Quantum networks of the future will be required to span the globe and interconnect many different real world systems employed by different commercial, academic, and government users. Thus, an important measure of such a network's capacity will be its ability to interact with and distribute entanglement among different mediums and devices with potentially disparate properties. Few experiments have to date shown this sort of interconnectivity between different systems with different atomic species. Here I will present our demonstration of a system in which we store two correlated photons in solid state quantum memories implemented in different rare earth ion-doped materials using the atomic frequency comb protocol. The photon pairs are generated through a spontaneous parametric down-conversion process with their wavelengths chosen to be compatible with quantum repeater implementations. One member, with a wavelength at 795 nm, is stored in an Tm:LiNbO3 crystal while, simultaneously, the other member, generated at 1535 nm wavelength, is stored in an amorphous erbium doped optical fiber. The measured cross-correlation function between the recalled photons is g(2) = 16 +/- 2, which verifies that the non-classical correlations are preserved and were present during the storage of both photons. The two storage mediums are diverse not only in terms of their different photon acceptance wavelengths, but also with regards to the material properties as hosts for the dopant rare-earth ions. Our results show that quantum nodes and networks based on fundamentally different systems can be interfaced to distribute entanglement.
Quantum networks of the future will be required to span the globe and interconnect many different real world systems employed by different commercial, academic, and government users. Thus, an important measure of such a network's capacity will be its ability to interact with and distribute entanglement among different mediums and devices with potentially disparate properties. Few experiments have to date shown this sort of interconnectivity between different systems with different atomic species. Here I will present our demonstration of a system in which we store two correlated photons in solid state quantum memories implemented in different rare earth ion-doped materials using the atomic frequency comb protocol. The photon pairs are generated through a spontaneous parametric down-conversion process with their wavelengths chosen to be compatible with quantum repeater implementations. One member, with a wavelength at 795 nm, is stored in an Tm:LiNbO3 crystal while, simultaneously, the other member, generated at 1535 nm wavelength, is stored in an amorphous erbium doped optical fiber. The measured cross-correlation function between the recalled photons is g(2) = 16 +/- 2, which verifies that the non-classical correlations are preserved and were present during the storage of both photons. The two storage mediums are diverse not only in terms of their different photon acceptance wavelengths, but also with regards to the material properties as hosts for the dopant rare-earth ions. Our results show that quantum nodes and networks based on fundamentally different systems can be interfaced to distribute entanglement.
(English) Future networks for quantum communication will require a new form of technology in order to operate over long distances. The no-cloning theorem precludes the use of amplification, so quantum repeater schemes have been proposed to achieve long-distance quantum communication through the distribution of entanglement. A key device for this setup is a quantum memory, which is required in order to store entanglement and synchronise its distribution. Among the many physical systems than can be used as a quantum memory, rare-earth ion-doped crystals stand out due to their long coherence times and potential for multiplexing and integration. This thesis reports the use of one such system, Pr3+:Y2SiO5, as a quantum memory using the atomic frequency comb (AFC) protocol. Building on previous work, we improved the performance of the memory to be able to demonstrate light-matter entanglement with a telecommunications wavelength photon and the quantum memory, for both a bulk memory and an integrated version. To measure light-matter entanglement, we use photon pairs generated through cavity-enhanced spontaneous parametric down conversion, where one photon (the signal) is stored in the memory and the other (the idler) is at a telecommunications wavelength. These photon pairs exhibit energy-time entanglement, which we analyse in the time basis using fibre- and AFC-based Mach-Zehnder interferometers. In the first experiment, we demonstrate light-matter entanglement where the bulk quantum memory is used with on-demand retrieval via storage in a spin-wave. We measure interference fringes with average visibilities of 89(2)% for AFC storage, and 70(3)% for spin-wave storage, sufficient to demonstrate entanglement. This is the first such demonstration using an on-demand multimode solid-state memory and telecom photon. We show that entanglement is maintained for up to 47.7 µs of storage. These results were made possible through improvements in the AFC efficiency and the noise filtering. Furthermore, we perform on-demand storage and retrieval of up to 30 temporal modes. We take the next step towards implementing our system in a real world scenario by measuring entanglement over a distance. To do so, we send the idler photons through both optical fibre spools and deployed fibre in the metropolitan area of Barcelona, Spain, while the photon detection still occurs in the same lab. The resulting visibilities (80% or higher) demonstrate that the photonic qubit does not decohere during transmission through the optical fibre. We then decouple the photon creation and detection by measuring non-classical correlations between signal photons detected in the lab, and idler photons detected 16 km away (44 km in fibre) in a different location. The final experiment uses a fibre-integrated memory for light-matter entanglement. We use a Pr3+:Y2SiO5 crystal containing a Type I laser-written waveguide, interfaced directly with optical fibre. The fibre-integration allows for improved transmission and AFC efficiency compared to a free-space coupled waveguide memory. To analyse the performance of the memory, we demonstrate non-classical correlations for storage times up to 28 µs. We perform qubit tomography in the time basis for storage times of 3 and 10 µs, measuring two-qubit fidelities of 86(2)% and 86(4)%, respectively, demonstrating storage of entanglement. These experiments demonstrate the potential of our system for use as part of a quantum repeater, with many opportunities for further improvement to the storage time, efficiency, and multiplexing capability.
