A primary challenge in quantum science and technology is to isolate the fragile quantum states from their environment in order to prevent the irreversible leakage of energy and information which causes decoherence. In the late 1990s, however, a new paradigm emerged, in which the environment itself, as well as the coupling to this environment of the quantum state, are engineered in ways which, counterintuitively, facilitate the creation and stabilization of desired quantum properties. This paradigm, coined reservoir engineering, has been pursued experimentally in various implementations, in which the states of trapped ions, atomic clouds or artificial atoms based on superconducting circuits were driven into a desired target state using a dissipative reservoir. In all these cases, the cold electromagnetic environment served as the engineered reservoir, capitalizing on the tremendous progress in the ability to shape the modes of the electromagnetic field using masers and lasers. In optomechanics, which is the study of the coupling between light and mechanical motion, a similar scenario has been prevalent. Light is used to read out and control the mechanical motion, and in the past few years, various optomechanical architectures both in the optical and microwave domain have enabled to push mechanical systems into the quantum regime. These results can be interpreted in the context of reservoir engineering: cooling and many other optomechanical phenomena exploit the cold, dissipative nature of light. This thesis reports on the development of a multimode superconducting circuit with a mechanically compliant element - fitting into the field of circuit cavity electromechanics -, with which we pursue two themes. In the first set of experiments, reversing the roles of dissipation described above, we engineer the mechanical oscillator into a cold, dissipative environment for microwave light. The mechanical element is the fundamental mode of a free-standing top electrode of a capacitor, 100 nm thick and 32 micron in diameter made of aluminum with an effective mass of around 170 pg, vibrating at a resonance frequency of 5.5 MHz. The dissipative mechanical reservoir is prepared using an auxiliary microwave mode with engineered parameters.We utilize it to control the properties - in particular, the susceptibility - of the electromagnetic field and to perform low-noise amplification close to the quantum limit. The noise analysis reveals that the reservoir is close to its quantum ground state with a mean thermal occupation number well below 1, demonstrating its utility as a resource in the quantum regime. We also show that the system can be driven to the parametric instability threshold, above which self-sustained oscillations of the microwave field (masing) is observed. Finally, we demonstrate injection locking of the maser using an external seed pump. In a second set of experiments, a similar electromechanical circuit is used to implement a microwave isolator based on optomechanical interactions. The overarching theme is that dissipation of the mechanical oscillator, albeit intrinsic and not engineered via an auxiliary mode s a key ingredient for the device to function as a nonreciprocal frequency converter and isolator. In these experiments, an additional mechanical mode is used, such that a 4-mode optomechanical plaquette is realized.
A primary challenge in quantum science and technology is to isolate the fragile quantum states from their environment in order to prevent the irreversible leakage of energy and information which causes decoherence. In the late 1990s, however, a new paradigm emerged, in which the environment itself, as well as the coupling to this environment of the quantum state, are engineered in ways which, counterintuitively, facilitate the creation and stabilization of desired quantum properties. This paradigm, coined reservoir engineering, has been pursued experimentally in various implementations, in which the states of trapped ions, atomic clouds or artificial atoms based on superconducting circuits were driven into a desired target state using a dissipative reservoir. In all these cases, the cold electromagnetic environment served as the engineered reservoir, capitalizing on the tremendous progress in the ability to shape the modes of the electromagnetic field using masers and lasers. In optomechanics, which is the study of the coupling between light and mechanical motion, a similar scenario has been prevalent. Light is used to read out and control the mechanical motion, and in the past few years, various optomechanical architectures both in the optical and microwave domain have enabled to push mechanical systems into the quantum regime. These results can be interpreted in the context of reservoir engineering: cooling and many other optomechanical phenomena exploit the cold, dissipative nature of light. This thesis reports on the development of a multimode superconducting circuit with a mechanically compliant element - fitting into the field of circuit cavity electromechanics -, with which we pursue two themes. In the first set of experiments, reversing the roles of dissipation described above, we engineer the mechanical oscillator into a cold, dissipative environment for microwave light. The mechanical element is the fundamental mode of a free-standing top electrode of a capacitor, 100 nm thick and 32 micron in diameter made of aluminum with an effective mass of around 170 pg, vibrating at a resonance frequency of 5.5 MHz. The dissipative mechanical reservoir is prepared using an auxiliary microwave mode with engineered parameters.We utilize it to control the properties - in particular, the susceptibility - of the electromagnetic field and to perform low-noise amplification close to the quantum limit. The noise analysis reveals that the reservoir is close to its quantum ground state with a mean thermal occupation number well below 1, demonstrating its utility as a resource in the quantum regime. We also show that the system can be driven to the parametric instability threshold, above which self-sustained oscillations of the microwave field (masing) is observed. Finally, we demonstrate injection locking of the maser using an external seed pump. In a second set of experiments, a similar electromechanical circuit is used to implement a microwave isolator based on optomechanical interactions. The overarching theme is that dissipation of the mechanical oscillator, albeit intrinsic and not engineered via an auxiliary mode s a key ingredient for the device to function as a nonreciprocal frequency converter and isolator. In these experiments, an additional mechanical mode is used, such that a 4-mode optomechanical plaquette is realized.
