sources. Both remarkable properties of higher-order intensity correlations have been experimentally verified using statistically independent pseudothermal light sources. Due to the fact that the reported correlation measurements require neither special quantum tailoring of light nor N-photon absorbing media, they are of particular interest for the field of quantum imaging and quantum information processing. The thesis is divided into three main parts: In the first part (Chapter 2 and 3) we introduce a quantum path formalism which allows to describe multi-photon interferences arising in both classical and nonclassical light fields. This quantum path approach explains the origin of the underlying interference mechanism of the higher-order spatial intensity correlation functions in a transparent and simple manner. Moreover, it enables us to compare the multi-photon interferences obtained by nonclassical single-photon emitters with those generated by classical light sources. In the course of this discussion it appears that Dirac's famous statement “Each photon interferes only with itself. Interference between two different photons never occurs.” should better read “A multi-photon state of independent photons only interferes with itself. Interference between different multi-photon states never occurs.” This general statement summarizes the physics behind all multi-photon interference phenomena investigated in this thesis. In the second part of the thesis (Chapter 4) we investigate particular multi-photon interference measurements of independent light sources in the context of quantum imaging. We demonstrate that the Nth-order spatial intensity correlation functions display at specific ‘magic’ detector positions the ability to filter sub-wavelength information out of the light fields arising from N incoherently radiating light sources. These multi-photon interference patterns achieve a higher resolution for N>2 than the classical Abbe/Rayleigh limit for imaging the light source. In case of N single-photon emitters we theoretically show that the super-resolving interference patterns obtained for the ‘magic’ detector positions are identical to the ones generated by NOON states with N-1 photons. Quite unexpected, the same is true for N thermal light sources, except for a reduced visibility. Experimental results with up to eight independent thermal light sources confirm this approach to improve the spatial resolution in imaging. In the last part of this thesis (Chapter 5) we finally demonstrate that multi-photon detections can lead to a strong angular focussing of incoherent photons emitted again by either uncorrelated single-photon sources or statistically independent classical light sources. For this effect the sources can be far away from each other and do not interact. The mth-order intensity correlation measurement causes source correlations which produce a heralded peaked emission pattern for the initially uncorrelated light sources. In particular, we show that if m-1 photons have been detected in a particular direction, the conditional probability to detect the mth photon in the same direction can be as high as 100 %. Owing to the great flexibility of detector positions for the correlation measurement, a wide variety of additional detection schemes exists which produces similar directional photon emission patterns. This theoretically predicted measurement-induced focussing was experimentally confirmed with up to eight pseudothermal light sources for three particular detection schemes.
Today, the nature of light is accounted for by one of the jewels of physics, quantum electrodynamics (QED), the fundamental theory of light and matter. Yet owing to its infinite complexity, scientists still debate how its central concept, the photon, can be reconciled with the perceived existence of light waves, emerging 200 years ago in the wake of Young's double slit diffraction experiment. Ever since, the phenomenon of diffraction has been viewed to embody the wave nature of light, leading to the schizophrenic wave-particle duality. The latter does not exist in QED which is photon based without the existence of waves. Here we introduce the new paradigm that diffraction images directly reflect the fundamental quantum states of light. This is revealed by analysis of the evolution of modern versions of Young's experiment performed with differently modified laser light and photon-based detection. In conventional quantum mechanics, corresponding to first order QED, the fundamental photon nature of light remains hidden since different quantum states produce only two basic types of diffraction patterns that may also be explained by coherent and incoherent wave superposition. The true photon based substructure of light is shown to clearly emerge through characteristic diffraction images in second order QED. The degeneracy of the first order images is lifted, the wave-particle equivalence breaks down, and the patterns directly reveal the true quantum substructure of light. This allows the replacement of the conventional concept of wave coherence by a precise order-dependent degree of coherence that quantifies the interference and diffraction behavior of all quantum states of light.
