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Complex Light and Optical Forces

Manipulation of structured light in an atom-clad optical nanofiber (Conference Presentation)

Thomas Nieddu, Tridib Ray, Simon Peter Mekhail, Jinjin Du, Síle Nic Chormaic

Published Mar 8, 2019• 0 citations
Publisher

Abstract

Optical nanofibers (ONF) have been proved useful tools to probe cold atomic systems. Due to the intense evanescent field at their waist, ONFs have been used to probe or even trap atoms. However, very little experimental work has been done on exploiting the higher order modes (HOM) of such devices. The HOMs feature inhomogeneous polarization distributions around the ONF’s waist and can lead to the guiding of light carrying orbital angular momentum (OAM), via selective excitation of modes. In this work, we have experimentally studied the interaction between an ensemble of cold rubidium atoms and the HOMs of an ONF. The ONF, tailored to allow propagation of the first 6 guided modes at 780 nm, is embedded in a cold atomic ensemble and its modes are selectively excited by coupling vector beams from free-space. Using modal decomposition at the output of the ONF, we can calculate the transfer matrix of the system. This information, when combined with the amplitude extinction resulting from the scattering of the guided light by atoms surrounding the waist, allows us to non-destructively infer the modal excitation at the waist of the ONF. We further investigate the effect of temperature-induced strain on the modal decomposition at the waist and fiber output pigtail. Our results allow us to encode more than one quantum of information on the total angular momentum of a single guided photon. The inhomogeneous polarization distributions featured by the HOMs also offer a new tool to study chiral quantum systems.

