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Nature Communications

Highly-efficient extraction of entangled photons from quantum dots using a broadband optical antenna

Yan Chen, Michael Zopf, Robert Keil, Fei Ding, Oliver G. Schmidt

Published Jul 25, 2018• 184 citations
Publisher

Abstract

Many quantum photonic technologies require the efficient generation of entangled pairs of photons, but to date there have been few ways to produce them reliably. Sources based on parametric down conversion operate at very low efficiency per pulse due to the probabilistic generation process. Semiconductor quantum dots can emit single pairs of entangled photons deterministically but they fall short due to the extremely low-extraction efficiency. Strategies for extracting single photons from quantum dots, such as embedding them in narrowband optical cavities, are difficult to translate to entangled photons. Here, we build a broadband optical antenna with an extraction efficiency of 65% ± 4% and demonstrate a highly-efficient entangled-photon source by collecting strongly entangled photons (fidelity of 0.9) at a pair efficiency of 0.372 ± 0.002 per pulse. The high brightness achieved by our source represents a step forward in the development of optical quantum technologies.

DOI
10.1038/s41467-018-05456-2

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Many quantum photonic technologies require the efficient generation of entangled pairs of photons, but to date there have been few ways to produce them reliably. Sources based on parametric down conversion operate at very low efficiency per pulse due to the probabilistic generation process. Semiconductor quantum dots can emit single pairs of entangled photons deterministically but they fall short due to the extremely low-extraction efficiency. Strategies for extracting single photons from quantum dots, such as embedding them in narrowband optical cavities, are difficult to translate to entangled photons. Here, we build a broadband optical antenna with an extraction efficiency of 65% ± 4% and demonstrate a highly-efficient entangled-photon source by collecting strongly entangled photons (fidelity of 0.9) at a pair efficiency of 0.372 ± 0.002 per pulse. The high brightness achieved by our source represents a step forward in the development of optical quantum technologies.
Long-distance fiber-based quantum communication relies on efficient non-classical light sources operating at telecommunication wavelengths. Semiconductor quantum dots are promising candidates for on-demand generation of single photons and entangled photon pairs for such applications. However, their brightness is strongly limited due to total internal reflection at the semiconductor/vacuum interface. Here we overcome this limitation using a dielectric antenna structure. The non-classical light source consists of a gallium phosphide solid immersion lens in combination with a quantum dot nanomembrane emitting single photons in the telecom O-band. With this device, the photon extraction is strongly increased in a broad spectral range. A brightness of 17 % (numerical aperture of 0.6) is obtained experimentally, with a single photon purity of g ( 2 ) ( 0 ) = 0.049 ± 0.02 at saturation power. This brings the practical implementation of quantum communication networks one step closer.
The quick development of quantum technologies and quantum communication demands a continuous search for more efficient and with higher performance quantum sources and devices. In particular, quantum dots are firmly established sources of single photon emitters and entangled photon pairs, with entanglement of photons emitted by a single quantum dot probed in polarization[1], time-bin[2] and hyperentanglement[3]. Although spontaneous parametric down conversion sources (SPDC) are widely used as entangled photon sources with the highest values of entanglement[4], are being reached by quantum dot devices[5]. With similar quality as SPDC sources, QDs however stand out as sources with sub-Poissonian statistics, essential for safe quantum communication. Still, most of the quantum dots devices exhibit low extraction efficiencies. Attempts to maximize the extraction efficiency involve sophisticated engineered photonic systems[6,7]. Furthermore, the accurate alignment of the quantum dot-cavity system is crucial for an effective quantum dotcavity coupling and hence an emission enhancement into free space[8]. All of this implies the need of intricated nanofabrication processes. Here we present a simple, scalable photonic device that grants efficient creation of entangled photon pairs from InAs quantum dots. The device, spontaneously formed during the growth process, is based on pairs of bottom/top distributed bragg reflectors (DBRs). A propagating deformation in the DBRs, leads to the formation of self-aligned dimples on top of the QDs, resulting in a self-aligned quantum-dot cavity system[9]. Therefore, costly and complex deterministic nanofabrication techniques are not required. In this work, the device performance was characterized, showing experimental collection efficiencies of 0.17, with theoretically pair extraction efficiencies above 0.45. Furthermore, a Purcell enhancement up to 1.7 was obtained. Finally, the device potential to generate time-bin entangled photons was investigated performing state tomography measurements. The subsequent reconstruction of the density matrix yields a concurrence of 0.70(10) and a fidelity of 0.84(5).