Electromagnetic Wave Theory and Measurement of Light Electromagnetic Wave Theory of Light Classical Superposition Measurement of Light Intensity of Light: Expectation and Fluctuation Measurement of Intensity: Ensemble Average and Time Average Coherence Property of Light-The State of the Radiation Coherence Property of Light Temporal Coherence Spatial Coherence Diffraction and Propagation Diffraction Field Propagation Optical Imaging A Classic Imaging System Fourier Transform via a Lens First-Order Coherence of Light First-Order Temporal Coherence First-Order Spatial Coherence Second-Order Coherence of Light Second-Order Coherence of Coherent Light Second-Order Correlation of Chaotic-Thermal Radiation and the HBT Interferometer The Physical Cause of the HBT Phenomenon Near-Field Second-Order Spatial Coherence of Thermal Light Nth-Order Coherence of Light Nth-Order Near-Field Spatial Coherence of Thermal Light Homodyne Detection and Heterodyne Detection of Light Optical Homodyne and Heterodyne Detection Balanced Homodyne and Heterodyne Detection Balanced Homodyne Detection of Independent and Coupled Thermal Fields Quantum Theory of Light: Field Quantization and Measurement The Experimental Foundation-Part I: Blackbody Radiation The Experimental Foundation-Part II: Photoelectric Effect The Light Quantum and the Field Quantization Photon Number State of Radiation Field Coherent State of Radiation Field Density Operator and Density Matrix Composite System and Two-Photon State of Radiation Field A Simple Model of Incoherent and Coherent Radiation Source Pure State and Mixed State Product State, Entangled State, and Mixed State of Photon Pairs Time-Dependent Perturbation Theory Measurement of Light: Photon Counting Measurement of Light: Joint Detection of Photons Field Propagation in Space-Time Quantum Theory of Optical Coherence Quantum Degree of First-Order Coherence Photon and Effective Wavefunction Measurement of the First-Order Coherence or Correlation Quantum Degree of Second-Order Coherence Two-Photon Interference vs. Statistical Correlation of Intensity Fluctuations Second-Order Spatial Correlation of Thermal Light Photon Counting and Measurement of G(2) Quantum Entanglement EPR Experiment and EPR State Product State, Entangled State, and Classically Correlated State Entangled States in Spin Variables Entangled Biphoton State EPR Correlation of Entangled Biphoton System Subsystem in an Entangled Two-Photon State Biphoton in Dispersive Media Quantum Imaging Biphoton Imaging Ghost Imaging Ghost Imaging and Uncertainty Relation Thermal Light Ghost Imaging Classical Simulation of Ghost Imaging Turbulence-Free Ghost Imaging Two-Photon Interferometry I: Biphoton Interference Is Two-Photon Interference the Interference of Two Photons? Two-Photon Interference with Orthogonal Polarization Franson Interferometer Two-Photon Ghost Interference Delayed Choice Quantum Eraser Two-Photon Interferometry II: Quantum Interference of Chaotic Light Two-Photon Young's Interference Two-Photon Anticorrelation with Incoherent Chaotic Light Two-Photon Interference with Incoherent Orthogonal Polarized Chaotic Light Bell's Theorem and Bell's Inequality Measurement Hidden Variable Theory and Quantum Calculation for the Measurement of Spin 1/2 Bohm State Bell's Theorem and Bell's Inequality Bell States Bell State Preparation
Optical interference is regarded as a classical phenomenon and is usually completely described in classical terms, in which optical fields are represented by classical waves. Does it mean that optical interference, which is fundamentally ascribable to the phenomenon of a superposition of wave amplitudes, cannot be applied to test quantum phenomena? The superposition principle is at the heart of quantum physics and one could expect that it should distinguish the quantum nature of light from thewave nature. Our experience based on extensive theoretical analysis and experimental observations shows that classical and quantum theories of optical interference readily explain the presence of an interference pattern resulting from the first-order coherence. However, there are interference effects involving the higher order (second-order) coherence that distinguish the quantum (photon) nature of light from the wave nature. Quantum interference has recently returned to prominence because of its utility in manipulating spontaneous emission and other radiative properties of atomic systems. In this chapter, we present elementary concepts and definitions of both the classical and quantum theory of optical interference and discuss similarities and differences between these two approaches [80].
When a parallel beam of light illuminates an aperture, the uncertainty principles require associating probability amplitude to a photon at each point of the aperture. Superposition of the amplitudes at the observation point behind the aperture, determines the probability that the photon strikes the point. In this paper, we show that this "photon approach" explains several optical concepts. The approach is applied to study the diffraction from a single slit, double slit, and transmission phase step. Then, we apply it to explain the diffraction from a bi-prism and a Michelson's interferometer, and show that the photon approach to the appearance of the interference fringes is more reasonable than the wave approach. We deduce the coherence behavior of light from the uncertainty principles, and finally, we use the photon approach to extract the ray optics laws and image formation formulae.
Imaging is the estimation of the spatial distribution of a physical object by measuring the optical radiation it emits, or by making use of an optical wave that interacts with the object, via reflection or transmission, for example, before being measured by a detector. The resolution of an imaging system is limited by the inability to localize the optical field at points of the object. Under otherwise ideal conditions, resolution is limited by diffraction. The sensitivity of an imaging system is limited by the uncertainty in the measurement. Under ideal conditions, this is determined by photon noise, which depends on the statistical fluctuations of the light. In conventional imaging systems, an extended detector, such as a CCD camera or an array detector, measures the spatial distribution of the optical intensity, which is proportional to the photon flux density. In interferometric systems, the spatial distribution of the optical field is inferred from measurements of the optical intensity. With the emergence of coherence theory, imaging systems based on measurements of the second-order coherence function at pairs of points in the detection plane were developed. An example is the imaging of an incoherent object based on the van Cittert-Zernike theorem. Imaging systems based on measurement of intensity correlation, or the photon coincidence rate, at pairs of points, were developed in the 1960s. A classic example of the photon-correlation imaging of an object emitting thermal light is stellar imaging using a Hanbury-Brown-Twiss intensity-correlation interferometer. More recently, two-photon light, which may be generated via spontaneous parametric downconversion in a second-order nonlinear optical crystal, has been used for imaging. This type of two-photon (or biphoton) imaging, which has come to be called quantum imaging, is also based on the measurement of photon coincidence by the use of photon-counting array detectors or by scanning two photon-counting detectors at pairs of points. To compare the resolution and sensitivity of imaging systems based on the aforementioned types of measurements, it is necessary to derive expressions for the measured quantities in terms of the object distribution. The point-spread functions based on such expressions can be used to assess the resolution. One measure of the sensitivity of the imaging process is the signal-to-noise ratio (SNR) of the measured variables. The statistical nature of the light source must be known in order to determine the SNR. The purpose of this chapter is to compare the resolution and sensitivity of photon-correlation imaging systems that make use of thermal light and two-photon light. We will henceforth refer to these two imaging modalities as classical and quantum photon-correlation imaging, or simply classical and quantum imaging, respectively. Clearly, light in other quantum states can also be used for imaging.