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Observation of a Dynamical Phase Transition in the Collective Heisenberg Model

Scott Smale, Peiru He, Ben A. Olsen, Kenneth G. Jackson, Haille Sharum, Stefan Trotzky, Jamir Marino, Ana María Rey, Joseph H. Thywissen

Published Jun 28, 2018• 3 citations
OpenAlex

Abstract

Ultracold atoms, benefiting from long-lived coherence and controllable interactions, offer an ideal system to shed light on the organizing principles of out-of-equilibrium quantum systems. Here, we investigate a dynamical phase transition from a state with ferromagnetic order to a demagnetized state in a quantum simulator of the collective Heisenberg model with an inhomogeneous axial field. Two hyperfine states of fermionic potassium atoms encode the spin degrees of freedom, while single-particle oscillator modes serve as lattice sites. We benchmark the simulator using detailed comparisons to theory and by testing the reversibility of the collective dynamics. Our observations open a route for applications of large controllable fermionic ensembles to enhanced metrology and quantum technologies.

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This thesis reports on the deterministic preparation of magnetically ordered states in systems of few fermionic atoms. We follow the concept of quantum simulation and use 6Li atoms in two different hyperfine states to mimic the behavior of electrons in a solidstate system. In a first experiment, we simulate the two-site Hubbard model by using two atoms in an isolated double-well potential. We prepare the two-particle ground state of this model with a fidelity exceeding 90%. By introducing strong repulsive interactions, we are able to realize a pure spin model and describe the energy spectrum with a two-site Heisenberg Hamiltonian. In a second experiment, we realize Heisenberg spin chains of up to four atoms in a single strongly-elongated trapping potential. Here, the atoms self-align along the potential axis due to strong repulsive interactions. We introduce two novel measurement techniques to identify the state of the spin chains and thereby confirm that we can deterministically prepare antiferromagnetic ground-state systems. This constitutes the first observation of quantum magnetism with fermionic atoms that exceeds nearest-neighbor correlations. Both the double-well system and the spin chains can be seen as building blocks of larger ground-state spin systems. Their deterministic preparation therefore opens up a new bottom-up approach to the experimental realization of quantum many-body systems with ultracold atoms.