Advanced applications of quantum information science, such as long-distance quantum communication based on quantum repeaters, require photons to be interfaced with different devices. These devices, such as single photon detectors, quantum memories, quantum signal processors, and linear optical elements, may be integrated on a single chip to enable efficient, robust and scalable implementations. With aim of constructing a quantum repeater, and towards realizing integrated optical quantum memories and signal processors in general, we experimentally develop quantum light-matter interfaces using a cryogenically-cooled rare-earth-ion-doped waveguide, namely thulium-doped lithium niobate (Tm3+:LiNbO3). As the basis for our work, we describe a quantum repeater architecture that uses spectral multiplexing and quantum memories that operate with a fixed storage time. Our repeater architecture promises efficient operation, is compatible with the properties of cryogenically-cooled rare-earth-ion-doped crystals, and simplifies the demands of quantum memories compared to other architectures. To demonstrate the feasibility of our repeater design, we utilize our light-matter interface as a quantum memory to perform several experimental demonstrations. These include high-fidelity storage and retrieval of 26 spectrally-multiplexed quantum bits encoded into single-photon-level laser pulses, high-fidelity storage and retrieval of single and entangled photons derived from a photon-pair source, and high-visibility two-photon interference between weak laser pulses that are stored in one or two, separate, quantum memories. The unique properties of our light-matter interface allow us to demonstrate additional protocols that further highlight its promise for integrated quantum signal processing. By combining our Tm3+:LiNbO3 waveguide with a LiNbO3 waveguide phase modulator, we demonstrate operations such as sequencing, filtering, interference, and compression of laser pulses attenuated to the single-photon level. In another experiment, we measure the cross-phase modulation between strong pulses, by which we demonstrate photon-photon interactions that point towards non-destructive measurements of quantum bits. Since the performance of all aforementioned protocols, and future light-matter applications, hinge on the basic spectroscopic properties of our waveguide, we measure these properties at temperatures as low as 800 millikelvin. Our findings, discussed over several attached publications, usher the development of integrated quantum memories and processors for multi-component optical quantum information applications such as repeaters and networks.
The quantum internet, when finally deployed, will enable a plethora of new applications such as theoretically proven secure communication and networked quantum computing, much the same as its classical counterpart whose development began back in the 1990’s. The task of creating a globe-spanning quantum network, however, is proving a rather difficult task due to the detrimental effect of loss on photon transmission. This problem can in theory be solved using so-called quantum repeaters. In one of the most well-known configurations, the long-distance span is divided into smaller segments—so called elementary links—at whose ends pairs of entangled photons are generated. One photon per pair is stored in a quantum memory, and the second member is transmitted via optical fiber to a remote measurement stations positioned at the centre of the segment. There, a joint measurement of the two photons, one from each end, then heralds the distribution of entanglement between the two quantum memories, i.e. heralds entanglement over the elementary link. In the final step, all neighbouring links are combined via a second joint measurement, and end-to-end entanglement is created...
Entangling quantum systems with different characteristics through the exchange of photons is a prerequisite for building future quantum networks. Proving the presence of entanglement between quantum memories for light working at different wavelengths furthers this goal. Here, we report on a series of experiments with a thulium-doped crystal, serving as a quantum memory for 794-nm photons, an erbium-doped fiber, serving as a quantum memory for telecommunication-wavelength photons at 1535 nm, and a source of photon pairs created via spontaneous parametric down-conversion. Characterizing the photons after re-emission from the two memories, we find nonclassical correlations with a cross-correlation coefficient of g(12)((2)) = 53 +/- 8; entanglement preserving storage with input-output fidelity of F-IO approximate to 93 +/- 2%; and nonlocality featuring a violation of the Clauser-Horne-Shimony-Holt Bell inequality with S = 2.6 +/- 0.2. Our proof-of-principle experiment shows that entanglement persists while propagating through different solid-state quantum memories operating at different wavelengths.
Rare-earth-ion doped materials are studied for a quantum information protocol, controlled reversible inhomogeneous broadening, for storing single photons. Coherence properties of Er-doped silicate optical fibers and Er-doped LiNbO3 waveguiding structures are investigated. Spectral hole burning spectroscopy is performed in Erbium and Neodymium doped crystals and spectral tailoring is demonstrated in Nd³?:YVO4. The preservation of information encoded into the relative phase and amplitudes of optical pulses during storage and retrieval in an optical memory based on stimulated photon echo is demonstrated. Furthermore photon echoes stored in spatially separated optical memories in several temporal modes, are retrieved and then combined at a beam splitter. They show almost perfect interference demonstrating both phase preserving storage and indistinguishability of photon echoes. Finally, we report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms and the resulting high fringe visibility implies that the observed spontaneous emission is coherent.