Quantum metrology of solid-state single-photon sources using photon-number-resolving detectors
Martin von Helversen, Jonas Böhm, Marco Schmidt, Manuel Gschrey, Jan-Hindrik Schulze, A. Strittmatter, Sven Rodt, J. Beyer, Tobias Heindel, Stephan Reitzenstein
Quantum-light sources based on semiconductor quantum dots (QDs) are promising candidates for many applications in quantum photonics and quantum communication. Important emission characteristics of such emitters, namely the single-photon purity and photon indistinguishability, are usually assessed via time-correlated measurements using standard 'click' detectors in Hanbury Brown and Twiss or Hong-Ou-Mandel (HOM-) type configurations. In this work, we employ a state-of-the-art photon-number-resolving (PNR) detection system based on superconducting transition-edge sensors (TESs) to directly access the photon-number distribution of deterministically fabricated solid-state single-photon sources. Offering quantum efficiencies close to unity and high energy resolution, our TES-based two-channel detector system allows us to analyse the quantum optical properties of a QD-based non-classical light source. In particular, it enables the direct observation of the two-particle Fock-state resulting from interference of quantum mechanically indistinguishable photons in HOM-experiments. Additionally, comparative measurements reveal excellent quantitative agreement of the photon-indistinguishabilities obtained with PNR ((90 ± 7)%) and standard click ((90 ± 5)%) detectors. Our work thus demonstrates that TES-based detectors are perfectly suitable for the quantum metrology of non-classical light sources and higlights appealing prospects for the efficient implementation of quantum information tasks based on multi-photon states.
Quantum-light sources based on semiconductor quantum dots (QDs) are promising candidates for many applications in quantum photonics and quantum communication. Important emission characteristics of such emitters, namely the single-photon purity and photon indistinguishability, are usually assessed via time-correlated measurements using standard 'click' detectors in Hanbury Brown and Twiss or Hong-Ou-Mandel (HOM-) type configurations. In this work, we employ a state-of-the-art photon-number-resolving (PNR) detection system based on superconducting transition-edge sensors (TESs) to directly access the photon-number distribution of deterministically fabricated solid-state single-photon sources. Offering quantum efficiencies close to unity and high energy resolution, our TES-based two-channel detector system allows us to analyse the quantum optical properties of a QD-based non-classical light source. In particular, it enables the direct observation of the two-particle Fock-state resulting from interference of quantum mechanically indistinguishable photons in HOM-experiments. Additionally, comparative measurements reveal excellent quantitative agreement of the photon-indistinguishabilities obtained with PNR ((90 ± 7)%) and standard click ((90 ± 5)%) detectors. Our work thus demonstrates that TES-based detectors are perfectly suitable for the quantum metrology of non-classical light sources and higlights appealing prospects for the efficient implementation of quantum information tasks based on multi-photon states.
Light sources for applications in quantum information, quantum-enhanced sensing and quantum metrology are attracting increasing scientific interest. To gain inside into the underlying physical processes of quantum light generation, efficient photon detectors and experimental techniques are required to access the photon statistics. In this work, we employ photon-number-resolving (PNR) detectors based on superconducting transition-edge sensors (TESs) for the metrology of photonic microstructures with semiconductor quantum dots (QDs) as emitters. For the PNR analysis, we developed a state of the art PNR detection system based on fiber-coupled superconducting TESs. Our stand-alone system comprises six tungsten TESs, read out by six 2-stage-SQUID current sensors, and operated in a compact detector unit integrated into an adiabatic demagnetization refrigerator. This PNR detection system enables us to directly access the photon statistics of the light field emitted by our photonic microstructures. In this contribution, we focus on the PNR study of deterministically fabricated quantum light sources emitting single indistinguishable photons as well as twin-photon states. Additionally, we present a PNR-analysis of electrically pumped QD micropillar lasers exhibiting a peculiar bimodal behavior. Employing TESs our work provides direct insight into the complex emission characteristics of QD- based light sources. We anticipate, that TES-based PNR detectors, will be a viable tool for implementations of photonic quantum information processing relying on multi-photon states.