•Jan 1, 2015•1 citation
Ultracold atoms, benefiting from long-lived coherence and controllable interactions, offer an ideal system to shed light on the organizing principles of out-of-equilibrium quantum systems. Here, we investigate a dynamical phase transition from a state with ferromagnetic order to a demagnetized state in a quantum simulator of the collective Heisenberg model with an inhomogeneous axial field. Two hyperfine states of fermionic potassium atoms encode the spin degrees of freedom, while single-particle oscillator modes serve as lattice sites. We benchmark the simulator using detailed comparisons to theory and by testing the reversibility of the collective dynamics. Our observations open a route for applications of large controllable fermionic ensembles to enhanced metrology and quantum technologies.
A proposed paradigm for out-of-equilibrium quantum systems is that an analog of quantum phase transitions exists between parameter regimes of qualitatively distinct time-dependent behavior. Here, we present evidence of such a transition between dynamical phases in a cold-atom quantum simulator of the collective Heisenberg model. Our simulator encodes spin in the hyperfine states of ultracold fermionic potassium. Atoms are pinned in a network of single-particle modes, whose spatial extent emulates the long-range interactions of traditional quantum magnets. We find that below a critical interaction strength, magnetization of an initially polarized fermionic gas decays quickly, while above the transition point, the magnetization becomes long-lived because of an energy gap that protects against dephasing by the inhomogeneous axial field. Our quantum simulation reveals a nonequilibrium transition predicted to exist but not yet directly observed in quenched s-wave superconductors.
Quantum simulation with ultracold atoms has become a powerful technique to gain insight into interacting many-body systems. In particular, the possibility to study nonequilibrium dynamics offers a unique pathway to understand correlations and excitations in strongly interacting quantum matter. So far, coherent nonequilibrium dynamics has exclusively been observed in ultracold many-body systems of bosonic atoms. Here we report on the observation of coherent quench dynamics of fermionic atoms. A metallic state of ultracold spin-polarized fermions is prepared along with a Bose–Einstein condensate in a shallow three-dimensional optical lattice. After a quench that suppresses tunnelling between lattice sites for both the fermions and the bosons, we observe long-lived coherent oscillations in the fermionic momentum distribution, with a period that is determined solely by the Fermi–Bose interaction energy. Our results show that coherent quench dynamics can serve as a sensitive probe for correlations in delocalized fermionic quantum states and for quantum metrology. In ultracold quantum gases, coherent nonequilibrium dynamics has been observed for bosons, but remained elusive in fermionic systems. Here, Will et al. demonstrate coherent quench dynamics in a hybrid quantum system composed of a metallic state of fermionic atoms and a Bose–Einstein condensate.
Strongly interacting many-body systems exhibit collective properties that emerge from complex correlations among microscopic degrees of freedom. These cooperative phenomena govern the non-equilibrium response of quantum systems, with relevance ranging from condensed matter physics to quantum field theories describing fundamental aspects of our universe. Understanding such emergent dynamics from first principles remains one of the central challenges in quantum many-body physics. Here we report on the observation of collective cluster nucleation dynamics following quenches in 2D ferromagnetic quantum Ising systems implemented in an atomic Rydberg array. Our experiments reveal two distinct regimes: In the confined regime, we observe an energy-dependent cluster size, revealing large collective clusters exceeding ten spins. In contrast, the deconfined regime is characterized by kinetically constrained, avalanche-like nucleation dynamics involving the entire system. Our findings establish a new frontier for quantum simulations with Rydberg arrays, enabling controlled exploration of non-equilibrium phenomena previously out of reach. Beyond advancing experimental capabilities, they provide fundamental insights into highly correlated processes with implications that reach from quantum magnetism and glassy dynamics to cosmological models of the early universe.
Many-body physics describes phenomena that cannot be understood by looking only at the constituents of a system1. Striking examples are broken symmetry, phase transitions and collective excitations2. To understand how such collective behaviour emerges as a system is gradually assembled from individual particles has been a goal in atomic, nuclear and solid-state physics for decades3–6. Here we observe the few-body precursor of a quantum phase transition from a normal to a superfluid phase. The transition is signalled by the softening of the mode associated with amplitude vibrations of the order parameter, usually referred to as a Higgs mode7. We achieve fine control over ultracold fermions confined to two-dimensional harmonic potentials and prepare closed-shell configurations of 2, 6 and 12 fermionic atoms in the ground state with high fidelity. Spectroscopy is then performed on our mesoscopic system while tuning the pair energy from zero to a value larger than the shell spacing. Using full atom counting statistics, we find the lowest resonance to consist of coherently excited pairs only. The distinct non-monotonic interaction dependence of this many-body excitation, combined with comparison with numerical calculations allows us to identify it as the precursor of the Higgs mode. Our atomic simulator provides a way to study the emergence of collective phenomena and the thermodynamic limit, particle by particle. An atomic simulator formed of a few ultracold fermionic atoms trapped in a two-dimensional harmonic potential exhibits precursors of a quantum phase transition, revealing the onset of collective quantum many-body phenomena in a few-body system.
Using an ensemble of atoms in an optical cavity, we engineer a family of nonlocal Heisenberg Hamiltonians with continuously tunable anisotropy of the spin-spin couplings. We thus gain access to a rich phase diagram, including a paramagnetic-to-ferromagnetic Ising phase transition that manifests as a diverging magnetic susceptibility at the critical point. The susceptibility displays a symmetry between Ising interactions and XY (spin-exchange) interactions of the opposite sign, which is indicative of the spatially extended atomic system behaving as a single collective spin. Images of the magnetization dynamics show that spin-exchange interactions protect the coherence of the collective spin, even against inhomogeneous fields that completely dephase the noninteracting and Ising systems. Our results underscore prospects for harnessing spin-exchange interactions to enhance the robustness of spin squeezing protocols.
This thesis reports on the deterministic preparation of magnetically ordered states in systems of few fermionic atoms. We follow the concept of quantum simulation and use 6Li atoms in two different hyperfine states to mimic the behavior of electrons in a solidstate system. In a first experiment, we simulate the two-site Hubbard model by using two atoms in an isolated double-well potential. We prepare the two-particle ground state of this model with a fidelity exceeding 90%. By introducing strong repulsive interactions, we are able to realize a pure spin model and describe the energy spectrum with a two-site Heisenberg Hamiltonian. In a second experiment, we realize Heisenberg spin chains of up to four atoms in a single strongly-elongated trapping potential. Here, the atoms self-align along the potential axis due to strong repulsive interactions. We introduce two novel measurement techniques to identify the state of the spin chains and thereby confirm that we can deterministically prepare antiferromagnetic ground-state systems. This constitutes the first observation of quantum magnetism with fermionic atoms that exceeds nearest-neighbor correlations. Both the double-well system and the spin chains can be seen as building blocks of larger ground-state spin systems. Their deterministic preparation therefore opens up a new bottom-up approach to the experimental realization of quantum many-body systems with ultracold atoms.