In this manuscript I present an experimental investigation of the dynamics of an ultracold gas of bosonic ytterbium loaded into optical lattices and exposed to resonant light. The interaction between atoms and light makes it possible to study the coherence properties of the gas. The resonant driving is performed on the relevant optical transitions featured by ytterbium. On the one hand, I demonstrate the coherent driving of the internal state of the atoms on the clock transition, the excited state of which is metastable and can not spontaneously decay, thus preserving the coherence of the gas. The temporal internal dynamics in a deep lattice allows me to measure the collisional properties at low temperature for both clock states. On the other hand, I use the spontaneously emitted photons of the intercombination transition excited level to induce a coupling to the atomic external degrees of freedom. I present the momentum diffusion of a superfluid excited on this transition. Strong interactions between atoms slow down the decoherence and lead to an anomalous sub-diffusive relaxation. A simple model comprising atomic motion, interactions and dissipation accounts for our observations. A theoretical study of the dissipative dynamics in optical lattices sheds light on complementary phenomena such as induced dipole-dipole interactions or collective effects in spontaneous emission.
In this manuscript I present an experimental investigation of the dynamics of an ultracold gas of bosonic ytterbium loaded into optical lattices and exposed to resonant light. The interaction between atoms and light makes it possible to study the coherence properties of the gas. The resonant driving is performed on the relevant optical transitions featured by ytterbium. On the one hand, I demonstrate the coherent driving of the internal state of the atoms on the clock transition, the excited state of which is metastable and can not spontaneously decay, thus preserving the coherence of the gas. The temporal internal dynamics in a deep lattice allows me to measure the collisional properties at low temperature for both clock states. On the other hand, I use the spontaneously emitted photons of the intercombination transition excited level to induce a coupling to the atomic external degrees of freedom. I present the momentum diffusion of a superfluid excited on this transition. Strong interactions between atoms slow down the decoherence and lead to an anomalous sub-diffusive relaxation. A simple model comprising atomic motion, interactions and dissipation accounts for our observations. A theoretical study of the dissipative dynamics in optical lattices sheds light on complementary phenomena such as induced dipole-dipole interactions or collective effects in spontaneous emission.
Interaction résonante entre un champ laser et un gaz d'atomes d'ytterbium ultrafroids sur réseau optique : du contrôle cohérent au régime dissipatif Dans ce manuscrit je décris une série d'études expérimentales portant sur la dynamique d'un nuage d'atomes d'ytterbium bosonique dégénérés chargés dans un réseau optique et soumis à de la lumière résonante. L'interaction atome-lumière permet d'étudier les propriétés de cohérence quantique du gaz. Dans un premier temps, je démontre la manipulation cohérente de l'état interne des atomes sur la transition d'horloge, dont l'état excité est métastable et ne peux pas émettre de photons spontanément, protégeant ainsi la cohérence du gaz. La dynamique temporelle de l'état interne d'atomes chargés dans un réseau optique profond permet de mesurer les propriétés collisionelles à basse température pour les états horloges de l'ytterbium. Dans un second temps, j'utilise l'émission spontanée associée à la transition d'intercombinaison, ce qui permet un couplage aux degrés de liberté externes des atomes. Je présente l'étude de la diffusion en impulsion d'un superfluide excité sur cette transition. Les fortes interactions entre atomes conduisent à l'observation d'une décohérence ralentie aux temps longs et caractérisée par un régime sous-diffusif. Un modèle simple de type Bose-Hubbard incluant la dissipation permet de rendre compte de ces observations. Une étude théorique des effets à N-corps dans l'interaction atome-lumière vient en compléter l'analyse.
