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Bulletin of the Lebedev Physics Institute

Microwave Antenna for Exciting Optically Detected Magnetic Resonance in Diamond NV Centers

Vladimir V. Soshenko, Olga R. Rubinas, Vadim Vorobyov, Stepan V. Bolshedvorskii, Polina V. Kapitanova, Vadim N. Sorokin, Alexey V. Akimov

Published Aug 1, 2018• 14 citations
Publisher

Abstract

A microwave antenna configuration shaped as coaxial resonant coils is proposed for exciting magnetic dipole transitions of the optical ground state of the nitrogen—vacancy color center in diamond. The field within the antenna is simulated, field amplitudes are experimentally measured.
DOI
10.3103/s1068335618080043

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Dielectric resonator antenna with circular polarization of microwave magnetic field for efficient, coherent and uniform spin manipulation at nitrogen-vacancy centers in diamond is discussed. The results of numerical simulations of the microwave magnetic field generated by the antenna are reported and analyzed. The uniform magnetic field with circular polarization is obtained inside the antenna. Using the simulated amplitude of the magnetic field inside the antenna the Rabi frequency is estimated. The Rabi frequency of 41 MHz with inhomogeneity less then 1 % for the diamond volume of 3 mm 3 is demonstrated under 10 W of input microwave power.
The nitrogen vacancy (NV) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels $({m}_{s}=\ifmmode\pm\else\textpm\fi{}1)$ degenerate at zero magnetic field. Polarization-selective microwave excitation is an attractive method to address the spin transitions independently since this allows operation down to zero magnetic field. Using a resonator designed to produce circularly polarized microwaves, we have investigated the polarization selection rules of the NV center. We first apply this technique to NV ensembles in [100]- and [111]-oriented samples. Next, we demonstrate an imaging technique, based on optical polarization dependence, which allows rapid identification of the orientations of many single NV centers. Finally, we test the microwave polarization selection rules of individual NV centers of known orientation.
Nitrogen vacancy (NV) centres are a type of defect in diamond that exhibit a number of interesting properties. NV centres can be optically excited around 450-650 nm and emit fluorescence at around 550-800 nm [1]. The optical excitation also spin polarises the negatively charged NV centres, permitting optical detection of magnetic resonance [2]. This allows nanotesla scale sensitive magnetometry to be performed with nanometre scale spatial resolution [3].To date, a direct measurement of stimulated emission from ensembles of NV centres in diamond has yet to be demonstrated experimentally. Despite this, stimulated emission depletion microscopy has been utilised in superresolution imaging that relies on the stimulated emission of single NV centres to quench fluorescence [4]. Recently, there has also been similar indirect experimental evidence of stimulated emission in NV ensembles [5]. We thus aimed to show both optical gain of a probe beam in a pumped NV-rich diamond sample and a modulation of this gain via microwave excitation of its ground level spin transitions. The experimental set-up consisted of a pump (532 nm) and probe (723-950 nm) laser beam combined with a dichroic mirror and focused into a bulk diamond specimen to a spot-size of around 90 microns. Pump excitation powers of up to 3 W and probe powers up to 0.5 W were used. The beams were then collimated and separated with a prism and the probe power measured with a photodiode. The diamond specimen was placed on an antenna to allow simultaneous excitation with microwaves. A double modulation scheme was employed to measure either the change in probe power due to the pump laser or the microwave excitation during any one experiment.
For quantum sensing based on nitrogen-vacancies (NV) ensembles, microwave antennas can couple the microwave field to the NV center, which leads it to becoming the core of spin manipulation and can directly affect the sensitivity of quantum sensing. The double split-ring resonator is a widely used microwave device for NV ensembles due to the advantages of high radiation efficiency and uniform magnetic field in millimeter-scale areas. But the bandwidth (30 MHz) is quite narrow which limits the application in quantum sensing with NV ensembles. Here, we experimentally achieve continuous tuning of the resonant frequency of the double split-ring resonator by changing the copper sheet position on the edge of the outer ring. The frequency tuning range can reach 80 MHz, up to 2-3 times the bandwidth, which can cover the transition of the electron spin under different magnetic field conditions. The performance of the tunable antenna in the quantum operation of NV centers is verified by optically detected magnetic resonance and Rabi oscillation. This tunable antenna is promising in the fabrication of integrated and arrayed quantum sensors based on NV ensembles.