Isolation of a system from its environment is often desirable; however, dissipation can also be a useful resource. Remarkably, engineered dissipation enables the preparation and stabilization of quantum states of atoms, ions or superconducting qubits. This is achieved by a suitably engineered coupling to a dissipative cold reservoir formed by electromagnetic modes. Similarly, in the field of cavity electro- and optomechanics the control over mechanical oscillators utilizes the inherently cold dissipative nature of the electromagnetic degree of freedom. Breaking from this paradigm, recent theoretical work has considered the opposite regime in which the dissipation of the mechanical oscillator dominates and provides a cold dissipative reservoir to the electromagnetic mode. Here we report the experimental realization of this reversed dissipation regime in a microwave cavity optomechanical system and realize a quasi-instantaneous, cold reservoir for microwave light. We evidence this regime by decreasing or increasing the damping rate of the cavity on demand, that corresponds to amplification and de-amplification of the microwave field. Additionally, we observe the onset of parametric instability, i.e. the stimulated emission of microwaves (masing). Moreover, we employ the engineered cold reservoir to implement a low-noise, large-gain phase-preserving amplifier. Beyond offering the manipulation of microwave fields, such a dissipative reservoir for microwave light, when coupled to multiple cavity modes, forms the basis of microwave entanglement schemes, electromechanical amplifiers with unlimited gain-bandwidth product and dissipative quantum phase transitions. Equally important, combining such reservoir-mediated interaction with coherent dynamics allows for the realization of non-reciprocal devices, which would extend the available toolbox of quantum-limited microwave manipulation techniques.
Harmonic oscillators might be one of the most fundamental entities described by physics. Yet they stay relevant in recent research. The topological properties associated with exceptional points that can occur when two modes interact have generated much interest in recent years. Harmonic oscillators are also at the heart of new quantum technological applications: the long lifetime of high-Q resonators make them advantageous as quantum memories, and they are employed for narrowband processing of quantum signals, as in Josephson parametric amplifiers. The goal of this thesis is to explore different fundamental regimes of two coupled harmonic oscillators using cavity optomechanics as the experimen- tal platform. With consistent progress in attaining ever increasing Q factors, mechanical and electromagnetic resonators realize near-ideal harmonic oscillators. By parametrically modulating the nonlinear optomechanical interaction between them, an effective linear coupling is achieved, which is tunable in strength and in the relative frequencies of the two modes. Thus cavity optomechanics provides a framework with excellent control over system parameters for the study of two coupled harmonic modes. The specific optomechanical implementation employed are superconducting circuits with the vibrating top plate of a capacitor as the mechanical element. Multimode optomechanical circuits are realized, with two microwave modes interacting with one or two mechanical oscillators. The supplementary modes serve either as intermediaries in the relation of the two modes of interest, or as auxiliaries used to control a parameter of the system. Three main experimental results are achieved. First, an auxiliary microwave mode allows the engineering of the effective dissipation rate of a mechanical oscillator. The latter then acts as a reservoir for the main microwave mode with which it interacts. The microwave mode susceptibility can be tuned, resulting in an instability akin to that of a maser and in resonant amplification of incoming microwave signals with an added noise close to the quantum minimum. Second, we study the conditions for a nonreciprocal interaction between two microwave modes, when the information flows in one direction but not in the other. The two modes interact through two mechanical oscillators, leading to frequency conversion between the two cavities. Dissipation in the mechanical modes is essential to the scheme in two ways: it provides a reciprocal phase necessary for the interference and eliminates the unwanted signals. Third, level attraction between a microwave and a mechanical mode is demonstrated, where the eigenfrequencies of the system are drawn closer as the result of interaction, rather distancing themselves as in the more usual case of level repulsion. The phenomenon is theoretically connected to exceptional points, and a general classification of the possible regimes of interaction between two harmonic modes is exposed, including level repulsion and attraction as special cases.