Quantum gases in optical lattices allow for fundamental studies in atomic and condensed-matter physics and the exploration of novel effects. After a brief introduction to the fundamentals of quantum gas experiments in optical lattices, we discuss two recent experiments focusing on driven matter waves in a one-dimensional optical lattice. The first experiment uses a tilted bichromatic optical lattice to investigate the interplay of disorder and collisional interactions in the accelerated transport of a Bose-Einstein condensate. Here, a screening effect is observed, in which the interactions effectively cancel the damping of Bloch oscillations induced by a (quasi-)disordered potential. This effect can be understood through a modification of the underlying band structure by the interactions. The second experiment studies the dynamics of a weakly trapped condensate resonantly coupled to the orbitals of a strongly confining state-selective lattice. We observe momentum distributions that correspond to matter wave diffraction from a periodic structure; however, the diffractive dynamics remain strongly linked to the internal-state Rabi oscillations. In the regime investigated, which we call the nonadiabatic regime, no diffracting potential can be defined. We show how only for much stronger coupling, the internal and external dynamics decouple, transitioning from nonadiabatic diffraction to the well-studied Kapitza-Dirac diffraction. We further investigate prospects for realizing dissipative spin models in our ultracold atomic gas experiment. To this end, we develop and test in the laboratory several possible implementations of effective spins with differential coupling to a superfluid background and examine their viability for a realization of the spin-boson model. | 94 pages
Recently, a new generation of experiments with ultracold quantum gases has emerged where the many-body properties are probed and manipulated using ultra-narrow “clock” transitions. We describe here our experimental project, which aims at engineering a special kind of optical lattice realizing an effective magnetic field coupling to the atomic motion - the Hofstadter optical lattice. Our specific experimental scheme uses the ultra-narrow optical transition linking the ground state to a metastable excited state of 174 Ytterbium atoms. We present the current status of the experiment, including the observation of coherent Rabi oscillations between the ground and excited states.
This thesis describes experiments focused on investigating out-of-equilibrium phenomena in the Bose-Hubbard Model and exploring novel cooling techniques for ultracold gases in optical lattices. In the first experiment, we study quenches across the Mott-insulator-to-superfluid quantum phase transition in the 3D Bose-Hubbard Model. The quench is accomplished by continuously tuning the ratio of the Hubbard energies. We observe that the degree of excitation is proportional to the fraction of atoms that cross the phase boundary, and that the amount of excitations and energy produced during the quench have a power-law dependence on the quench rate. These phenomena suggest an excitation process analogous to the mechanism for defect generation in non-equilibrium classical phase transitions. This experiment constitutes the first observation of the Kibble-Zurek mechanism in a quantum quench. We have reported our findings in Ref. [1]. In a second experiment, published in Ref. [2], we investigate dissipation as a method for cooling a strongly interacting gas. We introduce dissipation via a bosonic reservoir to a strongly interacting bosonic gas in the Mott-insulator regime of a 3D spin-dependent optical lattice. The lattice atoms are excited to a higher energy band using laser-induced Bragg transitions. A weakly interacting superfluid comprised of atoms in a state that does not experience the lattice potential acts as a dissipative bath that interacts with the lattice atoms through collisions. We measure the resulting bath-induced decay using the atomic quasimomentum distribution, and we compare the decay rate with predictions from a weakly interacting model with no free parameters. A competing intrinsic decay mechanism arising from collisions between lattice atoms is also investigated. The presence of intrinsic decay can not be accommodated within a non-interacting framework and signals that strong interactions may play a central role in the lattice-atom dynamics. The intrinsic decay process we observe may negatively impact the success of cooling via dissipation because a fraction of intrinsic decay events can deposit a large amount of energy into the lattice gas. In a third experiment, we develop and carry out the first demonstration of cooling an atomic quasimomentum distribution. Our scheme, applied in a proof-of-principle experiment to 3D Bose-Hubbard gas in the superfluid regime, involves quasimomentum-selective Raman transitions. This experiment is motivated by the search of new cooling techniques for lattice-trapped gases. Efficient cooling exceeding heating rates is achieved by iteratively removing high quasimomentum atoms from the lattice. Quasimomentum equilibration, which is necessary for cooling, is investigated by directly measuring rethermalization rates after bringing the quasimomentum distribution of the gas out of equilibrium. The measured relaxation rate is consistent at high lattice depths with a short-range, two-particle scattering model without free parameters, despite an apparent violation of the Mott-Ioffe-Regel bound. Our results may have implications for models of unusual transport phenomena in materials with strong interactions, such as heavy fermion materials and transition metal oxides. The cooling method we have developed is applicable to any species, including fermionic atoms. Our results are available in Ref. [3]