DOI
10.1117/12.2509267

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Optical nanofibers (ONF) have been proved useful tools to probe cold atomic systems. Due to the intense evanescent field at their waist, ONFs have been used to probe or even trap atoms. However, very little experimental work has been done on exploiting the higher order modes (HOM) of such devices. The HOMs feature inhomogeneous polarization distributions around the ONF’s waist and can lead to the guiding of light carrying orbital angular momentum (OAM), via selective excitation of modes. In this work, we have experimentally studied the interaction between an ensemble of cold rubidium atoms and the HOMs of an ONF. The ONF, tailored to allow propagation of the first 6 guided modes at 780 nm, is embedded in a cold atomic ensemble and its modes are selectively excited by coupling vector beams from free-space. Using modal decomposition at the output of the ONF, we can calculate the transfer matrix of the system. This information, when combined with the amplitude extinction resulting from the scattering of the guided light by atoms surrounding the waist, allows us to non-destructively infer the modal excitation at the waist of the ONF. We further investigate the effect of temperature-induced strain on the modal decomposition at the waist and fiber output pigtail. Our results allow us to encode more than one quantum of information on the total angular momentum of a single guided photon. The inhomogeneous polarization distributions featured by the HOMs also offer a new tool to study chiral quantum systems.
Optical nanofibres (ONFs) are very thin optical waveguides with sub-wavelength diameters. ONFs have very high evanescent fields and the guided light is confined strongly in the transverse direction. These fibres can be used to achieve strong light-matter interactions. Atoms around the waist of an ONF can be probed by collecting the atomic fluorescence coupling or by measuring the transmission (or the polarisation) of the probe beam sent through it. This thesis presents experiments using ONFs for probing and manipulating laser-cooled 87Rb atoms. As an initial experiment, a single mode ONF was integrated into a magneto-optical trap (MOT) and used for measuring the characteristics of the MOT, such as the loading time and the average temperature of the atom cloud. The effect of a near-resonant probe beam on the local temperature of the cold atoms has been studied. Next, the ONF was used for manipulating the atoms in the evanescent fields region in order to generate nonlinear optical effects. Four-wave mixing, ac Stark effect (Autler-Townes splitting) and electromagnetically induced transparency have been observed at unprecedented ultralow power levels. In another experiment, a few-mode ONF, supporting only the fundamental mode and the first higher order mode group, has been used for studying cold atoms. A higher pumping rate of the atomic fluorescence into the higher order fibreguided modes and more interactions with the surrounding atoms for higher order mode evanescent light, when compared to signals for the fundamental mode, have been identified. The results obtained in the thesis are particularly for a fundamental understanding of light-atom interactions when atoms are near a dielectric surface and also for the development of fibre-based quantum information technologies. Atoms coupled to ONFs could be used for preparing intrinsically fibre-coupled quantum nodes for quantum computing and the studies presented here are significant for a detailed understanding of such a system.
We describe advancements towards coupling superconducting qubits to neutral atoms. To produce a measurably large coupling, the atoms will need to be on the order of a few micrometers away from the qubit. A consequence of combining superconducting qubits and atoms is addressing their operational constraints, such as the deleterious light effects on superconducting systems and the magnetic field sensitivity of superconducting qubits. Our group proposes the use of optical-nanofiber-based optical dipole traps to confine atoms near the superconductor. Optical nanofibers (ONFs) have high-intensity evanescent waves that require less power than equivalent standard dipole traps. This thesis focuses on the fabrication and analysis of the behavior of ONFs. First we present the construction of the pulling apparatus. We outline the necessary steps for a typical pull, detailing the cleaning and alignment process. Then we examine the quality of the fibers by measuring their transmission and comparing our results to other reported measurements, demonstrating a two-order of magnitude decrease in loss. Next we present the modal evolution in ONFs using simulations and spectrogram analysis. We identify crucial elements to improve the transmission and demonstrate understanding of the modal dynamics during the pull. Then we study higher-order modes (HOMs) with ONFs using the first excited TE01, TM01, and HE21 modes. We demonstrate transmissions greater than 97% for 780 nm light when we launch the first excited LP11 family of modes through fibers with a 350 nm waist. This setup enables us to launch these three modes with high purity at the output, where less than 1% of the light is coupled to the fundamental mode. We then focus on the identification of modes on the ONF waist. First we use Rayleigh scattering to identify the modal content of an ONF. Bulk optics can convert the modes in the ONF, and we observe the controllable conversion of superpositions of modes. Finally, we use an evanescently-coupled tapered optical fiber probe that allows for the identification of the fundamental mode beating with HOMs and compare the results to simulations.
Tapered optical fiber with subwavelength diameter waist, an optical nanofiber, provides a unique and versatile platform for manipulating atoms and photons. In the guided modes of the nanofibers, the optical field can be tightly confined in the transverse direction while enabling strong interaction with the surrounding medium in the evanescent region. Combining laser-cooled atoms with nanofibers has enabled surprising quantum optics experiments, e.g. the efficient channeling of emission from single atoms into the fiber-guided modes, spectroscopy of near-surface atoms, high optical depth with an array of atoms optically trapped around the nanofiber, atomic memories and Bragg reflectors for fiber-guided photons, chiral light-matter interaction etc. In addition, using moderate longitudinal confinement in nanofiber cavities has enabled strong coupling between a single atom and fiber-guided photons. In this article, I review some of the key experimental demonstrations on the “atom+nanofiber” platform.
The development of optical nanofibers (ONF) and the study and control of their optical properties when coupling atoms to their electromagnetic modes has opened new possibilities for their use in quantum optics and quantum information science. These ONFs offer tight optical mode confinement (less than the wavelength of light) and diffraction-free propagation. The small cross section of the transverse field allows probing of linear and non-linear spectroscopic features of atoms with exquisitely low power. The cooperativity -- the figure of merit in many quantum optics and quantum information systems -- tends to be large even for a single atom in the mode of an ONF, as it is proportional to the ratio of the atomic cross section to the electromagnetic mode cross section. ONFs offer a natural bus for information and for inter-atomic coupling through the tightly-confined modes, which opens the possibility of one-dimensional many-body physics and interesting quantum interconnection applications. The presence of the ONF modifies the vacuum field, affecting the spontaneous emission rates of atoms in its vicinity. The high gradients in the radial intensity naturally provide the potential for trapping atoms around the ONF, allowing the creation of one-dimensional arrays of atoms. The same radial gradient in the transverse direction of the field is responsible for the existence of a large longitudinal component that introduces the possibility of spin-orbit coupling of the light and the atom, enabling the exploration of chiral quantum optics.
We built a new experiment using cold atoms interacting with the light guided by an optical nanofiber. We first developed a nanofiber manufacturing bench. By heating and stretching a commercial optical fiber, a silica cylinder of 400 nm diameter is obtained. The light guided in these nanofibers is strongly focused over the whole length and exhibits strong evanescent fields. We then prepared a vacuum chamber and the laser system necessary for the manipulation of cold atoms. After inserting a nanofiber amid a cloud of cold atoms, we observed the phenomenon of slow light under the conditions of electromagnetically induced transparency: the light guided by the fiber is slowed down to a speed 3000 times smaller than its usual speed. We also stored the light guided by an optical fiber. After several microseconds, the information stored as a collective atomic excitation could be retrieved in the fiber. We have shown that this optical memory works for light pulses containing less than one photon on average. This system may therefore be used as a quantum memory, an essential tool for future quantum communication networks. Finally, we trapped atoms in an array in the vicinity of the nanofiber thanks to the light guided by the latter. Compared to our first set of experiments, the resulting cloud has a longer lifetime (25 ms) and interacts more strongly with the guided light (OD ~ 100). This new system should allow to efficiently implement other quantum optics protocols, such as the generation of single photons, or the entanglement of two remote atomic ensembles.
Optical nanofibres are used to confine light to sub-wavelength regions and are very promising tools for the development of optical fibre-based quantum networks using cold, neutral atoms. To date, experimental studies on atoms near nanofibres have focussed on fundamental fibre mode interactions. In this work, we demonstrate the integration of a few-mode optical nanofibre into a magneto-optical trap for 87 Rb atoms. The nanofibre, with a waist diameter of ∼700 nm, supports both the fundamental and first group of higher order modes (HOMs) and is used for atomic fluorescence and absorption studies. In general, light propagating in higher order fibre modes has a greater evanescent field extension around the waist in comparison with the fundamental mode. By exploiting this behaviour, we demonstrate that the detected signal of fluorescent photons emitted from a cloud of cold atoms centred at the nanofibre waist is larger if HOMs are also included. In particular, the signal from HOMs appears to be about six times larger than that obtained for the fundamental mode. Absorption of on-resonance, HOM probe light by the laser-cooled atoms is also observed. These advances should facilitate the realization of atom trapping schemes based on HOM interference.