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Journal of Applied Spectroscopy

Transition from the Fluctuation Mode of Stimulated Resonant Coherent Raman Scattering to the Energy–Stabilized Mode

N. I. Shamrov

Published Jul 1, 2001• 0 citations
Publisher
DOI
10.1023/a:1012557619140

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Annual Meeting Optical Society of America•Jan 1, 1987•1 citation
The far field direction of propagation of light pulses generated by transient, single pass stimulated Raman scattering (SRS) is observed to fluctuate front pulse to pulse due to quantum mechanical uncertainties in the occupation numbers of different coherent spatial modes. When SRS is generated on the Q(l) vibrational transition in hydrogen with an interaction region Fresnel number near unity, the lowest-order coherent spatial mode dominates the generation process, leading to near-diffraction-limited Stokes light.
An experimental study of stimulated Raman scattering (SRS) has been performed using a subnanosecond pulse to investigate the statistical properties of Stokes light generation.1 There are macroscopic fluctuations of Stokes pulse energy as well as random generation of spatial mode patterns. When the scattering volume has a low Fresnel number, the spatial patterns of the SRS resemble cavity modes. When the Fresnel number is large, there are irregular structures appearing across the Stokes profile in a random fashion. A theoretical study of the spatial and temporal coherence properties of Raman generation using a Gaussian-profile pump pulse has also been carried out. Using a Gaussian-Laguerre mode expansion technique,2 it is found that the higher-order spatial coherence modes1 experience different gain than the lower-order spatial coherence modes, and consequently the temporal coherence associated with each individual spatial coherence mode is different.