Abstract Due to their frequency scaling and long-term coherence, frequency combs at the single-photon level can provide a fascinating platform for developments in quantum technology. Here we demonstrate frequency comb single-photon interferometry in an unheralded manner. We are able to induce coherence by erasing the which-way information of path-entangled photon pairs. The photon pairs are prepared using a dual parametric down-conversion pumped by a highly stable frequency comb laser and an ultra-narrow seed laser. This is conducted at the extremely low-conversion efficiency regime. The unique feature of our quantum interferometer is that the induced one-photon interference of the path-encoded single photons (signal), with multiple frequency components, is observed with a unit visibility without heralding conjugate photons (idler). We demonstrate that quantum information and frequency comb technology can be combined to realize quantum information platforms. We expect this will contribute to the application of quantum information and optical measurements beyond the classical limit.
Abstract Due to their frequency scaling and long-term coherence, frequency combs at the single-photon level can provide a fascinating platform for developments in quantum technology. Here we demonstrate frequency comb single-photon interferometry in an unheralded manner. We are able to induce coherence by erasing the which-way information of path-entangled photon pairs. The photon pairs are prepared using a dual parametric down-conversion pumped by a highly stable frequency comb laser and an ultra-narrow seed laser. This is conducted at the extremely low-conversion efficiency regime. The unique feature of our quantum interferometer is that the induced one-photon interference of the path-encoded single photons (signal), with multiple frequency components, is observed with a unit visibility without heralding conjugate photons (idler). We demonstrate that quantum information and frequency comb technology can be combined to realize quantum information platforms. We expect this will contribute to the application of quantum information and optical measurements beyond the classical limit.
Quantum spectroscopy with undetected photons (QSUP) utilizing the quantum entanglement of parametrically down-converted photons has emerged as a new spectroscopic platform. Here, we demonstrate a high-resolution and remote-measurement QSUP, where light-matter interactions and photon detections are performed in spectrally and spatially different regions. A dual-stimulated parametric down-conversion scheme with an optical frequency-comb pump and ultra-narrow coherent seed beam in an idler mode is used to generate path-entangled pairs of the undetected idler and measured frequency-comb signal photons. To demonstrate the frequency resolution of this scheme, a Fabry-Pérot cavity with a narrow bandwidth is used as a sample that modulates the distinguishability of one-photon-added coherent idler beams, which directly affects the interference fringe visibility of the entangled signal photons. We thus anticipate that the remote QSUP whose frequency resolution is determined by the linewidth of the coherent seed laser will enable the development of quantum spectroscopy featuring high resolution.
The on-chip generation of optical quantum states will enable accessible advances for quantum technologies. We demonstrate that integrated quantum frequency combs (based on high-Q microring resonators made from a CMOS-compatible, high refractive-index doped-glass platform) can enable the generation of pure heralded single photons, cross-polarized photon pairs, as well as bi- and multi-photon entangled qubit states over a broad frequency comb covering the S, C, L telecommunications band, with photon frequencies corresponding to standard telecommunication channels spaced by 200 GHz. Exploiting a self-locked, intra-cavity excitation configuration, a highly-stable source of multiplexed heralded single photons is demonstrated, operating continuously for several weeks with less than 5% fluctuations. The photon bandwidth of 110 MHz is compatible with quantum memories, and high photon purity was confirmed through single-photon auto-correlation measurements. In turn, by simultaneously exciting two orthogonal polarization mode resonances, we demonstrate the first realization of type-II spontaneous FWM (in analogy to type-II spontaneous parametric down-conversion), allowing the direct generation of orthogonally-polarized photon pairs on a chip. By using a double-pulse excitation, we demonstrate the generation of time-bin entangled photon pairs. We measure qubit entanglement with visibilities above 90%, enabling the implementation of quantum information processing protocols. Finally, the excitation field and the generated photons are intrinsically bandwidth-matched due to the resonant characteristics of the ring cavity, enabling the multiplication of Bell states and the generation of a four-photon time-bin entangled state. We confirm the generation of this four-photon entangled state through four-photon quantum interference.