Quantum photonics benefits from the scientific advances in the development of quantum light sources. To gain inside into the underlying physical processes of light generation, we use photon-number-resolving (PNR) transition edge sensors (TESs), which are able to directly access the photon-number distribution of nanophotonic devices. We present results on the transition from thermal to coherent emission of two different classes of microlasers: electrically driven bimodal quantum dot micropillar lasers and exciton polariton lasers. Furthermore, the photon number distribution of deterministically fabricated quantum dot based single-photon sources is investigated to explore the single-photon purity and indistinguishability of photons emitted by these sources.
As single-photon sources become more mature and are used more often in quantum information, communications and measurement applications, their characterization becomes more important. Single-photon-like light is often characterized by its brightness, and two quantum properties: the single-photon composition and the photon indistinguishability. While it is desirable to obtain these quantities from a single measurement, currently two or more measurements are required. Here, we simultaneously determine the brightness, the single photon purity, the indistinguishability, and the statistical distribution of Fock states to third order for a quantum light source. The measurement uses a pair of two-photon (n = 2) number-resolving detectors. n > 2 number-resolving detectors provide no additional advantage in the single-photon characterization. The new method extracts more information per experimental trial than a conventional measurement for all input states, and is particularly more e cient for statistical mixtures of photon states. Thus, using this n=2, number- resolving detector scheme will provide advantages in a variety of quantum optics measurements and systems.
Strong interests on optical quantum based metrology, quantum information and particularly in quantum cryptography are continuously growing. The main limitations to the developments in these fields are due to non-ideal devices: both single photon sources and single photon detectors. In these field of applications, detectors require to be able to resolve the number of photons in a light pulse. Presently state of the art indicates that classical semiconductor light detectors (i.e. avalanche photodiode or single photon avalanche diode) are not able to discriminate the number of photon arriving at the same time. In the meanwhile, superconducting devices have shown the possibility to resolve single photon pulses. One of the most promising superconducting detectors is the Transition-Edge Sensor (TES): a microcalorimeter that takes advantage of the sharp transition (few millikelvin) from the superconducting to the normal phase; for this reason it is sometimes called Superconductive Phase Thermometer (SPT). In the ultraviolet (UV) to infrared (IR) wavelength range, the photons are absorbed directly by the superconductive thin film and the absorbed energy induces an increase of the TES resistance. Thanks to the applied bias voltage, which maintains the device in the transition region the photon absorption induces a decrease of the TES current, measured by a dc-SQUID amplifier, and the pulse integral of the bias power reduction corresponds to the absorbed energy. This means that TESs have the very interesting properties to be able to detect single photons with an intrinsic energy resolution, without filters or gratings, that limit the quantum efficiency. By contrary of classical detectors, if monochromatic light irradiates TESs, as usually happens in communication systems, they show the photon-number resolving (PNR) capability and due to the good signal to noise ratio TESs are almost free from dark counts. Moreover, in the superconducting detector family, TESs are the only true photon-number resolving detectors operating in the VIS-NIR range. Together with quantum information science, the PNR property results useful even for optical radiometry too. In the optical community, the candela - the International System (SI) unit for the luminous intensity - has not a common consensus whether its present definition fully satisfies the current and future needs of growing associated technology. Furthermore, actually there are substantial efforts directed toward a new definitions of four base SI units: the proposal wants to link the SI units to fundamental constants, leaving f.i. material artifact. Considering the recent advances in optical radiometry and in quantum technologies, for the candela world it means redefine its unit linking to the Planck constant and consequently expressing the luminous intensity unit in terms of photon number rather than optical power. This challenge has been accepted by several national metrology institutes to demonstrate the feasibility of redefining the candela. Inside this research project called `qu-candela', the TES PNR capability has been considered to build the bridge between the quantum and classical world of radiometry: i.e. the detector possibility to measure optical powers from one single photon per second to