An outstanding goal in quantum optics and scalable photonic quantum technology is to develop a source that each time emits one and only one entangled photon pair with simultaneously high entanglement fidelity, extraction efficiency, and photon indistinguishability. By coherent two-photon excitation of a single InGaAs quantum dot coupled to a circular Bragg grating bull's-eye cavity with a broadband high Purcell factor of up to 11.3, we generate entangled photon pairs with a state fidelity of 0.90(1), pair generation rate of 0.59(1), pair extraction efficiency of 0.62(6), and photon indistinguishability of 0.90(1) simultaneously. Our work will open up many applications in high-efficiency multiphoton experiments and solid-state quantum repeaters.
A bright source of on-demand entangled photons is needed for quantum networks. A single quantum dot in a site-selected nanowire waveguide is a promising candidate for realizing such sources. However, such sources are associated with poor single-photon indistinguishability, limiting their applicability in quantum networks. A common approach for enhancing the single-photon indistinguishability in quantum dot-based entangled photon sources is to implement a broadband optical cavity. Achieving a high-Purcell cavity while retaining the advantages of the nanowire, such as directional emission, a broad operational bandwidth, and high light extraction efficiency, has been a significant challenge. Here, we propose a nanowire cavity based on quasi-bound states in the continuum formed by the strong coupling of two resonant optical modes. We numerically predict this design to support a cavity mode with 4 nm bandwidth and a Purcell enhancement of $\sim$17. This cavity mode enables a directional far-field emission profile (88% overlap with a Gaussian) with a light extraction efficiency of $\sim$74%. Our solution opens up a route for generating entangled photon pairs with enhanced extraction efficiency and single-photon indistinguishability for the practical realization of quantum networks.
The generation of entangled photon pairs is a fundamental cornerstone of quantum optics, and an essential technology in the high profile field of quantum communication and computing. Currently the most widely used techniques for generating entangled photon pairs are nonlinear optical processes, such as parametric down conversion, which produce a probabilistic number of pairs per excitation cycle. Such a source is of limited use in quantum information/processing applications where a regular stream of single entangled photon pairs is usually required. We have produced such a triggered source from a semiconductor device for the first time, using a two-photon cascade in a single quantum dots, demonstrating efficiencies up to 70%, close to the level required for useful applications. Single quantum dots could prove to be the first robust and compact triggered source of entangled photons.
Entangled photon pairs are a ubiquitous resource in quantum technologies, used in quantum key distribution and quantum networking as well as fundamental tests of non-locality. For scalable quantum networks, pairs that are indistinguishable in all unentangled degrees of freedom are essential, as they enable high-fidelity entanglement swapping across network nodes. To date the most-studied sources of "swappable" entangled photon pairs have been based on spontaneous parametric down-conversion (SPDC) in non-linear crystals. However, the probabilistic nature and unavoidable trade-off between brightness and unwanted multi-photon emission limits their performance in lossy channels. Here, we demonstrate a high-fidelity source of "swappable" entangled photon pairs using a semiconductor quantum dot (QD) coupled to a tunable microcavity. By actively modulating the QD emission between orthogonal polarisation states, delaying one path in a low-loss Herriott cell, and recombining the two on a balanced beam splitter, we generate entangled photon pairs with a fidelity of 96.1±0.596.1\pm0.596.1±0.5 %. We identify and mitigate fidelity-limiting factors, achieving a maximum fidelity of 98.1±0.598.1\pm0.598.1±0.5 % through time-resolved post-selection. The scheme suppresses residual multi-photon events concentrated near the excitation pulse and has only a modest impact on the rate. Furthermore, the photons are mutually indistinguishable, enabling efficient entanglement swapping. Our results establish semiconductor QDs as a viable platform for quantum network-compatible swappable entangled photon pair generation, with feasible entanglement generation rates exceeding 0.5 Gpairs/s.