Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical review. B./Physical review. B

Third-order frequency-resolved photon correlations in resonance fluorescence

Yamil Nieves, Andreas Müller

Published Oct 22, 2018• 15 citations
Publisher

Abstract

Recently, the concept of an ''$N$-photon spectrum'' -- a spectrally resolved $N$-photon correlation function -- has been introduced as an innovative quantum optics characterization tool that uniquely reveals information about pathways underlying the generation of light in a given source. Here, the authors investigate experimentally the three-photon spectrum of resonance fluorescence from a single semiconductor quantum dot. The observations agree with previous theoretical work, revealing significantly more pronounced photon antibunching at the Mollow triplet sidebands and more strongly correlated emission through virtual states compared to the two-photon counterpart.

DOI
10.1103/physrevb.98.165432

Related papers

Measurements of Frequency-Resolved Third-Order Correlations in Quantum Dot Resonance Fluorescence

Yamil Nieves, Andreas Müller

We investigated the three-photon spectrum of quantum dot resonance fluorescence, revealing significantly more pronounced photon antibunching at the Mollow triplet sidebands and more strongly correlated emission through virtual states than at second order. © 2019 The Author(s)

Conference on Lasers and Electro-Optics•May 5, 2019•0 citations

Measurements of Frequency-Resolved Third-Order Correlations in Quantum Dot Resonance Fluorescence

Yamil Nieves, Andreas Müller

We investigated the three-photon spectrum of quantum dot resonance fluorescence, revealing significantly more pronounced photon antibunching at the Mollow triplet sidebands and more strongly correlated emission through virtual states than at second order.

Conference on Lasers and Electro-Optics•Jan 1, 2019•0 citations

Fluorescence spectrum of a hybrid three-level quantum dot nanoparticle system

Aryan Iliat

Quantum optics provides a fundamental framework for understanding the interaction between light and matter at the quantum level. Recently, it has been shown that under incoherent pumping, the resonance fluorescence spectrum dramatically changes. Engineering the resonance fluorescence spectrum paves the way towards solid-state-based single-photon sources. In this paper, we start by reviewing and reproducing some of the results concerning the resonance fluorescence spectrum, single-photon sources, dressed-state lasers, and luminescence spectrum of a quantum dot in a microcavity. Photon correlations in quantum optical systems and spectral properties of radiation emitted by atomic and semiconductor systems interacting with external fields are investigated. The well known Mollow triplet structure of the emission spectrum is discussed, together with the role of dressed states in explaining the origin of the three spectral peaks. Furthermore, the luminescence spectra of quantum emitters coupled to microcavities are reviewed. The numerical results presented here contribute to the theoretical understanding of resonance fluorescence, photon correlations, and engineered emission in quantum optical systems. These studies highlight the rich physical properties arising from light matter interaction at the quantum level and demonstrate their relevance for emerging quantum technologies.

quant-pharXiv:2603.24805•Mar 27, 2026•0 citations

Coherence and photon statistical properties of the Mollow triplet sideband emission of a quantum dot

P. Michler

We present a detailed photon statistical analysis of the resonance fluorescence emission triplet from a single semiconductor quantum dot. The photon correlation measurements demonstrate both ‘single’ and ‘cascaded’ photon emission from the Mollow triplet sidebands.

Frontiers in Optics•Jan 1, 2012•0 citations

Markovian Approach to N -Photon Correlations beyond the Quantum Regression Theorem

Mateusz J. Salamon, Oliver Dudgeon, Ahsan Nazir +1 more

Multiphoton correlations from quantum emitters coupled to vibrational environments lie beyond the reach of standard tools such as the quantum regression theorem. Here, we introduce a Markovian framework for computing frequency-resolved N-photon correlation functions that overcomes this limitation. Applying our approach to a driven semiconductor quantum dot provides a tractable description of phonon effects on fluorescence beyond the single-photon spectrum. Our method accurately captures the emergence of the phonon sideband, missed by conventional quantum regression theorem treatments, and reveals rich phonon-induced structure in the filtered two-photon spectrum. Strikingly, we find that photons emitted via the phonon sideband inherit second-order coherence properties of the Mollow triplet.