This thesis summarizes the research work we did in the past years, which focuses on the theoretical study of quantum effects of ordered atomic structures interacting with the quantum electric field of an optical resonator. Within this work we investigated the quantum properties of the light at the cavity output, emitted by this kind of system, and the quantum state of the atoms confined by the light fields of the cavity mode. Following one possible partition, we have organized the thesis in two parts. The first part of the thesis is devoted to the quantum properties of the light at the output of optical cavities, in which atoms are confined. After a brief introduction on the basics of atom-photon interactions, we show theoretically, that two atomic dipoles in a resonator can behave as a quantum non-linear medium, whose response can be controlled through the interactomic distance of the atoms inside the resonator. We identify the parameter regime, for which the system operates as a parametric amplifier, based on the atoms' collective dipole cascade emission. Moreover we also determine the corresponding field squeezing spectrum at the cavity output. These dynamics could be observed as a result of self-organization processes of laser-cooled atoms in resonators. The second part of the thesis studies the quantum ground state of an ultracold atomic gas trapped inside an optical resonator by the mechanical effects of atom-photon interactions. Due to the strong coupling regime, the ultracold atomic gas feels a quantum potential, where the fluctuations at the single photon level may be relevant in determining the trapping conditions. This potential depends on the atomic distribution, which at the same time determines the intracavity field amplitude. Here, after a brief introduction on ultracold atoms in optical lattices, we study the low temperature physics of an ultracold atomic gas in the quantum potential formed inside a pumped cavity, by mapping the dynamics to an effective Bose-Hubbard model. We predict the existence of non-compressible states of the atomic gas, and determine a phase diagram as a function of the cavity parameters. Novel effects are encountered, such as the existence of overlapping stability regions corresponding to competing insulator-like states when the laser pumps the cavity, to provide one example out of many. At the end of the thesis a concluding chapter presents some general outlooks to this thesis work.
Quantum degenerate atomic gases offer a unique platform for the exploration of a wide variety of interacting many-body systems in a pristine environment, based on a set of powerful tools for the coherent control of the atoms' internal and external degrees of freedom. Here, we present experimental studies of strongly interacting bosonic mixtures in one-dimensional (1D) systems, in which the mobilities of the two species are independently controlled with a state-selective optical lattice. In a first experiment, we freeze out the tunneling of one species from a binary mixture, and study the formation of ``quantum emulsion'' states, where immobile atoms serve as a static, random disorder for a more mobile species. We investigate the 1D superfluid-to-insulator transition in the presence of this disorder, and make comparisons to the effects of quasi-disorder from an incommensurate optical lattice. We observe enhanced localization in the more random potential, highlighting the important role of correlations in disordered systems. Through a combined measurement of transport, localization, and excitation spectra, we are able to obtain strong evidence for observation of a disordered, insulating quantum phase, the 1D Bose glass. In a second experiment, we introduce a new experimental technique for the characterization of ultracold gases held in optical lattices. In analogy to neutron diffraction from solids, we use atomic de Broglie waves to non-destructively probe the spatial structure of 1D Mott insulators through elastic Bragg diffraction, and to probe inelastic band-structure excitations of more weakly interacting 1D Bose gases. Furthermore, we use the diffraction of matter waves to detect the formation of forced-antiferromagnetic ordering in a crystalline atomic spin mixture. Lastly, we study the dynamical response of matter waves to a periodically pulsed, incommensurate optical lattice, a situation that realizes a system of two coupled kicked quantum rotors. We observe that the coupling induces a suppression of energy growth at quantum resonances, and a localization-to-delocalization transition in momentum space for off-resonant driving. Our observations confirm a long-standing theoretical prediction for the two-rotor system, and illustrate how classical behavior can emerge from the evolution of a simple quantum system. | 193 pages