the lower limits of cryogenic radiometry, 104 photons per second. The theme of this work of thesis is to investigate both optical and electrical characterization of different kind of TESs based on a titanium/gold multilayer film, produced and developed at the National Institute of Metrological Research (INRIM) of Torino. Thanks to the proximity effect, the multilayer allows to lower with continuity the critical temperature from that of the Ti bulk (Tc ~ 390 mK) to those of interest: ~ 300 mK and ~ 100 mK. Detectors with higher Tc have shown a faster response pulse with a relaxing time constant of the order of 200 ns, while for the lower Tc sensors, the time constant is about 10 µs. By contrary to the response time, the detector intrinsic energy resolution is proportional to its film critical temperature. Our sensors work to discriminate incident photon from UV wavelengths to those typical of the telecommunications, 1310 nm and 1550 nm. Irradiating a TES with an active area of 10x10 µm^2 by incident photons of 0.79 eV (corresponds to a wavelength 1570 nm), the best energy resolution obtained has been 0.18 eV. Detectors with higher active area 20x20 µm^2 have a worse energy resolution, because it is also proportional to the material film heat capacity. In the meanwhile due to the same reason these kind of sensors present a bigger saturation energy. This has allowed to investigate on the TES capability to discriminate up to 29 incident photons simultaneously. Until now, such count represents the bigger amount of photons discriminated by single photon detectors, without reaching the device saturation, with a linear behaviour. From this count it has been estimated 12 photons on average, per pulse, at 9 kHz repetition rate; this results in a photon flux of about 105 photons/s, demonstrating the possibility of having a detector able to work from low flux regime to 1 photon/s to flux measurable by conventional semiconductor device (f.i. single photon avalanche detector SPAD). An innovative absolute calibration technique for PNR detector has been demonstrated. The absolute technique is based on the Klyshko's efficient solution to measure detection efficiency in photon counting rate and well know for common click-no-click detector. In fact, exploiting the recent developments in quantum state world, it is possible to work with quasi single photon state, by using a parametric down conversion heralded single photon source, and calibrate PNR detectors without requiring reference standards. The best detection efficiency, of ca. 50%, has been reached by coupling the smaller active area detectors with a 9 µm core optical fiber, single mode at telecom wavelengths
We investigate the use of a photon-number resolving (PNR) detector as an alternative method for measuring the second-order correlation function g2(0). Our implementation employs four spatially multiplexed single-photon detectors to reconstruct the photon number distribution P(n) from click statistics. We estimate g2(0) for both coherent and quantum dot excition emission, and compare the results to those obtained from a conventional Hanbury Brown-Twiss (HBT) setup. In the single-mode regime, we observe close agreement between both approaches. We additionally compare the acquisition times required for each method and find that PNR-based measurements enable faster estimation of g2(0), offering potential advantages for scalable characterisation of quantum light sources.
Since their first demonstration in 2001 [Gol’tsman et al., Appl. Phys. Lett. 79, 705–707 (2001)], superconducting-nanowire single-photon detectors (SNSPDs) have witnessed two decades of great developments. SNSPDs are the detector of choice in most modern quantum optics experiments and are slowly finding their way into other photon-starved fields of optics. Until now, however, in nearly all experiments, SNSPDs were used as “binary” detectors, meaning that they could only distinguish between 0 and >=1 photons, and photon number information was lost. Recent research has demonstrated proof-of-principle photon-number resolution (PNR) SNSPDs counting 2–5 photons. The photon-number-resolving capability is highly demanded in various quantum-optics experiments, including Hong–Ou–Mandel interference, photonic quantum computing, quantum communication, and non-Gaussian quantum state preparation. In particular, PNR detectors at the wavelength range of 850–950 nm are of great interest due to the availability of high-quality semiconductor quantum dots (QDs) [Heindel et al., Adv. Opt. Photonics 15, 613–738 (2023)] and high-performance cesium-based quantum memories [Ma et al., J. Opt. 19, 043001 (2017)]. In this paper, we demonstrate NbTiN-based SNSPDs with >94% system detection efficiency, sub-11 ps timing jitter for one photon, and sub-7 ps for 2 photons. More importantly, our detectors resolve up to 7 photons using conventional cryogenic electric readout circuitry. Through theoretical analysis, we show that the PNR performance of demonstrated detectors can be further improved by enhancing the signal-to-noise ratio and bandwidth of our readout circuitry. Our results are promising for the future of optical quantum computing and quantum communication.