arXiv:2509.21569•Physical Review Letters•Jan 22, 2026•2 citations

Frequency-resolved N-photon correlations in the ultra-strong coupling regime

Wen Huang, Qian Bin, Ying Wu +1 more

Frequency-resolved photon emission is central to applications from quantum information encoding to high-resolution spectroscopy, and then studying their correlations is therefore essential for revealing the underlying emission pathways and multiphoton statistics. Here, we investigate frequency-resolved N-photon correlations in an ultrastrongly coupled cavity QED system where a qubit interacts with a single-mode cavity. Owing to counter-rotating interactions, the eigenstates and energy spectrum are strongly modified, giving rise to rich spectral and statistical properties in the emitted frequency-resolved photons. Through frequency-selective detection, we reveal pronounced multiphoton antibunching, as well as multiphoton bunching originating from cascade transitions among dressed eigenstates. In particular, we show that parity symmetry plays a decisive role in shaping these correlations. The symmetry-breaking opens additional transition channels and dramatically enhances the generation of correlated photon pairs and even photon triplets of different frequencies. Our work extends frequency-resolved correlations to the ultra-strong coupling regime and demonstrates their potential as a sensitive probe of symmetry in light-matter interaction systems.

quant-pharXiv:2603.14201•Mar 17, 2026•0 citations
Recently, the concept of an ''NNN-photon spectrum'' -- a spectrally resolved NNN-photon correlation function -- has been introduced as an innovative quantum optics characterization tool that uniquely reveals information about pathways underlying the generation of light in a given source. Here, the authors investigate experimentally the three-photon spectrum of resonance fluorescence from a single semiconductor quantum dot. The observations agree with previous theoretical work, revealing significantly more pronounced photon antibunching at the Mollow triplet sidebands and more strongly correlated emission through virtual states compared to the two-photon counterpart.
Quantum optics provides a fundamental framework for understanding the interaction between light and matter at the quantum level. Recently, it has been shown that under incoherent pumping, the resonance fluorescence spectrum dramatically changes. Engineering the resonance fluorescence spectrum paves the way towards solid-state-based single-photon sources. In this paper, we start by reviewing and reproducing some of the results concerning the resonance fluorescence spectrum, single-photon sources, dressed-state lasers, and luminescence spectrum of a quantum dot in a microcavity. Photon correlations in quantum optical systems and spectral properties of radiation emitted by atomic and semiconductor systems interacting with external fields are investigated. The well known Mollow triplet structure of the emission spectrum is discussed, together with the role of dressed states in explaining the origin of the three spectral peaks. Furthermore, the luminescence spectra of quantum emitters coupled to microcavities are reviewed. The numerical results presented here contribute to the theoretical understanding of resonance fluorescence, photon correlations, and engineered emission in quantum optical systems. These studies highlight the rich physical properties arising from light matter interaction at the quantum level and demonstrate their relevance for emerging quantum technologies.
Multiphoton correlations from quantum emitters coupled to vibrational environments lie beyond the reach of standard tools such as the quantum regression theorem. Here, we introduce a Markovian framework for computing frequency-resolved N-photon correlation functions that overcomes this limitation. Applying our approach to a driven semiconductor quantum dot provides a tractable description of phonon effects on fluorescence beyond the single-photon spectrum. Our method accurately captures the emergence of the phonon sideband, missed by conventional quantum regression theorem treatments, and reveals rich phonon-induced structure in the filtered two-photon spectrum. Strikingly, we find that photons emitted via the phonon sideband inherit second-order coherence properties of the Mollow triplet.
Frequency-resolved photon emission is central to applications from quantum information encoding to high-resolution spectroscopy, and then studying their correlations is therefore essential for revealing the underlying emission pathways and multiphoton statistics. Here, we investigate frequency-resolved N-photon correlations in an ultrastrongly coupled cavity QED system where a qubit interacts with a single-mode cavity. Owing to counter-rotating interactions, the eigenstates and energy spectrum are strongly modified, giving rise to rich spectral and statistical properties in the emitted frequency-resolved photons. Through frequency-selective detection, we reveal pronounced multiphoton antibunching, as well as multiphoton bunching originating from cascade transitions among dressed eigenstates. In particular, we show that parity symmetry plays a decisive role in shaping these correlations. The symmetry-breaking opens additional transition channels and dramatically enhances the generation of correlated photon pairs and even photon triplets of different frequencies. Our work extends frequency-resolved correlations to the ultra-strong coupling regime and demonstrates their potential as a sensitive probe of symmetry in light-matter interaction systems.