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Nature Communications

Universal holonomic quantum gates over geometric spin qubits with polarised microwaves

Kodai Nagata, Kouyou Kuramitani, Yuhei Sekiguchi, Hideo Kosaka

Published Aug 7, 2018• 92 citations
Publisher

Abstract

A microwave shares a nonintuitive phase called the geometric phase with an interacting electron spin after an elastic scattering. The geometric phase, generally discarded as a global phase, allows universal holonomic gating of an ideal logical qubit, which we call a geometric spin qubit, defined in the degenerate subspace of the triplet spin qutrit. We here experimentally demonstrate nonadiabatic and non-abelian holonomic quantum gates over the geometric spin qubit on an electron or nitrogen nucleus. We manipulate purely the geometric phase with a polarised microwave in a nitrogen-vacancy centre in diamond under a zero-magnetic field at room temperature. We also demonstrate a two-qubit holonomic gate to show universality by manipulating the electron-nucleus entanglement. The universal holonomic gates enable fast and fault-tolerant manipulation for realising quantum repeaters interfacing between universal quantum computers and secure communication networks.

DOI
10.1038/s41467-018-05664-w

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A microwave shares a nonintuitive phase called the geometric phase with an interacting electron spin after an elastic scattering. The geometric phase, generally discarded as a global phase, allows universal holonomic gating of an ideal logical qubit, which we call a geometric spin qubit, defined in the degenerate subspace of the triplet spin qutrit. We here experimentally demonstrate nonadiabatic and non-abelian holonomic quantum gates over the geometric spin qubit on an electron or nitrogen nucleus. We manipulate purely the geometric phase with a polarised microwave in a nitrogen-vacancy centre in diamond under a zero-magnetic field at room temperature. We also demonstrate a two-qubit holonomic gate to show universality by manipulating the electron-nucleus entanglement. The universal holonomic gates enable fast and fault-tolerant manipulation for realising quantum repeaters interfacing between universal quantum computers and secure communication networks.
We demonstrate universal non-adiabatic non-abelian holonomic single quantum gates over a geometric electron spin with phase-modulated polarized light and 93% average fidelity. This allows purely geometric rotation around an arbitrary axis by any angle defined by light polarization and phase using a degenerate three-level Λ-type system in a negatively charged nitrogen-vacancy center in diamond. Since the control light is completely resonant to the ancillary excited state, the demonstrated holonomic gate not only is fast with low power, but also is precise without the dynamical phase being subject to control error and environmental noise. It thus allows pulse shaping for further fidelity.
Abstract Spins in diamond are ideal for large-scale quantum processors and memories. Localized laser field offers spatial selectivity for electron spin manipulation through spin-obit coupling. However, it has been difficult to simultaneously achieve the precise and universal manipulation by itself. Here, we demonstrate microwave-driven holonomic quantum gates on an optically selected electron spin in a nitrogen-vacancy (NV) center in diamond. The electron spin is precisely manipulated with global microwave tuned to the frequency shift induced by the local optical Stark effect. We show the universality of the operations, including state initialization, preparation, readout, and echo. We also generate optically addressable entanglement between the electron and adjacent nitrogen nuclear spin, thus satisfying the scalability requirement of qubits. High fidelity operations are achieved by amplitude-alternating pulse, which are tolerant to fluctuations in microwave intensity and detuning. These techniques enable site-selective quantum teleportation transfer from a photon to a nuclear spin memory, paving the way for the realization of distributed quantum computers and the quantum Internet with large-scale quantum storage.
At its most fundamental level, circuit-based quantum computation relies on the application of controlled phase shift operations on quantum registers. While these operations are generally compromised by noise and imperfections, quantum gates based on geometric phase shifts can provide intrinsically fault-tolerant quantum computing. Here we demonstrate the high-fidelity realization of a recently proposed fast (non-adiabatic) and universal (non-Abelian) holonomic single-qubit gate, using an individual solid-state spin qubit under ambient conditions. This fault-tolerant quantum gate provides an elegant means for achieving the fidelity threshold indispensable for implementing quantum error correction protocols. Since we employ a spin qubit associated with a nitrogen-vacancy colour centre in diamond, this system is based on integrable and scalable hardware exhibiting strong analogy to current silicon technology. This quantum gate realization is a promising step towards viable, fault-tolerant quantum computing under ambient conditions. Quantum gates based on geometric phase shifts offer a promising approach for the realization of fault-tolerant quantum computing. Using nitrogen-vacancy centre qubits in diamond, this study experimentally realises a high-fidelty, non-adiabatic, non-Abelian holonomic single-qubit gate at room temperature.
Geometric phases and holonomies are a promising resource for the realization of high-fidelity quantum operations in noisy devices, due to their intrinsic fault-tolerance against parametric noise. However, for a long time their practical use in quantum computing was limited to proof of principle demonstrations. This was partly due to the need for adiabatic time evolution or the requirement of complex, high-dimensional state spaces and a large number of driving field parameters to achieve universal quantum gates employing holonomies. In 2016 Liang et al. proposed universal, superadiabatic, geometric quantum gates exploiting transitionless quantum driving, thereby offering fast and universal quantum gate performance on a simple two-level system. Here, we report on the experimental implementation of a set of non-commuting single-qubit superadiabatic, geometric quantum gates on the electron spin of the nitrogen-vacancy center in diamond under ambient conditions. This provides a promising and powerful tool for large-scale quantum computing under realistic, noisy experimental conditions.
The holonomic approach to controlling (nitrogen-vacancy) NV-center qubits provides an elegant way of theoretically devising universal quantum gates that operate on qubits via calculable microwave pulses. There is, however, a lack of simulated results from the theory of holonomic control of quantum registers with more than two qubits describing the transition between the dark states. Considering this, we have been experimenting with the IBM Quantum Experience technology to determine the capabilities of simulating holonomic control of NV-centers for three qubits describing an eight-level system that produces a non-Abelian geometric phase. The tunability of the geometric phase via the detuning frequency is demonstrated through the high fidelity (~85%) of three-qubit off-resonant holonomic gates over the on-resonant ones. The transition between the dark states shows the alignment of the gate's dark state with the qubit's initial state hence decoherence of the multi-qubit system is well-controlled through a π/3 rotation.
Abstract Geometric phases and holonomies are a promising resource for the realization of high-fidelity quantum operations in noisy devices, due to their intrinsic fault-tolerance against parametric noise. However, for a long time their practical use in quantum computing was limited to proof of principle demonstrations. This was partly due to the need for adiabatic time evolution or the requirement of complex, high-dimensional state spaces and a large number of driving field parameters to achieve universal quantum gates employing holonomies. In 2016 Liang et al. proposed universal, superadiabatic, geometric quantum gates exploiting transitionless quantum driving, thereby offering fast and universal quantum gate performance on a simple two-level system. Here, we report on the experimental implementation of a set of non-commuting single-qubit superadiabatic, geometric quantum gates on the electron spin of the nitrogen-vacancy center in diamond under ambient conditions. This provides a promising and powerful tool for large-scale quantum computing under realistic, noisy experimental conditions.