In the late 1960s and early 1970s, the development of mechanical resonators was pushed forward in efforts to record gravitational waves. In order to push down the limit of the smallest detectable force, the radiation circulating in a Fabry-Perot cavity was demonstrated to modify the damping of the cavity end-mirror suspended to act as a mechanical resonator. A few years later, motivated by the study of the internal properties of atoms and ions, the radiation pressure of light was realized as a means to cool atomic motion. In the following years, the ground-state cooling of ion motion was achieved in landmark studies. For mechanical resonators parametrically coupled to Fabry-Perot cavities, it took much longer to reach quantum ground-state cooling, both in the microwave domain, where the original experiments took place, and in the optical domain. Ground-state cooling in both regimes was reached by three groups during the preparation of this thesis and was largely due to advancements in the fabrication methods. \n \nGround-state cooling allows, in principle, the quantum nature of mechanical resonators to be probed and harnessed. Microwave domain devices, which are focused on in this thesis, have the advantage that nonlinear elements (superconducting quantum bits, qubits) are readily available. These elements enable nonclassical state preparation of the qubit and the subsequent transfer to the microwave cavity. The goal is to transfer these quantum states to mechanical resonators. This would allow mechanics to be used as a quantum mechanical memory in quantum information processing thanks to their long lifetimes. \n \nIn this thesis, various aspects of microwave domain circuit optomechanics are studied. The main goal of this thesis is to study how to enhance the coupling between a quantum regime microwave device and a mechanical resonator by using Josephson junction –based qubits. Coherent interaction between a superconducting qubit and a classical driven mechanical field is demonstrated. The analysis presented in this thesis predicts that ground-state cooling and coherent state transfer is possible in the single-phonon regime with transmon-regime qubits. Also, traditional linear optomechanical systems are considered in which the mechanical resonator is coupled to an electrical resonator. Such systems exhibit a rich spectrum of phenomena from which the quantum-limited amplification and multimode effects are considered in this thesis. It is shown that the system operates near quantum-limited amplification, which could be reached if the mechanical resonator was in the ground state.
Superconducting circuits are a powerful platform for studying and controlling the interaction between light and matter at the quantum level. In these systems, superconducting qubits act as artificial atoms (with matter-like degrees of freedom), whereas microwave resonators play the role of oscillators hosting photons (with photonic-like degrees of freedom). A major advantage of this platform is the ability to tailor the electromagnetic environment to which the qubits are coupled. This degree of control makes it possible to realize well-known quantum optics models, like the Jaynes-Cummings model, as well as more complex systems, like quantum electrodynamics close to a bandgap. In this thesis, we engineer structured electromagnetic environments and couple superconducting qubits to them to experimentally study their interaction. By coupling multiple microwave resonators together, we create a metamaterial. When an atom interacts with the metamaterial, an atom-photon bound state emerges. We observe the dynamics of the creation and dissolution of the atom-photon bound state, as well as the spectral content of its photonic component, for the first time to our knowledge.Our metamaterial is intrinsically nonlinear because each resonator is formed by an array of Josephson junctions to serve as an inductor. When the system is pumped, its phase diagram exhibits multimode dissipative phase transitions with timescales on the order of hundred seconds. There is ongoing theoretical debate about whether such phase transitions can occur in one-dimensional systems, a question we address and resolve in this work.Furthermore, we engineer qubit decay using two different approaches. In the first one, we engineer the decay of two coupled atoms to two waveguides by using a symmetric–antisymmetric coupling configuration. This approach enables selective coupling to bright and dark states of the system. In the second one, we suppress the Purcell decay of a qubit using a compact lumped-element Purcell filter. In addition, we characterize the Purcell decay by employing an auxiliary superconducting qubit as a sensitive power detector directly coupled to the feedline waveguide used for the qubit readout.In summary, this thesis presents three different methods for controlling light–matter interactions in structured quantum systems, including decay suppression with both Purcell filters and symmetry-selective couplings. The thesis also introduces new experimental techniques for probing atom-photon bound states and provides direct evidence of collective phenomena in driven-dissipative quantum metamaterials.