The exploitation of quantum mechanics has the potential to solve important challenges and \nintroduce novel technologies enabling, among others, powerful computation (which can solve \ncertain problems exponentially faster than classical computers), perfectly secure communications, \nas well as sensing and imaging with precision and resolutions not achievable by classical means. \nIn order to make use of the unique properties of quantum physics, experimental platforms \nthat provide access to, and allow the control of quantum states, need to be developed. In \nparticular, quantum systems composed of multiple parties are required, where each party is in a \ncoherent superposition of states, and where multiples of such parties are in a coherent \nsuperposition with each other (e.g. being entangled). Additionally, in order to make use of such \nentangled quantum systems, it is required that each individual party can be coherently controlled \nand measured. The usability and available quantum resources of the entangled system is related \nto its size, which is proportional to the number of entangled parties, as well as the dimensionality \nof the superposition each party is in. For this reason, there is a imminent demand to achieve, \ninvestigate, and improve the generation and control of large quantum systems, comprised of as \nmany entangled parties as possible, where each party is in an ideally high-dimensional \nsuperposition. \nMany quantum platforms are currently subject to extensive research, such as trapped ions, \nsuperconducting circuits, defect centers in solid-state crystals, mechanical oscillators, and optical \nquantum states (i.e. photons). While all platforms provide distinct advantages (as well as \nchallenges), optical photon states are of particular interest, because they can interact with other \nquantum systems, and can be transmitted over long distances while preserving their quantum \ncoherence without the need for extensive shielding. A large variety of sources for optical \nquantum states has been demonstrated, however most such implementations suffer from high \ncomplexity, ultimately limiting their scalability. Integrated photonics has recently become a \nleading platform for the compact, cost-efficient, and stable generation and processing of optical \nquantum states. However, to date, integrated quantum sources have only been able to generate \nphoton pairs, which operated on single channels, and single polarization modes. Furthermore, in \nthe few realizations of on-chip entanglement, they were limited to two entangled parties, where \neach party was in a two-dimensional superposition. These limitations of current integrated photon sources arise in large part from the concepts currently exploited to generate and control these \nstates. In particular, path-entangled sources are the most commonly used, but increasing the \nquantum state complexity requires a significant, and very challenging, increase in device \ncomplexity. There is therefore an urgent need to develop new concepts that can achieve the onchip \ngeneration of large and complex photon states without increasing source complexity, while \nstill enabling coherent quantum state control and detection. \nIn this work, we aim to address these limitations by making use of multiple frequency and \ntemporal modes within a single spatial waveguide mode (therefore readily compatible with \nstandard optical fibers) of an on-chip microring resonator. This approach is in contrast to more \ncommonly used techniques relying on path entanglement, which exploits multiple spatial modes \nand generates entanglement by means of complex waveguide structures. Working within a single \nspatial mode, we achieve the first demonstration of pure heralded single photons and entangled \nphoton pairs, which are emitted on multiple frequency modes from a single source. We then \ndemonstrate the first generation of multi-photon entangled quantum states on a photonic chip. \nFinally, by making use of the spectral multi-mode nature of optical frequency combs, we achieve \nthe generation of photon pairs in a coherent superposition of multiple frequency modes, \nrepresenting the first generation of high-dimensional entangled states on a photonic chip. \nOur work represents a significant step forward in the generation of complex quantum \nstates on a photonic chip and in a single spatial mode compatible with standard optical fibers. In \naddition, we demonstrated coherent quantum state control and manipulation for all generated \nstates by means of standard telecommunications components, which could in the future be also \nintegrated on single, monolithic chip. Our results indicate that the exploitation of integrated \noptical frequency comb sources for the generation of optical quantum states can provide a \nscalable and practical platform for quantum technologies.
The investigation of integrated frequency comb sources characterized by equidistant spectral modes was initially driven by considerations toward classical applications, seeking a more practical and miniaturized way to generate stable broadband sources of light. Recently, in the context of scaling the complexity of optical quantum circuits, these on-chip approaches have provided a new framework to address the challenges associated with non-classical state generation and manipulation. For example, multi-photon and high-dimensional states were to date either inaccessible, lacked scalability, or were difficult to manipulate, requiring elaborate approaches. The emerging field of quantum frequency combs studying spectral multimode sources based on the judicious excitation of (typically) third-order nonlinear optical micro-cavities has begun to address these issues. Several quantum sources based on this concept have already been demonstrated, among them are combs of correlated photons, cross-polarized photon pairs, entangled photon pairs, multi-photon states, and high-dimensional entangled states. While sources have achieved increasing complexity, so have coherent state processing operations, demonstrated in a practical manner using standard telecommunications components. Here, we review our recent work in the development of this framework, with a focus on multi-photon and high-dimensional states. The integrated frequency comb platform thus demonstrates significant potential for the development of meaningful quantum optical technologies.
The Hong-Ou-Mandel interferometer is a versatile tool for analyzing the joint properties of photon pairs, relying on a truly quantum interference effect between two-photon probability amplitudes. While the theory behind this form of two-photon interferometry is well established, the development of advanced photon sources and exotic two-photon states has highlighted the importance of quantifying precisely what information can and cannot be inferred from features in a Hong-Ou-Mandel interference trace. Here we examine Hong-Ou-Mandel interference with regard to a particular class of states, so-called quantum frequency combs, and place special emphasis on the role spectral phase plays in these measurements. We find that this form of two-photon interferometry is insensitive to the relative phase between different comb line pairs. This is true even when different comb line pairs are mutually coherent at the input of a Hong-Ou-Mandel interferometer and the fringe patterns display sharp temporal features. Consequently, Hong-Ou-Mandel interference cannot speak to the presence of high-dimensional frequency-bin entanglement in two-photon quantum frequency combs.