Engineered quantum systems are poised to revolutionize information science in the near future. A persistent challenge in applied quantum technology is creating controllable, quantum interactions while preventing information loss to the environment, decoherence. In this thesis, we realize mesoscopic superconducting circuits whose macroscopic collective degrees of freedom, such as voltages and currents, behave quantum mechanically. We couple these mesoscopic devices to microwave cavities forming a cavity quantum electrodynamics (QED) architecture comprised entirely of circuit elements. This application of cavity QED is dubbed Circuit QED and is an interdisciplinary field seated at the intersection of electrical engineering, superconductivity, quantum optics, and quantum information science. Two popular methods for taming active quantum systems in the presence of decoherence are discrete feedback conditioned on an ancillary system or quantum reservoir engineering. Quantum reservoir engineering maintains a desired subset of a Hilbert space through a combination of drives and designed entropy evacuation. Circuit QED provides a favorable platform for investigating quantum reservoir engineering proposals. A major advancement of this thesis is the development of a quantum reservoir engineering protocol which maintains the quantum state of a microwave cavity in the presence of decoherence. This thesis synthesizes strongly coupled, coherent devices whose solutions to its driven, dissipative Hamiltonian are predicted a priori. This work lays the foundation for future advancements in cavity centered quantum reservoir engineering protocols realizing hardware efficient circuit QED designs.
Microscale and nanoscale mechanical resonators have been used in advanced technological applications, from high precision time keeping and mass sensing, to processing high frequency signals in mobile communications. In the last few decades, they have been an important part of progress in the field of quantum information and metrology and have been proposed as quantum memories or transducers for measuring or connecting different types of quantum systems. The field of cavity optomechanics and electromechanics is concerned with coupling the electromagnetic field of a resonant optical cavity or electrical circuit to mechanical motion. These systems provide potential means to control and engineer the state of a mechanical object at the quantum level. This thesis contains the description of mechanical systems in megahertz to a few hundred megahertz frequency range formed by nano-fabricating photonic, phononic, and electrical circuits on a chip. These structures are designed to provide a large radiation pressure coupling between mechanical motion and electromagnetic fields to address and manipulate motional degrees of freedom. Qualitatively novel quantum effects are expected when one takes a step beyond linear coupling and exploits higher order interactions. To that end, we integrate electrical, mechanical and photonic structures in a multimode photonic crystal structure to observe "x2-coupling", where the optical cavity frequency is coupled to the square of the mechanical displacement. Moreover, we have developed two integrated on-chip platforms based on Si3N4 and Si nanomembranes capable of interfacing superconducting qubits and optical photons and realizing reversible microwave-to-optical conversion. We employ radiation pressure to cool these mechanical resonators to their quantum ground state. Finally, we demonstrate a form of electromechanical crystal for coupling microwave photons and hypersonic phonons of frequency ωm/2π = 0.425 GHz by capacitively coupling a phononic crystal acoustic cavity to a superconducting microwave resonator. Moving to higher frequency acoustic cavities not only facilitates the integration of electromechanical circuits and nanophotonic systems capable of operation in the resolved sideband limit of optomechanics for noise-free quantum signal conversion, but it opens up the possibility of using phonons as information carriers via phononic circuits. Utilizing a two-photon resonance condition for efficient microwave pumping and phononic bandgap shield to eliminate acoustic radiation, we achieve large cooperative electromechanical coupling (C ≈ 30) and intrinsic decay time of 2.3 ms. Moreover, electrical read-out of the phonon occupancy shows that the acoustic mode thermalizes close to its quantum ground-state of motion (phonon occupancy nm=1.5) at a fridge temperature of Tf = 10 mK. We conclude by considering several designs and fabrication improvements to the hypersonic electromechanical crystals that would enable them to perform quantum conversion between the electrical and acoustic domain.